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Negative thermal expansion (NTE) - the phenomenon where some materials shrink rather than expand when heated - is both intriguing and useful, but remains poorly understood. Current understanding hinges on the role of specific vibrational…

Materials Science · Physics 2020-09-23 Martin T Dove , Juan Du , Zhongsheng Wei , David A Keen , Matthew G Tucker , Anthony E Phillips

Thermal expansion is a problem in many technological applications and its control represents a challenge in materials design. In this Letter, after studying the correlation between thermal expansion, cubic-to-rhombohedral transition and…

Materials Science · Physics 2018-09-13 Andrea Sanson

The discovery of unusual negative thermal expansion (NTE) provides the opportunity to control the common but much desired property of thermal expansion, which is valuable not only in scientific interests but also in practical applications.…

While most solids expand when heated, some materials show the opposite behavior: negative thermal expansion (NTE). In polymers and biomolecules, NTE originates from the entropic elasticity of an ideal, freely-jointed chain. The origin of…

Recently, uniaxial negative thermal expansion (NTE) has been observed in transition-metal zirconides including tetragonal (CuAl2-type) CoZr2 and orthorhombic (Re3B-type) CoZr3. Here, we report the observation of uniaxial NTE in tetragonal…

Materials Science · Physics 2023-06-14 Yoshikazu Mizuguchi

We study negative thermal expansion (NTE) in model lattices with multiple atoms per cell and first- and second-nearest neighbor interactions using the (anharmonic) Morse potential. By exploring the phase space of neighbor distances and…

Materials Science · Physics 2016-06-15 Joseph T. Schick , Andrew M. Rappe

We use a symmetry-motivated approach to analysing X-ray pair distribution functions to study the mechanism of negative thermal expansion in two ReO$_3$-like compounds; ScF$_3$ and CaZrF$_6$. Both average and local structure suggest that it…

Materials Science · Physics 2020-02-26 Tobias Bird , Jessica Woodland-Scott , Lei Hu , Michael Wharmby , Jun Chen , Andrew Goodwin , Mark Senn

Scandium fluoride (ScF3) belongs to a class of negative thermal expansion (NTE) materials. It shows a strong lattice contraction up to about 1000 K switching to expansion at higher temperatures. Here the NTE effect in ScF3 is studied in the…

Materials Science · Physics 2020-02-25 D. Bocharov , M. Krack , Yu. Rafalskij , A. Kuzmin , J. Purans

The phenomenon of negative thermal expansion (NTE) deals with the increase of the lattice parameters and the volume of the unit cell when the material is thermally cooled. The NTE is typically associated with thermal phonons and anomalous…

Strongly Correlated Electrons · Physics 2023-03-10 Wojciech Brzezicki , Filomena Forte , Canio Noce , Mario Cuoco , Andrzej M. Oleś

The rare physical property of negative thermal expansion (NTE) is intriguing because materials with large NTE over a wide temperature range can serve as high-performance thermal expansion compensators. However, applications of NTE are…

We have investigated temperature dependence of the lattice parameters and the unit cell volume of ZnF$_2$ by neutron diffraction and have discovered negative thermal expansion (NTE) at low temperature. To understand why this simple compound…

Materials Science · Physics 2012-07-03 Tapan Chatterji , Mohamed Zbiri , Thomas C. Hansen

The cubic Prussian Blue (PB) analog, Zn3 [Fe(CN)6]2, has been studied by X-ray powder diffraction and inelastic neutron scattering (INS). X-ray data collected at 300 and 84 K revealed negative thermal expansion (NTE) behaviour for this…

Materials Science · Physics 2011-08-17 S Adak , L L Daemen , H Nakotte

Materials with negative thermal expansion (NTE), which contract upon heating, are of great interest both technically and fundamentally. Here, we report giant NTE covering room temperature in mechanically milled antiperovksite GaNxMn3…

The negative thermal expansion (NTE) mechanism in Cu2O has been characterised via mapping of different Cu2O structural flexibility models onto phonons obtained using ab-initio lattice dynamics. Low frequency acoustic modes that are…

The thermal and lattice dynamical properties of seven silicon clathrate framework structures are investigated with ab initio density functional methods (frameworks I, II, IV, V, VII, VIII, and H). The negative thermal expansion (NTE)…

Materials Science · Physics 2014-01-28 Ville J. Härkönen , Antti J. Karttunen

We have devised an isotropic interaction potential that gives rise to negative thermal expansion (NTE) behavior in equilibrium many-particle systems in both two and three dimensions over a wide temperature and pressure range (including zero…

Materials Science · Physics 2008-07-24 Mikael C. Rechtsman , Frank H. Stillinger , Salvatore Torquato

We investigated the structural, electronic, and superconducting properties of Co1-xNixZr2, in which c-axis thermal expansion is systematically controlled. At x (smaller than) 0.3, c-axis negative thermal expansion (NTE) was observed, and…

Superconductivity · Physics 2023-03-28 Yuto Watanabe , Hiroto Arima , Hidetomo Usui , Yoshikazu Mizuguchi

Negative thermal expansion (NTE) describes the anomalous propensity of materials to shrink when heated. Since its discovery, the NTE effect has been found in a wide variety of materials with an array of magnetic, electronic and structural…

Materials Science · Physics 2018-11-09 Connor A. Occhialini , G. G. Guzmán-Verri , Sahan U. Handunkanda , Jason N. Hancock

We use a symmetry-motivated approach to analyse neutron pair distribution function data to investigate the mechanism of negative thermal expansion (NTE) in ReO$_3$. This analysis shows that the local structure of ReO$_3$ is dominated by an…

Bulk Scandium trifluoride ($\mathrm{ScF_3}$) is known for a pronounced negative thermal expansion (NTE) over a wide range of temperature, from $10~\mathrm{K}~\text{to}~ 1100~\mathrm{K}$. The structure of $\mathrm{ScF_3}$ can be described as…

Materials Science · Physics 2024-03-12 Amani S. Jayakody , Joseph Budnick , Jason N. Hancock , Daniela Morales , Barrett O. Wells
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