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The potential for low-threshold optical nonlinearity has received significant attention in the fields of photonics and conceptual optical neuron networks. Excitons in two-dimensional (2D) semiconductors are particularly promising in this…

We unravel the influence of quasiparticle screening in the non-equilibrium exciton dynamics of monolayer WS$_2$. We report pump photon energy-dependent exciton blue and red-shifts from time-resolved-reflectance contrast measurements. Based…

Mesoscale and Nanoscale Physics · Physics 2023-03-15 Stefano Calati , Qiuyang Li , Xiaoyang Zhu , Julia Stähler

Exciton-exciton interactions are key to understanding non-linear optical and transport phenomena in van der Waals heterobilayers, which emerged as versatile platforms to study correlated electronic states. We present a combined…

Optoelectronic excitations in monolayer MoS2 manifest from a hierarchy of electrically tunable, Coulombic free-carrier and excitonic many-body phenomena. Investigating the fundamental interactions underpinning these phenomena - critical to…

Interactions among a collection of particles generate many-body effects in solids resulting in striking modifications of material properties. The heavy carrier mass that yields strong interactions and gate control of carrier density over a…

In monolayer transition-metal dichalcogenide semiconductors, many-body correlations can manifest in optical spectra when photoexcited electron-hole pairs (excitons) are introduced into a 2D Fermi sea of mobile carriers. At low carrier…

Mesoscale and Nanoscale Physics · Physics 2022-01-04 Jing Li , Mateusz Goryca , Junho Choi , Xiaodong Xu , Scott A. Crooker

We study carrier interaction induced many-body effects on the excitonic optical properties of highly photoexcited one-dimensional semiconductor quantum wire systems by solving the dynamically screened Bethe-Salpeter equation using realistic…

Strongly Correlated Electrons · Physics 2009-11-07 D. W. Wang , S. Das Sarma

Many-body exciton interactions shape the optoelectronic response of atomically-thin transition metal dichalcogenides, yet optical control of these interactions remains largely unexplored. To date, modulation of exciton-exciton interactions…

Marrying the predictive power of ab initio calculations with many-body effects remains a challenging task in two-dimensional (2d) materials, where efficient carrier-carrier interaction challenges established approximation schemes. In…

Mesoscale and Nanoscale Physics · Physics 2025-09-22 Alexander Steinhoff , Frank Jahnke , Matthias Florian

In two-dimensional hybrid organic-inorganic metal-halide perovskites, the intrinsic optical lineshape reflects multiple excitons with distinct binding energies, each dressed differently by the hybrid lattice. Given this complexity, a…

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

The intriguing physics of carrier-carrier interactions, which likewise affect the operation of light emitting devices, stimulate the research on semiconductor structures at high densities of excited carriers, a limit reachable at large…

Enhanced Coulomb interactions in monolayer transition metal dichalcogenides cause tightly bound electron-hole pairs (excitons) which dominate their linear and nonlinear optical response. The latter includes bleaching, energy…

Mesoscale and Nanoscale Physics · Physics 2020-06-25 Florian Katsch , Malte Selig , Andreas Knorr

Optical excitation serves as a powerful approach to control the electronic structure of layered Van der Waals materials via many-body screening effects, induced by photoexcited free carriers, or via light-driven coherence, such as optical…

Many-body interactions in monolayer transition-metal dichalcogenides are strongly affected by their unique band structure. We study these interactions by measuring the energy shift of neutral excitons (bound electron-hole pairs) in gated…

Materials Science · Physics 2019-02-06 Dinh Van Tuan , Benedikt Scharf , Zefang Wang , Jie Shan , Kin Fai Mak , Igor Zutic , Hanan Dery

A particular difficulty in studying many-body interactions in a solid is the absence of an experimental technique that can directly probe their key characteristics. We show that 2D Fourier spectroscopy provides an efficient tool for the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Mikhail Erementchouk , Michael N. Leuenberger , L. J. Sham

Coherent coupling between excitons is at the heart of many-body interactions with transition metal dichalcogenide (TMD) heterostructures as an emergent platform for the investigation of these interactions. We employ multi-dimensional…

Mesoscale and Nanoscale Physics · Physics 2022-01-05 Torben L. Purz , Eric W. Martin , Pasqual Rivera , William G. Holtzmann , Xiaodong Xu , Steven T. Cundiff

Nonlinear interactions between excitons strongly coupled to light are key for accessing quantum many-body phenomena in polariton systems. Atomically-thin two-dimensional semiconductors provide an attractive platform for strong light-matter…

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl
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