Related papers: Response to 'Comment on "Time delays in molecular …
In a recent article by P. Hockett \textit{et al.}, time delays arising in the context of molecular single-photon ionization are investigated from a theoretical point of view. We argue that one of the central equations derived in the paper…
No, we cannot! The concept of Wigner time delay was introduced in scattering theory to quantify the delay or advance of an incoming particle in its interaction with the scattering potential. It was assumed that this concept can be…
Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…
In scattering theory, the Wigner-Smith time delay, calculated through a phaseshift derivative or its multichannel generalization, has been demonstrated to measure the amount of delay or advance experienced by colliding particles during…
We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…
We present a step by step introduction to the notion of time-delay in classical and quantum mechanics, with the aim of clarifying its foundation at a conceptual level. In doing so, we motivate the introduction of the concepts of "fuzzy" and…
Determination and interpretation of Wigner-like photoionisation delays is one of the most active fields of attosecond science. Previous results have suggested that large photoionisation delays are associated with structured continua, but a…
We apply Brunetti and Fredenhagen's [Phys. Rev. A 66 (2002) 044101] concept of the time of occurrence of an event in quantum mechanics to the example of scattering off a spherical potential. Thereby, we re-derive the expression of…
We advocate for the systematic use of a symmetrized definition of time delay in scattering theory. In two-body scattering processes, we show that the symmetrized time delay exists for arbitrary dilated spatial regions symmetric with respect…
We consider a fully quantized model of spontaneous emission, scattering, and absorption, and study propagation of a single photon from an emitting atom to a detector atom both with and without an intervening scatterer. We find an exact…
The decay of photoexcited quantum systems (examples are photodissociation of molecules and autoionization of atoms) can be viewed as a half-collision process (an incoming photon excites the system which subsequently decays by dissociation…
Spontaneous photon scattering by an atomic qubit is a notable example of environment-induced error and is a fundamental limit to the fidelity of quantum operations. In the scattering process the qubit loses its distinctive and coherent…
We demonstrate serious misrepresentation of existing experimental data and important omissions in the List of references in the paper [1]. We demonstrate that what is called in [1] total photoionization cross-section is in fact a partial…
Although many physical arguments account for using a modified definition of time delay in multichannel-type scattering processes, one can hardly find rigorous results on that issue in the literature. We try to fill in this gap by showing,…
We present a theory of light scattering consistent with modern physics. We proposed a spatial-temporal model of a photon based on classical model of atomic oscillator. Using this photon model, we established a criterion for single vs…
In this paper we present a mathematical analysis of the photoelectric effect for one-electron atoms in the framework of non-relativistic QED. We treat photo-ionization as a scattering process where in the remote past an atom in its ground…
Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…
The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…
In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…
We prove that the existence of time delay defined in terms of sojourn times, as well as its identity with Eisenbud-Wigner time delay, is a common feature of two Hilbert space quantum scattering theory. All statements are model-independent.