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Direct frequency-comb spectroscopy is used to probe the absolute frequencies of $6S_{1/2}$-$8S_{1/2}$ two-photon transitions of atomic cesium in hot vapor environment. By utilizing the coherent control method of temporally splitting the…

Atomic Physics · Physics 2018-01-15 Kyung-tae Kim , Jaewook Ahn

Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…

Optics · Physics 2025-10-01 D. Konnov , A. Muraviev , K. L. Vodopyanov

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to…

Instrumentation and Detectors · Physics 2018-08-15 David R. Carlson , Daniel D. Hickstein , Daniel C. Cole , Scott A. Diddams , Scott B. Papp

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

Four-wave-mixing-based quantum cascade laser frequency combs (QCL-FC) are a powerful photonic tool, driving a recent revolution in major molecular fingerprint regions, i.e. mid- and far-infrared domains. Their compact and frequency-agile…

Dual terahertz (THz) comb spectroscopy is a promising methods for high accuracy, high resolution, and broadband THz spectroscopy because the mode-resolved THz comb spectrum possesses both characteristics of broadband THz radiation and…

The advent of the laser frequency comb as the wavelength calibration unit allows us to measure the radial velocity at $cm\ s^{-1}$ precision level with high stability in long-term, which enable the possibility of the detection of…

Instrumentation and Methods for Astrophysics · Physics 2018-10-15 Zhao Fei , Zhao Gang , Liu Yujuan , Wang Liang , Wang Huijuan , Li Hongbin , Ye Huiqi , Hao Zhibo , Xiao Dong , Zhang Junbo , Kellermann Hanna , Grupp Frank

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral…

Laser spectroscopy and interferometry have provided an unparalleled view into the fundamental nature of matter and the universe through ultra-precise measurements of atomic transition frequencies and gravitational waves. Optical frequency…

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…

Atomic Physics · Physics 2009-11-11 Adela Marian , Matthew C. Stowe , Daniel Felinto , Jun Ye

We demonstrate balanced-detection dual-comb spectroscopy (DCS) using two free-running mechanical sharing dual-comb fiber lasers assisted by an all-computational digital phase correction algorithm. The mutual coherence between the combs…

We demonstrate the use of a femtosecond frequency comb to coherently drive stimulated Raman transitions between terahertz-spaced atomic energy levels. More specifically, we address the $3d~^2D_{3/2}$ and $3d~^2D_{5/2}$ fine structure levels…

Quantum Physics · Physics 2018-06-21 Cyrille Solaro , Steffen Meyer , Karin Fisher , Michael V. DePalatis , Michael Drewsen

We present an optical-optical double-resonance (OODR) spectrometer based on a 3.3 ${\mu}$m continuous wave pump and two cavity-enhanced probes: a frequency comb tunable in the 1.64 - 1.8 ${\mu}$m range, and a comb-referenced continuous wave…

We report a high-energy, bidirectional, dissipative soliton mode-locked fiber laser operating in the 1550 nm normal-dispersion regime. By leveraging intracavity dispersion management and a Lyot filtering mechanism, the laser achieves…

Optics · Physics 2026-02-17 Mingjun Wang , Zhangru Shi , Anshuang Wang , Bowen Li

We report precision atmospheric spectroscopy of $CO_2$ using a laser heterodyne radiometer (LHR) calibrated with an optical frequency comb. Using the comb-calibrated LHR, we record spectra of atmospheric $CO_2$ near 1572.33 nm with a…

Optics · Physics 2023-10-03 Ryan K. Cole , Connor Fredrick , Newton H. Nguyen , Scott A. Diddams

A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric…

Pulse trains emitted from dual-comb systems are designed to have low relative timing jitter, making them useful for many optical measurement techniques such as optical ranging and spectroscopy. However, the characterization of low-jitter…

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