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We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically…

The theory of elastic interaction of micron size axially symmetric colloidal particles immersed into confined nematic liquid crystal has been proposed. General formulas are obtained for the self energy of one colloidal particle and…

Soft Condensed Matter · Physics 2015-05-14 S. B. Chernyshuk , B. I. Lev

Via mechanisms not accessible at equilibrium, self-propelled particles can form phases with positional order, such as crystals, and with orientational order, such as polar flocks. However, the interplay between these two types of order…

Soft Condensed Matter · Physics 2025-08-13 Till Welker , Ricard Alert

Colloidal systems find important applications ranging from fabrication of photonic crystals to direct probing of phenomena typically encountered in atomic crystals and glasses. New applications - such as nanoantennas, plasmonic sensors, and…

Soft Condensed Matter · Physics 2016-12-30 Rahul P. Trivedi , Ivan I. Klevets , Bohdan Senyuk , Taewoo Lee , Ivan I. Smalyukh

We study elastic interactions between colloidal particles and deformation landscapes of undulations in a cholesteric liquid crystal under an electric field applied normal to cholesteric layers. The onset of undulation instability is…

Soft Condensed Matter · Physics 2016-12-06 Michael C. M. Varney , Qiaoxuan Zhang , Bohdan Senyuk , Ivan I. Smalyukh

We propose a simple theoretical model which explains a formation of dipolar 2D and 3D colloidal structures in nematic liquid crystal. Colloidal particles are treated as effective hard spheres interacting via their elastic dipole, quadrupole…

Soft Condensed Matter · Physics 2015-06-15 S. B. Chernyshuk , O. M. Tovkach , B. I. Lev

We demonstrate a variety of ordered patterns, including hexagonal structures and chains, formed by colloidal particles (droplets) at the free surface of a nematic liquid crystal (LC). The surface placement introduces a new type of particle…

Soft Condensed Matter · Physics 2009-11-10 I. I. Smalyukh , S. Chernyshuk , B. I. Lev , A. B. Nych , U. Ognysta , V. G. Nazarenko , O. D. Lavrentovich

Bottom-up assembly of nanocrystals (NCs) into ordered arrays, or superlattices (SLs), is a promising route to design materials with new functionalities, but the degree of control over assembly into functional structures remains challenging.…

Mixing colloid shapes with distinctly different anisotropy generates composite nematics in which the order of the individual components can be fundamentally different. In colloidal rod-disk mixtures or hybrid nematics composed of…

Soft Condensed Matter · Physics 2018-11-20 H. H. Wensink

We study by simulation the physics of two colloidal particles in a cholesteric liquid crystal with tangential order parameter alignment at the particle surface. The effective force between the pair is attractive at short range and favors…

Soft Condensed Matter · Physics 2015-03-19 J. S. Lintuvuori , K. Stratford , M. E. Cates , D. Marenduzzo

Self-assembly is one of the crucial mechanisms allowing to design multifunctional materials. Soft hybrid materials contain components of different nature and exhibit competitive interactions which drive self-organisation into structures of…

Combining topology and plasmonics paradigms in nanocolloidal systems may enable new means of pre-engineering desired composite material properties. Here we design and realize orientationally ordered assemblies of noble metal nanoparticles…

Soft Condensed Matter · Physics 2016-12-01 Ye Yuan , Ivan I. Smalyukh

The geometric shape, symmetry, and topology of colloidal particles often allow for controlling colloidal phase behavior and physical properties of these soft matter systems. In liquid crystalline dispersions, colloidal particles with low…

Soft Condensed Matter · Physics 2024-10-14 Ye Yuan , Ivan I. Smalyukh

Dynamics of small particles, both living such as swimming bacteria and inanimate, such as colloidal spheres, has fascinated scientists for centuries. If one could learn how to control and streamline their chaotic motion, that would open…

Soft Condensed Matter · Physics 2023-02-08 Oleg D. Lavrentovich

The directed self-assembly of colloidal nanoparticles (NPs) using external fields guides the formation of sophisticated hierarchical materials but becomes less effective with decreasing particle size. As an alternative, electron-beam-driven…

Soft Condensed Matter · Physics 2024-09-13 Jonathan G. Raybin , Ethan J. Dunsworth , Veronica Guo , Naomi S. Ginsberg

The assembly of colloids in nematic liquid crystals via topological defects has been extensively studied for spherical particles, and investigations of other colloid shapes have revealed a wide array of new assembly behaviors. We show,…

Soft Condensed Matter · Physics 2014-12-16 Daniel A. Beller , Mohamed A. Gharbi , Iris B. Liu

Manipulating the way in which colloidal particles self-organise is a central challenge in the design of functional soft materials. Meeting this challenge requires the use of building blocks that interact with one another in a highly…

Soft Condensed Matter · Physics 2021-03-30 Joe G Donaldson , Peter Schall , Laura Rossi

Freezing of charged colloids on square or triangular two-dimensional periodic substrates has been recently shown to realize a rich variety of orientational orders. We propose a theoretical framework to analyze the corresponding structures.…

Statistical Mechanics · Physics 2009-11-10 R. Agra , F. van Wijland , E. Trizac

Colloids dispersed in nematic liquid crystals form topological composites in which colloid-associated defects mediate interactions while adhering to fundamental topological constraints. Better realising the promise of such materials…

Soft Condensed Matter · Physics 2024-04-16 Louise C. Head , Yair A. G. Fosado , Davide Marenduzzo , Tyler N. Shendruk

Dispersions of rodlike colloidal particles exhibit a plethora of liquid crystalline states, including nematic, smectic A, smectic B, and columnar phases. This phase behavior can be explained by presuming the predominance of hard-core volume…

Soft Condensed Matter · Physics 2019-04-01 Andrii Repula , Mariana Oshima Menegon , Cheng Wu , Paul van der Schoot , Eric Grelet