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State-of-the-art techniques for simulating deeply supercooled liquids require a high degree of size polydispersity to be effective. While these techniques have enabled great insight into the microscopic dynamics near the glass transition,…

Soft Condensed Matter · Physics 2023-08-10 Ilian Pihlajamaa , Corentin C. L. Laudicina , Liesbeth M. C. Janssen

Many glass-forming fluids exhibit a remarkable thermodynamic scaling in which dynamic properties, such as the viscosity, the relaxation time, and the diffusion constant, can be described under different thermodynamic conditions in terms of…

Soft Condensed Matter · Physics 2015-06-16 Wen-Sheng Xu , Karl F. Freed

We discuss the general link between mode-coupling like equations (which serve as the basis of some recent theories of supercooled liquids) and the dynamical equations governing mean-field spin-glass models, or the dynamics of a particle in…

Condensed Matter · Physics 2015-06-25 Jean-Philippe Bouchaud , Leticia Cugliandolo , Jorge Kurchan , Marc Mézard

We introduce a new quantity to probe the glass transition. This quantity is a linear generalized compressibility which depends solely on the positions of the particles. We have performed a molecular dynamics simulation on a glass forming…

Disordered Systems and Neural Networks · Physics 2009-11-07 Herve M. Carruzzo , Clare C. Yu

We use recently introduced three-point dynamic susceptibilities to obtain an experimental determination of the temperature evolution of the number of molecules, N_corr, that are dynamically correlated during the structural relaxation of…

We use molecular dynamics simulation to study the relationship between structure and dynamics in supercooled binary Lennard--Jones nanoparticles over a range of particle sizes. The glass transition temperature of the nanoparticles is found…

Soft Condensed Matter · Physics 2025-05-15 Weikai Qi , Shreya Tiwary , Richard K. Bowles

The dramatic slowdown of dynamics in supercooled liquids approaching the glass transition remains one of the central unresolved problems in condensed matter physics. We review approaches that attribute this slowdown to growing thermodynamic…

Soft Condensed Matter · Physics 2026-03-06 Massimo Pica Ciamarra , Jeppe C. Dyre , Edan Lerner , Matthieu Wyart

We give a brief introduction to the mode-coupling theory of the glass transition, a theory which was proposed a while ago to describe the dynamics of supercooled liquids. After presenting the basic equations of the theory, we review some of…

Statistical Mechanics · Physics 2008-02-03 W. Kob

As one increases the concentration of a colloidal suspension, the system exhibits a dramatic increase in viscosity. Structurally, the system resembles a liquid, yet motions within the suspension are slow enough that it can be considered…

Soft Condensed Matter · Physics 2012-05-22 Gary L. Hunter , Eric R. Weeks

We present molecular dynamics results for a two component, two-dimensional Lennard-Jones supercooled liquid near the glass transition. We find that the supercooled liquid is spatially heterogeneous and that there are long-lived clusters…

Disordered Systems and Neural Networks · Physics 2009-10-31 Gregory Johnson , Andrew I. Melcuk , Harvey Gould , W. Klein , Raymond D. Mountain

We show that a generalized fluctuation-dissipation relation applies upon instantaneously increasing the temperature of a deeply supercooled liquid. This has the same two-step shape of the relation found upon cooling the liquid, but with…

Statistical Mechanics · Physics 2013-05-30 Nicoletta Gnan , Claudio Maggi , Giorgio Parisi , Francesco Sciortino

Melt supercooling leads to glass formation. Liquid-to-liquid phase transitions are observed depending on thermal paths. Viscosity, density and surface tension thermal dependences measured at heating and subsequent cooling show hysteresis…

Materials Science · Physics 2016-12-21 Robert F. Tournier

While lot of measurements describe the relaxation dynamics of the liquid state, experimental data of the glass dynamics at high temperatures are much scarcer. We use ultrafast scanning calorimetry to expand the timescales of the glass to…

Specific heat and linear thermal expansivity are fundamental thermal dynamics and have been proven as interesting relaxing quantities to investigate in glass transition and glassy state. However, their possibility has much less been…

Soft Condensed Matter · Physics 2021-09-06 Pengfei Zhang , Marco Gandolfi , Francesco Banfi , Christ Glorieux , Liwang Liu

We investigate dynamic scaling properties of the two-dimensional gauge glass model for the vortex glass phase in superconductors with quenched disorder. From extensive Monte Carlo simulations we obtain static and dynamic finite size scaling…

Disordered Systems and Neural Networks · Physics 2007-05-23 Marios Nikolaou , Mats Wallin

The universal behavior of the continuous superconducting (glass) phase transition is studied in a YBa$_2$Cu$_3$O$_{7-\delta}$ thin film. A new analysis technique for extracting critical exponents is developed, using current-voltage…

Superconductivity · Physics 2009-10-30 Katerina Moloni , Mark Friesen , Shi Li , Victor Souw , P. Metcalf , M. McElfresh

Attempts to understand zero temperature phase transitions have forced physicists to consider a regime where the standard paradigms of condensed matter physics break down [1-4]. These quantum critical systems lack a simple description in…

Quantum Gases · Physics 2012-07-04 Kaden R. A. Hazzard , Erich J. Mueller

We review the Random First Order Transition Theory of the glass transition, emphasizing the experimental tests of the theory. Many distinct phenomena are quantitatively predicted or explained by the theory, both above and below the glass…

Disordered Systems and Neural Networks · Physics 2015-06-25 Vassiliy Lubchenko , P. G. Wolynes

We use Photon Correlation Imaging, a recently introduced space-resolved dynamic light scattering method, to investigate the spatial correlation of the dynamics of a variety of jammed and glassy soft materials. Strikingly, we find that in…

We monitor the transformation of a liquid into an amorphous solid in simulations of a glass forming liquid by measuring the variation of a structural order parameter with either changing temperature or potential energy to establish the…

Soft Condensed Matter · Physics 2023-06-07 Gang Sun , Peter Harrowell
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