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Drops in contact with swollen, elastomeric substrates can induce a capillary-mediated phase separation in wetting ridges. Using laser scanning confocal microscopy, we visualize phase separation of oligomeric silicone oil from a crosslinked…

Soft Condensed Matter · Physics 2023-02-06 Lukas Hauer , Zhuoyun Cai , Doris Vollmer , Jonathan T. Pham

Anisotropically wetting substrates enable useful control of droplet behavior across a range of applications. Usually, these involve chemically or physically patterning the substrate surface, or applying gradients in properties like…

Soft Condensed Matter · Physics 2021-04-21 Katrina Smith-Mannschott , Qin Xu , Stefanie Heyden , Nicolas Bain , Eric R. Dufresne , Robert W. Style

We report an experimental investigation of the spontaneous motion of liquid droplets on soft gels with a crosslinking gradient. By systematically adjusting the spatial difference in crosslinking density, we observed that millimeter-sized…

Soft Condensed Matter · Physics 2025-01-29 Weiwei Zhao , Wenjie Qian , Chang Xu , Qin Xu

Soft materials are ubiquitous in technological applications that require deformability, for instance, in flexible, water-repellent coatings. However, the wetting properties of pre-strained soft materials are only beginning to be explored.…

Soft Condensed Matter · Physics 2025-04-15 Youchuang Chao , Hansol Jeon , Stefan Karpitschka

Understanding the dynamics of drops on polymer-coated surfaces is crucial for optimizing applications such as self-cleaning materials or microfluidic devices. While the static and dynamic properties of deposited drops have been well…

Soft Condensed Matter · Physics 2024-03-15 Rodrique G. M. Badr , Lukas Hauer , Doris Vollmer , Friederike Schmid

We present a molecular dynamics study of the motion of cylindrical polymer droplets on striped surfaces. We first consider the equilibrium properties of droplets on different surfaces, we show that for small stripes the Cassie-Baxter…

Soft Condensed Matter · Physics 2019-08-28 Ozlem Ozturk , James Servantie

When a liquid droplet completely wets a hard substrate, its spreading dynamics follow Tanner's law, with the droplet radius growing as the one-tenth power of time. Here, we investigate how these dynamics change when silicone oil droplets…

Soft Condensed Matter · Physics 2026-01-14 Lauren Dutcher , Benjamin Baylis , John R. Dutcher , Elie Raphael , Kari Dalnoki-Veress

Droplet coalescence is ubiquitous in nature and the same time key to various technologies, such as inkjet printing. Here, we report on the coalescence of polymer droplets with different chain lengths coalescing on substrates of different…

Soft Condensed Matter · Physics 2023-09-21 Soheil Arbabi , Panagiotis E. Theodorakis

A recent study has demonstrated that phase separation in binary liquid mixtures is arrested in the presence of elastic networks and can lead to a nearly uniformly-sized distribution of the dilute-phase droplets. At longer timescales, these…

Soft Condensed Matter · Physics 2020-10-28 Mrityunjay Kothari , Tal Cohen

This research introduces a new drop fluidics, which uses a deformable and stretchable elastomeric film as the platform, instead of the commonly used rigid supports. Such a soft film impregnated with magnetic particles can be modulated with…

Soft Condensed Matter · Physics 2016-07-01 Saheli Biswas , Yves Pomeau , Manoj K. Chaudhury

We consider a three-dimensional network of aqueous droplets joined by single lipid bilayers to form a cohesive, tissue-like material. The droplets in these networks can be programmed to have distinct osmolarities so that osmotic gradients…

Soft Condensed Matter · Physics 2016-03-23 T. Zhang , Duanduan Wan , J. M. Schwarz , M. J. Bowick

The surface tension of partially wetting droplets deforms soft substrates. These deformations are usually localized to a narrow region near the contact line, forming a so-called `elastocapillary ridge.' When a droplet slides along a…

Soft Condensed Matter · Physics 2024-10-30 Nan Xue , Lawrence A. Wilen , Robert W. Style , Eric R. Dufresne

The spontaneous migration of droplets on conical fibers is studied experimentally by depositing silicone oil droplets onto conical glass fibers. Their motion is recorded using optical microscopy and analysed to extract the relevant…

Soft Condensed Matter · Physics 2020-09-01 Clementine Fournier , Carmen Lee , Rafael Schulman , Elie Raphael , Kari Dalnoki-Veress

We study the influence of chain stiffness on droplet flow in a nano-channel, coated with semiflexible hydrophobic polymers by means of non-equilibrium molecular-dynamics simulations. The studied system is then a moving droplet in the slit…

Soft Condensed Matter · Physics 2017-10-18 Kevin Speyer , Claudio Pastorino

We present a comprehensive study of water drops sliding down chemically heterogeneous surfaces formed by a periodic pattern of alternating hydrophobic and hydrophilic stripes. Drops are found to undergo a stick-slip motion whose average…

Liquid droplets usually wet smooth and homogeneous substrates isotropically. Recent research works have revealed that droplets sit, slide and spread anisotropically on uniaxially stretched soft substrates, showing an enhanced wettability…

Soft Condensed Matter · Physics 2022-12-02 Yixuan Du , Elmar Bonaccurso , Jianwei Guo , Kai Uhlig , Longquan Chen , Binyu Zhao , Günter K. Auernhammer

Using multispeckle x-ray photon correlation spectroscopy, we have measured the slow, wave-vector dependent dynamics of concentrated, disordered nanoemulsions composed of silicone oil droplets in water. The intermediate scattering function…

Soft Condensed Matter · Physics 2007-05-23 H. Guo , J. N. Wilking , D. Liang , T. G. Mason , J. L. Harden , R. L. Leheny

Polymer gels are comprised of a three-dimensional, cross-linked network that can typically withstand the mechanical deformation associated with both swelling and de-swelling. Thus, gels can be designed with smart behaviors that require both…

Soft Condensed Matter · Physics 2024-06-24 Alyssa VanZanten , Shih-Yuan Chen , Michelle M. Driscoll , Caroline R. Szczepanski

Living and engineered systems rely on the stable coexistence of two interspersed liquid phases. Yet surface tension drives their complete separation. Here we show that stable droplets of uniform and tuneable size can be produced through…

We investigate the dynamics of alginate gels, an important class of biopolymer-based viscoelastic materials, by combining mechanical tests and non-conventional, time-resolved light scattering methods. Two relaxation modes are observed upon…

Soft Condensed Matter · Physics 2013-10-14 Domenico Larobina , Luca Cipelletti
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