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We demonstrate a single-beam, standoff (>10m) coherent anti-Stokes Raman scattering spectroscopy (CARS) of various materials, including trace amounts of explosives and nitrate samples, under ambient light conditions. The multiplex…

Optics · Physics 2010-12-02 O. Katz , A. Natan , S. Rosenwaks , Y. Silberberg

The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…

Astrophysics · Physics 2007-05-23 Jacques Moret-Bailly

Frequency modulation coherent anti-Stokes Raman scattering (FM CARS) is presented, using a compact as well as fast and widely tunable fiber-based light source. With this light source Raman resonances between 700 cm$^{-1}$ and 3200 cm$^{-1}$…

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

Broadband coherent anti-Stokes Raman scattering (CARS) spectroscopy plays a vital role in chemical sensing and label-free vibrational imaging, yet conventional methods suffer from limited acquisition speeds and complex detection schemes.…

Optics · Physics 2025-07-23 Jing Hu , Tianjian Lv , Zhaoyang Wen , Wending Huang , Ming Yan , Heping Zeng

We propose an elegant scheme towards phase locking of two independent degenerate coherent anti-Stokes Raman scattering (CARS) processes. The optical implementation involves a modified Mach-Zehnder interferometer that is utilized to transfer…

Optics · Physics 2008-12-25 Qun Zhang

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

Coherent anti-Stokes Raman scattering (CARS) microscope system was built and applied to a non-intrusive gas concentration measurement of a mixing flow in a millimeter-scale channel. Carbon dioxide and nitrogen were chosen as test fluids and…

Fluid Dynamics · Physics 2015-08-07 Ken Yamamoto , Yuki Yamagata , Madoka Moriya , Reiko Kuriyama , Yohei Sato

We propose a Bayesian statistical model for analyzing coherent anti-Stokes Raman scattering (CARS) spectra. Our quantitative analysis includes statistical estimation of constituent line-shape parameters, underlying Raman signal,…

Applications · Statistics 2020-05-15 Teemu Härkönen , Lassi Roininen , Matthew T. Moores , Erik M. Vartiainen

Early theoretical works on coherent anti-Stokes Raman scattering in optically active medium consider only heterodyne signal and subsequently, fourth- and fifth-rank tensor averages have been used. In this work, we presented a full signal…

Quantum Physics · Physics 2019-01-03 Tuguldur Kh. Begzjav , Marlan O. Scully , Girish S. Agarwal

We present a theoretical investigation of an integrated nonlinear light source for coherent anti-Stokes Raman scattering (CARS) based on silicon nitride waveguides. Wavelength tunable and temporally synchronized signal and idler pulses are…

Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…

We develop a computational framework to examine the factors responsible for scattering-induced distortions of coherent anti-Stokes Raman scattering (CARS) signals in turbid samples. We apply the Huygens-Fresnel Wave-based Electric Field…

Computational Physics · Physics 2020-12-18 Janaka C. Ranasinghesagara , Giuseppe de Vito , Vincenzo Piazza , Eric O. Potma , Vasan Venugopalan

We apply coherent anti-Stokes Raman Scattering (CARS) microscopy to characterize director structures in liquid crystals.

Soft Condensed Matter · Physics 2016-09-08 A. V. Kachynski , A. N. Kuzmin , P. N. Prasad , I. I. Smalyukh

We investigate the role of non-uniform spatial density profiles of trapped atomic Bose-Einstein condensates in the propagation of Raman-matched laser pulses under conditions for electromagnetically induced transparency (EIT). We find that…

Quantum Physics · Physics 2009-11-07 Özgür E. Müstecaplıoğlu , L. You

Raman lasers based on integrated silica whispering gallery mode resonant cavities have enabled numerous applications from telecommunications to biodetection. To overcome the intrinsically low Raman gain value of silica, these devices…

Optics · Physics 2020-01-06 Hyungwoo Choi , Dongyu Chen , Fan Du , Rene Zeto , Andrea M Armani

Coherent Anti-Stokes Raman Scattering (CARS) processes are ``coherent,'' but the phase of the anti-Stokes radiation is usually lost by most incoherent spectroscopic CARS measurements. We propose a novel Raman microscopy imaging method…

Optics · Physics 2009-11-10 D. L. Marks , S. A. Boppart

We present an improvement on the signal-to-background of single-beam coherent anti-Stokes Raman scattering (SB-CARS) spectroscopy measurements for systems employing ultrafast supercontinuum sources based on all-normal dispersion photonic…

We present a simple method and its experimental implementation to completely determine the characteristics of the pump-and-probe pulse and the Stokes pulse in a coherent anti-Stokes Raman scattering microscope at sample level without…

Coherent Raman scattering spectroscopy is studied purposely, with the Gaussian ultrashort pulses as a hands-on elucidatory extraction tool of the clean coherent Raman resonant spectra from the overall measured data contaminated with the…

Optics · Physics 2017-04-05 Gombojav O. Ariunbold , Narangerel Altangerel