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Electronic states and their dynamics are of critical importance for electronic and optoelectronic applications. Here, we probe various relevant electronic states in monolayer MoS2, such as multiple excitonic Rydberg states and free-particle…

Nuclear electric resonance (NER) spectroscopy is currently experiencing a revival as a tool for nuclear spin-based quantum computing. Compared to magnetic or electric fields, local electron density fluctuations caused by changes in the…

Quantum Physics · Physics 2025-01-30 Johannes K. Krondorfer , Andreas W. Hauser

We report a conceptually straightforward witness that isolates coherent electronic oscillations from their vibronic counterparts in nonlinear optical spectra of molecular aggregates: Coherent oscillations as a function of waiting time in…

Quantum Physics · Physics 2015-06-04 Joel Yuen-Zhou , Jacob J. Krich , Alán Aspuru-Guzik

A consistent semiquantitative theoretical analysis of electronic Raman scattering from many-electron quantum dots under resonance excitation conditions has been performed. The theory is based on random-phase-approximation-like wave…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez , D. J. Lockwood

We use nonlinear pump-probe spectroscopy to study optical excitations in a charge-tunable MoSe$_2$\WS$_2$ moir\'e heterostructure. An intense red-detuned laser pulse creates a photonic dressing of the material by introducing a large virtual…

Strongly Correlated Electrons · Physics 2025-06-02 B. Evrard , H. S. Adlong , A. A. Ghita , T. Uto , L. Ciorciaro , K. Watanabe , T. Taniguchi , M. Kroner , A. İmamoğlu

The analysis of Fourier-transformed scanning-tunneling-microscopy (STM) images with subatomic resolution is a common tool for studying properties of quasiparticle excitations in strongly correlated materials. While Fourier amplitudes are…

Strongly Correlated Electrons · Physics 2016-11-30 Emanuele G. Dalla Torre , Yang He , Eugene Demler

Magneto photoluminescence and excitation spectroscopy are used to probe the excited state spectrum of negatively charged trions in a InGaAs quantum dot. A single dot optical charging device allows us to selectively prepare specific few (1e,…

Mesoscale and Nanoscale Physics · Physics 2012-01-04 Vase Jovanov , Stephan Kapfinger , Gerhard Abstreiter , Jonathan J. Finley

We study the resonance fluorescence properties of an optically active spin 1/2 system, elucidating the effects of a magnetic field on the coherence of the scattered light. We derive a master equation model for this system that reproduces…

The last two decades experimentally affirmed the quantum nature of free electron wavepackets by the rapid development of transmission electron microscopes into ultrafast, quantum-coherent systems. In particular, ultrafast electron pulses…

Optics · Physics 2022-09-30 Roy Shiloh , Tomas Chlouba , Peter Hommelhoff

A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…

The coherent two-dimensional (2D) electronic spectra with respect to the singlet fission (SF) process in organic molecular aggregates are simulated by the Davydov ansatz combined with the Frenkel-Dirac time-dependent variational algorithm.…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Ke-Wei Sun , Yao Yao

The elementary optical excitations in two dimensional semiconductors hosting itinerant electrons are attractive and repulsive polarons -- excitons that are dynamically screened by electrons. Exciton-polarons have hitherto been studied in…

We study intriguing dynamical features of hot Rubidium atoms driven by two light fields. The fields resonantly drive multiple Zeeman states within two hyperfine levels, yielding a cascaded-$\Lambda$ like structure in the frequency space. A…

Quantum Physics · Physics 2025-10-08 Rupak Bag , Sayari Majumder , Saptarishi Chaudhuri , Dibyendu Roy

The proof test and debugging of the multi-pulsed electron accelerator, Dragon-2,requires a thorough comprehension of the quality of the beams. This puts forward a rigid requirement on the measurement system that it should have the ability…

Nonlinear manipulation of nuclear and electron spins is the basis for all advanced methods in magnetic resonance including multidimensional nuclear magnetic and electron spin resonance spectroscopies, magnetic resonance imaging, and in…

The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Joonho Jang , Heun Mo Yoo , Loren Pfeiffer , Ken West , K. W. Baldwin , Raymond Ashoori

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this…

Materials Science · Physics 2015-10-21 Steeve Cronenberger , Denis Scalbert , David Ferrand , Hervé Boukari , Joël Cibert

We show that the low-energy peak in the polarized resonant Raman spectra of quantum wires, which is commonly associated with ``single particle excitations'', can be interpreted as signature of intra-band collective spin excitations. A broad…

Strongly Correlated Electrons · Physics 2009-10-31 Maura Sassetti , Bernhard Kramer

We demonstrate the extension of coherence between all four two-electron spin ground states of an InAs quantum dot molecule (QDM) via non-local suppression of nuclear spin fluctuations in both constituent quantum dots (QDs), while optically…

Mesoscale and Nanoscale Physics · Physics 2016-08-17 Colin M. Chow , Aaron M. Ross , Danny Kim , Daniel Gammon , Allan S. Bracker , L. J. Sham , Duncan G. Steel