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Brownian Dynamics simulations are carried out to understand the effect of temperature and dielectric constant of the medium on microphase separation of charged-neutral diblock copolymer systems. For different dielectric media, we focus on…

Soft Condensed Matter · Physics 2011-07-20 Monojoy Goswami , Rajeev Kumar , Bobby G. Sumpter , Jimmy Mays

A two-component two-dimensional (2D) dipolar bosonic system in the bilayer geometry is considered. By performing quantum Monte Carlo simulations in a wide range of layer spacings we analyze in detail the pair correlation functions, the…

Quantum Gases · Physics 2016-08-03 Alexey Filinov

In earlier work we provided the first evidence that the collapse, or coil-globule, transition of an isolated polymer in solution can be seen in a four-dimensional model. Here we investigate, via Monte Carlo simulations, the canonical…

Statistical Mechanics · Physics 2009-10-31 T. Prellberg , A. L. Owczarek

We study the dynamics and conformation of polymers composed by active monomers. By means of Brownian dynamics simulations we show that when the direction of the self-propulsion of each monomer is aligned with the backbone, the polymer…

Soft Condensed Matter · Physics 2018-11-28 Valentino Bianco , Emanuele Locatelli , Paolo Malgaretti

The scaling of the bond-bond correlation function $C(s)$ along linear polymer chains is investigated with respect to the curvilinear distance, $s$, along the flexible chain and the monomer density, $\rho$, via Monte Carlo and molecular…

Soft Condensed Matter · Physics 2009-11-10 J. P. Wittmer , H. Meyer , J. Baschnagel , A. Johner , S. Obukhov , L. Mattioni , M. Mueller , A. N. Semenov

The physical chemistry of liquid-liquid phase separation (LLPS) of polymer solutions bears directly on the assembly of biologically functional droplet-like bodies from proteins and nucleic acids. These biomolecular condensates include…

Biomolecules · Quantitative Biology 2020-01-31 Yi-Hsuan Lin , Jacob P. Brady , Hue Sun Chan , Kingshuk Ghosh

Constitutive modeling of dielectric elastomers has been of long standing interest in mechanics. Over the last two decades rigorous constitutive models have been developed that couple the electrical response of these polymers with large…

Soft Condensed Matter · Physics 2021-10-19 Matthew Grasinger , Kaushik Dayal , Gal deBotton , Prashant K. Purohit

The dynamics of polymer-nanoparticle (NP) mixtures, which involves multiple scales and system-specific variables, has posed a long-standing challenge on its theoretical description. In this paper, we construct a microscopic theory for…

Soft Condensed Matter · Physics 2021-06-15 Bokai Zhang , Jian Li , Juan-mei Hu , Lei Liu

We investigate the role of the electron correlation effects in the calculations of the electric dipole polarizabilities (\alpha) of elements belonging to three different groups of periodic table. To understand the propagation of the…

Atomic Physics · Physics 2014-05-21 Yashpal Singh , B. K. Sahoo

We study the diffusion of a linear polymer in the presence of permeable membranes without excluded volume interactions, using scaling theory and Monte Carlo simulations. We find that the average time it takes for a chain with polymerization…

Condensed Matter · Physics 2016-08-31 Hyoungsoo Yoon , J. M. Deutsch

If many micelles adsorb onto the same polymer molecule then they are said to form a necklace. A minimal model of such a necklace is proposed and shown to be almost equivalent to a 1-dimensional fluid with nearest-neighbour interactions. The…

Soft Condensed Matter · Physics 2009-10-30 Richard P. Sear

We propose the quantitative mean-field theory of mechanical unfolding of a globule formed by long flexible homopolymer chain collapsed in poor solvent and subjected to an extensional force We show that with an increase in the applied force…

Soft Condensed Matter · Physics 2012-05-15 Alexey A. Polotsky , Elizaveta E. Smolyakova , Oleg V. Borisov , Tatiana M. Birshtein

We deduce the qualitative phase diagram of a long flexible neutral polymer chain immersed in a poor solvent near an attracting surface using phenomenological arguments. The actual positions of the phase boundaries are estimated numerically…

Statistical Mechanics · Physics 2009-11-07 R. Rajesh , Deepak Dhar , Debaprasad Giri , Sanjay Kumar , Yashwant Singh

Modeling ion correlations in inhomogeneous polymers and soft matters with spatially varying ionic strength or dielectric permittivity remains a great challenge. Here, we develop a new theory which systematically incorporates electrostatic…

Soft Condensed Matter · Physics 2024-07-01 Chao Duan , Nikhil R. Agrawal , Rui Wang

We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

Soft Condensed Matter · Physics 2020-04-13 Shalabh K. Anand , Sunil P. Singh

The system of polymers in solvent mixtures is a widely-used model to represent biomolecular condensates in intracellular environments. Here, we apply a variational theory to control the center-of-mass of two polymers and perform the first…

Soft Condensed Matter · Physics 2025-02-28 Luofu Liu , Rui Wang

The ability to tune the microstructures formed by block copolymers using accessible physical approaches provides control for practical material applications. A common strategy involves the addition of homopolymers, which can induce…

Soft Condensed Matter · Physics 2025-04-11 Xiangyu Zhang , Jing Zong , Dong Meng

As a model of soft confinement for polymers, we investigated equilibrium shapes of a flexible vesicle that contains a phase-separating polymer solution. To simulate such a system, we combined the phase field theory (PFT) for the vesicle and…

Biological Physics · Physics 2015-06-19 Yutaka Oya , Toshihiro Kawakatsu

I develop a kinetic mechanism to explain chain folding in polymer crystallization which is based on the competition between the formation of stems, which is due to frequent occupations of trans states along the chains in the supercooled…

Soft Condensed Matter · Physics 2014-09-23 S. Stepanow

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder
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