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Chemical processes on the surface of icy grains play an important role in the chemical evolution in molecular clouds. In particular, reactions involving non-energetic hydrogen atoms accreted from the gaseous phase have been extensively…

Astrophysics of Galaxies · Physics 2022-07-20 Masashi Tsuge , Akira Kouchi , Naoki Watanabe

We present subarcsecond-resolution ALMA mosaics of the Orion Bar PDR in [CI] 609um, C2H (4-3), and C18O (3-2) emission lines complemented by JWST images of H2 and aromatic infrared band (AIB) emission. The rim of the Bar shows very…

We present a new method to decompose the emission features of polycyclic aromatic hydrocarbons (PAHs) from mid-infrared spectra using theoretical PAH templates in conjunction with modified blackbody components for the dust continuum and an…

Astrophysics of Galaxies · Physics 2018-06-26 Yanxia Xie , Luis C. Ho , Aigen Li , Jinyi Shangguan

Rapid, efficient deactivation of the photoexcited PAH cations accounts for their remarkable photostability and have important implications for astrochemistry, as these cations are the leading candidates for the species responsible for the…

Electronic excitations near the surface of water ice lead to the desorption of adsorbed molecules, through a so far debated mechanism. A systematic study of photon-induced indirect desorption, revealed by the spectral dependence of the…

We adapt the computational hydrogen electrode approach to explicitly account for photo-generated charges and use it to computationally screen for viable catalyst/co-catalyst combinations for photo-catalytic water splitting. The hole energy…

Materials Science · Physics 2013-07-31 Harald Oberhofer , Karsten Reuter

The polymer of intrinsic microporosity PIM 1 is employed to disperse and deposit a Pt at titanate nanosheet photocatalyst film. The resulting microporous films allow electrolyte and oxygen permeation to give conventional oxygen reduction…

We propose a scheme of "$R$-type" photoassociative adiabatic passage (PAP) to create polar molecular condensates from two different species of ultracold atoms. Due to the presence of a quasi-coherent population trapping state in the scheme,…

Quantum Gases · Physics 2015-05-18 Jing Qian , Lu Zhou , Keye Zhang , Weiping Zhang

We have obtained new STIS/HST spectra to search for structure in the ultraviolet interstellar extinction curve, with particular emphasis on a search for absorption features produced by polycyclic aromatic hydrocarbons (PAHs). The presence…

The formation of Polycyclic Aromatic Hydrocarbons in the circumstellar outflows of evolved stars is reviewed, with an emphasis on carbon stars on the Asymptotic Giant Branch. Evidence for PAHs present in their winds is provided by…

Solar and Stellar Astrophysics · Physics 2015-05-20 Isabelle Cherchneff

In order to find out capable molecular source of astronomically well observed infrared (IR) spectrum, asymmetric molecular configuration polycyclic aromatic hydrocarbon (PAH) was analyzed by the density functional theory (DFT) analysis.…

Astrophysics of Galaxies · Physics 2015-10-27 Norio Ota

Mid-infrared (IR) observations of polycyclic aromatic hydrocarbons (PAHs) and molecular hydrogen emission are a potentially powerful tool to derive physical properties of dense environments irradiated by intense UV fields. We present new,…

Astrophysics of Galaxies · Physics 2014-11-20 O. Berne , A. Fuente , J. R. Goicoechea , P. Pilleri , M. Gonzalez-Garcia , C. Joblin

Assuming a delta pulse excitation, quantum wavepackets are propagated on the excited state manifold in the energy range from 3.4-5.0 eV for coronene and 2.4-3.5 eV for circumcoronene to study the time evolution of the states as well as…

Chemical Physics · Physics 2024-01-17 Alberto Martín Santa Daría , Lola González-Sánchez , Sandra Gómez

We present measurements of 5-25 {\mu}m emission features of brightest cluster galaxies (BCGs) with strong optical emission lines in a sample of 9 cool-core clusters of galaxies observed with the Infrared Spectrograph on board the Spitzer…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-27 Megan Donahue , Geneviève E. de Messières , Robert W. O'Connell , G. Mark Voit , Aaron Hoffer , Brian R. McNamara , Paul E. J. Nulsen

A mechanism based on the penetration of interstellar ultraviolet photons into the inner layers of clumpy circumstellar envelopes around AGB stars is proposed to explain the non-equilibrium chemistry observed in such objects. We show through…

Astrophysics of Galaxies · Physics 2015-05-20 Marcelino Agundez , Jose Cernicharo , Michel Guelin

Phosphorene is a new family member of two-dimensional materials. We observed strong and highly layer-dependent photoluminescence in few-layer phosphorene (2 to 5 layers). The results confirmed the theoretical prediction that few-layer…

Mesoscale and Nanoscale Physics · Physics 2014-09-05 Shuang Zhang , Jiong Yang , Renjing Xu , Fan Wang , Weifeng Li , Muhammad Ghufran , Yong-wei Zhang , Zongfu Yu , Gang Zhang , Qinghua Qin , Yuerui Lu

Using atomistic simulations, we characterize the adsorption process of organic molecules on carbon nanoparticles, both of which have been reported to be abundant in the interstellar medium (ISM). It is found that the aromatic organics are…

Astrophysics of Galaxies · Physics 2018-11-14 H. Qi , S. Picaud , M. Devel , E. liang , Z. Wang

Polycyclic Aromatic Hydrocarbons (PAHs) are believed to be the small-size tail of the interstellar carbonaceous dust grain population. Their vibrational emission is the most widely accepted source of the aromatic near-infrared features, and…

Astrophysics of Galaxies · Physics 2015-08-21 Yacine Ali-Haïmoud , Laura Pérez , Ronald Maddalena , Anish Roshi

We show theoretically that it is possible to form a cold molecular ion from a pair of colliding atom and ion at low energy by photoassociative two-photon Raman processes. We explore the possibility of stimulated Raman adiabatic passage…

Atomic Physics · Physics 2016-09-13 Dibyendu Sardar , Somnath Naskar , Arpita Pal , Bimalendu Deb

Water splitting reactions through photocatalysis is an efficient and sustainable technique for the generation of green energy. The photocatalyst's ability to effect simultaneous generation of hydrogen and oxygen, along with efficiency in…

Materials Science · Physics 2024-05-10 Swati Shaw , Subhradip Ghosh