Related papers: Mesoscopic Quantum Emitters from Deterministic Agg…
We present a single-scattering formalism for incoherent resonant light scattering by dilute quantum gas systems such as the atomic-trap Bose-Einstein condensates. We show that resonant scattering gives access to more information than the…
Absorption is usually expected to be detrimental to quantum coherence effects. However, the situation for complex absorption spectra has been little studied yet. We consider the resonance fluorescence of excitons in a semiconductor quantum…
Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…
We consider a quantum theory of elastic light scattering from a macroscopic atomic sample existing in the Bose-Einstein condensate (BEC) phase. The dynamics of the optical excitation induced by an incident photon is influenced by the…
We show that resonance fluorescence, i.e. the resonant emission of a coherently driven two-level system, can be realized with a semiconductor quantum dot. The dot is embedded in a planar optical micro-cavity and excited in a wave-guide mode…
Resonance fluorescence of natural or artificial atoms constitutes a prime method for generating non-classical light. While most efforts have focused on producing single-photons, multi-photon emission is unavoidably present in the resonant…
Resonance fluorescence arises from the interaction of an optical field with a two-level system and has played a fundamental role in the development of quantum optics and its applications. Despite its conceptual simplicity it entails a wide…
The interaction between molecules is commonly ignored in surface-enhanced Raman scattering (SERS). Under this assumption, the total SERS signal is described as the sum of the individual contributions of each molecule treated independently.…
Measurement-based quantum communication relies on the availability of highly entangled multi-photon cluster states. The inbuilt redundancy in the cluster allows communication between remote nodes using repeated local measurements,…
Coherent control, a central concept in physics and chemistry, has sparked significant interest due to its ability to fine-tune interference effects in atoms and individual molecules for applications ranging from light-harvesting complexes…
Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot…
The subtle and fundamental issue of indistinguishability and interference between independent pathways to the same target state is examined in the context of coherent control of atomic and molecular processes, with emphasis placed on…
Reduced abstract. This Thesis explores emergent cooperative phenomena in collective light-matter systems. We study ensembles of interacting quantum emitters coherently driven by a laser field and coupled to photonic structures, focusing on…
When an ensemble of quantum emitters couples to a common radiation field, their polarizations can synchronize and a collective emission termed superfluorescence can occur. Entering this regime in a free-space setting requires a large number…
Molecules are ubiquitous in natural phenomena and man-made products, but their use in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. We have now…
The theory of decoherence attempts to explain the emergent classical behaviour of a quantum system interacting with its quantum environment. In order to formalize this mechanism we introduce the idea that the information preserved in an…
We develop a microscopic model to investigate current-induced light emission in single-molecule tunnel junctions, where a two-level system interacts with a plasmonic field. Using the quantum master equation, we explore the transition from…
Collective coherent scattering of laser light induces strong light forces between polarizable point particles. These dipole forces are strongly enhanced in magnitude and distance within the field of an optical waveguide so that at low…
We analyze the light scattered by a single InAs quantum dot interacting with a resonant continuous-wave laser. High resolution spectra reveal clear distinctions between coherent and incoherent scattering, with the laser intensity spanning…
In conflict with standard notions of thermodynamics, mesoscopically-sized inclusions (``clusters'') of a solute-rich liquid have been observed in equilibrated solutions of proteins and other molecules. According to a complexation scenario…