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We study systematically the role of temperature in the optical response of doped two-dimensional semiconductors. By making use of a finite-temperature Fermi-polaron theory, we reveal a crossover from a quantum-degenerate regime with…

Mesoscale and Nanoscale Physics · Physics 2024-01-25 A. Tiene , B. C. Mulkerin , J. Levinsen , M. M. Parish , F. M. Marchetti

Half-light half-matter quasiparticles termed exciton-polaritons arise through the strong coupling of excitons and cavity photons. They have been used to demonstrate a wide array of fundamental phenomena and potential applications ranging…

Applied Physics · Physics 2020-01-08 Jie Gu , Biswanath Chakraborty , Mandeep Khatoniar , Vinod M. Menon

MoSe2-WSe2 heterostructures host strongly bound interlayer excitons (IXs) which exhibit bright photoluminescence (PL) when the twist-angle is near 0{\deg} or 60{\deg}. Over the past several years, there have been numerous reports on the…

Two-dimensional semiconductors exhibit pronounced many-body effects and intense optical responses due to strong coulombic interactions. Consequently, subtle differences in photoexcitation conditions can strongly influence how the material…

We describe recent experimental efforts to perform polarization-resolved optical spectroscopy of monolayer transition-metal dichalcogenide semiconductors in very large pulsed magnetic fields to 65 tesla. The experimental setup and technical…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Andreas V. Stier , Kathleen M. McCreary , Berend T. Jonker , Junichiro Kono , Scott A. Crooker

We show that a transition metal dichalcogenide monolayer with a radiatively broadened exciton resonance would exhibit perfect extinction of a transmitted field. This result holds for s- or p-polarized weak resonant light fields at any…

Mesoscale and Nanoscale Physics · Physics 2017-09-20 Sina Zeytinoglu , Charlaine Roth , Sebastian Huber , Atac Imamoglu

Formation of dressed light-matter states in optical structures, manifested as Rabi splitting of the eigen energies of a coupled system, is one of the key effects in quantum optics. In pursuing this regime with semiconductors, light is…

Strong Coulomb interaction in monolayer transition metal dichalcogenides can facilitate nontrivial many-body effects among excitonic complexes. Many-body effects like exciton-exciton annihilation (EEA) have been widely explored in this…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Garima Gupta , Sarthak Das , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Among all excitonic complexes in transition-metal dichalcogenides (TMDs), dark and semi-dark trions are poised to play a stellar role in future quantum technologies due to their long lifetimes, about two orders of magnitude greater than…

Mesoscale and Nanoscale Physics · Physics 2026-01-27 Sreyan Raha , Tara Shankar Bhattacharya , Indrani Bose , Achintya Singha

We present photoluminescence measurements in monolayer WSe$_2$, which point to the importance of the interaction between charged particles and excitonic complexes. The theoretical analysis highlights the key role played by exchange…

Materials Science · Physics 2022-02-15 Min Yang , Lei Ren , Cedric Robert , Dinh Van Tuan , Laurent Lombez , Bernhard Urbaszek , Xavier Marie , Hanan Dery

Exciton condensation--an interaction-driven, macroscopically coherent paired-fermion state--offers the prospect for dissipationless energy transport in solids, akin to that in superconductivity. Although their light effective mass and…

Two-dimensional dilute magnetic semiconductors has been recently reported in semiconducting transition metal dichalcogenides by the introduction of spin-polarized transition metal atoms as dopants. This is the case of vanadium-doped WS$_2$…

All-solid-state strong light-matter coupling systems with large vacuum Rabi splitting are great important for quantum information application, such as quantum manipulation, quantum information storage and processing. The monolayer…

Mesoscale and Nanoscale Physics · Physics 2017-04-27 Jinxiu Wen , Hao Wang , Huanjun Chen , Shaozhi Deng , Ningsheng Xu

The origin of the variation of photoluminescence (PL) spectra of monolayer tungsten disulfide (WS2) is investigated systematically. Dependence of the PL spectrum on the excitation power show that the relatively sharp component corresponds…

Mesoscale and Nanoscale Physics · Physics 2018-06-01 Yongjae Kwon , Kangwon Kim , Wontaek Kim , Sunmin Ryu , Hyeonsik Cheong

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors emerging promising applications in diverse optoelectronic devices. To improve performance, recent investigations have been systematically focused on the tuning…

Monolayer transition metal dichalcogenides (TMDs) support robust excitons in the visible to near-infrared spectral range. Their reduced dielectric screening results in large binding energies, and combined with a direct bandgap in monolayer…

We develop a theoretical description of Coulomb interactions between trions (charged excitons) that define a nonlinear optical response in doped two-dimensional semiconductors. First, we formulate a microscopic theory of trion-trion…

Mesoscale and Nanoscale Physics · Physics 2022-07-07 Kok Wee Song , Salvatore Chiavazzo , Ivan A. Shelykh , Oleksandr Kyriienko

Monolayer (1L) transition metal dichalcogenides (TMDC) are of strong interest in nanophotonics due to their narrow-band intense excitonic transitions persisting up to room temperature. When brought into resonance with surface plasmon…

The optical response of doped monolayer semiconductors is governed by trions, i.e. photoexcited electron-hole pairs bound to doping charges. While their photoluminescence (PL) signatures have been identified in experiments, a microscopic…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Raul Perea-Causin , Samuel Brem , Ole Schmidt , Ermin Malic

We have studied the ambient air oxidation of chemical vapor deposition (CVD) grown monolayers of the semiconducting transition metal dichalcogenide (S-TMD) WS$_{2}$ using optical microscopy, laser scanning confocal microscopy (LSCM),…