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Related papers: Symmetry Reduction in the Quantum Kagome Antiferro…

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Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

Nearest-neighbor interacting S = 1/2 spins on the ideal Kagom\'{e} lattice are predicted to form a variety of novel quantum entangled states, including quantum spin-liquid (SL) and valence bond solid (VBS) phases. In real materials, the…

Strongly Correlated Electrons · Physics 2019-10-31 N. J. Laurita , A. Ron , J. W. Han , A. Scheie , J. P. Sheckelton , R. W. Smaha , W. He , J. -J. Wen , J. S. Lee , Y. S. Lee , M. R. Norman , D. Hsieh

The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of…

Strongly Correlated Electrons · Physics 2011-03-16 Philippe Mendels , Fabrice Bert

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

Strongly Correlated Electrons · Physics 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

Strongly Correlated Electrons · Physics 2015-05-28 P. Mendels , F. Bert

The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR…

Strongly Correlated Electrons · Physics 2015-11-09 M. Fu , T. Imai , T. -H. Han , Y. S. Lee

Recent evidence from magnetic torque, electron spin resonance, and second harmonic generation indicate that the prototypical quantum spin liquid candidate, herbertsmithite, has a symmetry lower than its x-ray refined trigonal space group.…

Strongly Correlated Electrons · Physics 2020-01-17 M. R. Norman , N. J. Laurita , D. Hsieh

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

Strongly Correlated Electrons · Physics 2010-04-07 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Qiu , D. G. Nocera , Y. S. Lee

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we…

Strongly Correlated Electrons · Physics 2013-09-09 M. Jeong , F. Bert , P. Mendels , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrison

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities[1-4]. This has been suggested as the reason why it is not strongly supported in large-scale numerical calculations[5]. However,…

Strongly Correlated Electrons · Physics 2013-11-13 Bryan Clark , Jesse Kinder , Eric Neuscamman , Garnet Kin-Lic Chan , Michael J. Lawler

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by…

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

Strongly Correlated Electrons · Physics 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

The Heisenberg antiferromagnet on the Kagom\'{e} lattice is studied in the framework of Schwinger-boson mean-field theory. Two solutions with different symmetries are presented. One solution gives a conventional quantum state with…

Strongly Correlated Electrons · Physics 2007-11-06 Peng Li , Haibin Su , Shun-Qing Shen

Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The…

Strongly Correlated Electrons · Physics 2016-08-24 Tian-Heng Han , M. R. Norman , J. -J. Wen , Jose A. Rodriguez-Rivera , Joel S. Helton , Collin Broholm , Young S. Lee

In this work we investigate the ground state properties of a candidate quantum spin liquid using a superconducting Noisy Intermediate-Scale Quantum (NISQ) device. Specifically, we study the antiferromagnetic Heisenberg model on a Kagome…

Quantum Physics · Physics 2025-06-17 Tim Weaving , Alexis Ralli , Vinul Wimalaweera , Peter J. Love , Peter V. Coveney

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko
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