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We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

Modern nonlinear optical materials allow light of one wavelength be efficiently converted into light at another wavelength. However, designing nonlinear optical materials to operate with ultrashort pulses is difficult, because it is…

Although the frequency shift and odd-even intensity modulation in high-order harmonic generation (HHG) have both been observed for asymmetric laser-target systems, they are typically studied as two separate phenomena. In this Letter, we…

Optics · Physics 2024-06-14 Doan-An Trieu , Van-Hoang Le , Ngoc-Loan Phan

The dream of physico-chemists to control molecular reactions with light beyond electronic excitations pushes the development of laser pulse shaping capabilities in the mid-infrared (MIR) spectral range. Here, we present a compact optical…

The generation of ultra-strong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum…

We demonstrate that Freeman resonances have a strong impact on the nonlinear optical response in femtosecond filaments. These resonances decrease the transient refractive index within a narrow intensity window and strongly affect the…

Optics · Physics 2014-12-18 Michael Hofmann , Carsten Brée

Strong deformation of ultrashort laser pulse shapes is unavoidable when delivering high intensities at remote distances due to non-linear effects taking place while propagating. Relying on the reversibility of laser filamentation, we…

In this paper we examine the spectral changes in a white light laser filament due to different pulse shapes generated by a pulse shaping setup. We particularly explore how the properties of the filament spectra can be controlled by…

Nonlinear optics processes lie at the heart of photonics and quantum optics for their indispensable role in light sources and information processing. During the past decades, the three- and four-wave mixing ($\chi^{(2)}$ and $\chi^{(3)}$)…

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

A dramatic spectral modulation of third-order harmonic (TH) emission generated in a near in- frared femtosecond (fs) pulse filamentation, assisted by a two-dimensional plasma grating formed by two pump femtosecond pulses, is experimentally…

High-order nonlinear light-matter interactions in gases enable generation of x-ray and attosecond light pulses, metrology, and spectroscopy. Optical nonlinearities in solid-state materials are particularly interesting for combining optical…

Materials Science · Physics 2015-10-05 Muneaki Hase , Masayuki Katsuragawa , Anca Monia Constantinescu , Hrvoje Petek

We investigate parametric processes in magnetised plasmas, driven by a large-amplitude pump light wave. Our focus is on laser-plasma interactions relevant to high-energy-density (HED) systems, such as the National Ignition Facility and the…

Plasma Physics · Physics 2022-04-27 E. E. Los , D. J. Strozzi

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

In nonlinear nanophotonics, cascaded second-harmonic generation (SHG) in pure plasmonic waveguides for sequential signal transformation and complex on-chip functionality remains a long-standing challenge. Precise phase matching becomes…

Optics · Physics 2025-08-22 Komal Gupta , Anand Hegde , Xiaofei Wu , Jer-Shing Huang , Chen-Bin Huang

The nonlinear optical response of materials to exciting light is enhanced by resonances between the incident laser frequencies and the energy levels of the excited material. Traditionally, in molecular nonlinear spectroscopy one tunes the…

Optics · Physics 2019-01-30 Yael Blechman , Euclides Almeida , Basudeb Sain , Yehiam Prior

High quality lithium niobate thin film microresonators provide an ideal platform for on-chip nonlinear optics applications. However, the phase matching condition for efficient parametric process sets a high requirement for fabrication…

Up to now the long range filaments have been considered as a balance between Kerr focusing and defocusing by plasma generation in the nonlinear focus. However, it is difficult to apply the above explanation of filamentation in far-field…

Optics · Physics 2011-03-25 Lubomir Kovachev

We show that, nonlinear optical processes of nanoparticles can be controlled by the presence of interactions with a molecule or a quantum dot. By choosing the appropriate level spacing for the quantum emitter, one can either suppress or…

Mesoscale and Nanoscale Physics · Physics 2014-09-22 Deniz Turkpence , Gursoy B. Akguc , Alpan Bek , Mehmet Emre Tasgin

The impact of nonadiabatic laser-induced molecular alignment on filamentation is numerically studied. Weak and strong field model of impulsive molecular alignment are compared in the context of nonlinear pulse propagation. It is shown that…

Optics · Physics 2014-12-03 N. Berti , P. Béjot , J. -P. Wolf , O. Faucher
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