Related papers: Vacancy Relaxation in Cuprous Oxide (Cu$_{2-x}$O$_…
Energy- and time-resolved spectroscopy reveals a photoinduced softening of the charge-transfer gap in the insulating copper oxide Sr2CuO2Cl2 that indicates rapid and efficient photoproduction of optical phonons. By relating the pump-probe…
An experimental study of the yellow exciton series in Cu2O in strong magnetic fields up to 32 T shows the optical activation of direct and phonon-assisted paraexciton luminescence due to mixing with the quadruple allowed orthoexciton state.…
Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…
The energy relaxation of carriers in reduced graphene oxide thin films is studied using optical pump-probe spectroscopy with two probes of different colors. We measure the time difference between peaks of the carrier density at each probing…
The ability to maintain coherence and control in a qubit is a major requirement for quantum computation. We show theoretically that long coherence times can be achieved above boiling point of liquid helium in charge qubits of oxide double…
The various decay mechanisms of excitons in cuprous oxide (Cu2O) are highly sensitive to defects which can relax selection rules. Here we report cryogenic hyperspectral imaging of exciton luminescence from cuprous oxide crystals grown via…
Phonon modes within pristine crystalline resonators now routinely reach the quantum ground state. Such systems are attractive for quantum information science applications, as advanced fabrication and processing can enable relatively long…
Oxygen vacancies are introduced in the RuO2 and possibly CuO2 planes of RuSr2GdCu2O8 by annealing in vacuum above 600 K. The diffusive jumps of the O vacancies are accompanied by a reorientation of the local distortion, and are probed by…
We address a long standing problem concerning the origin of bosonic excitations that strongly interact with charge carriers. We show that the time-resolved pump-probe experiments are capable to distinguish between regular bosonic degrees of…
Cuprates are promising candidates for study in developing higher temperature superconductors. A thorough understanding of a material's phonon modes enables further investigation of its emergent properties, however, no complete reference of…
The superconducting properties of high-\tc\ materials are functions of carriers concentration, which is controlled by the concentration of defects including heterovalent cations, interstitial oxygen ions, and oxygen vacancies. Here we…
Extrinsic levels, formation energies, and relaxation geometries are calculated ab initio for oxygen vacancies in alpha-quartz SiO2. The vacancy is found to be thermodynamically stable in the charge states Q=+3, Q=0, Q=--2, and Q=-3. The…
Time resolved measurements provide a new way to disentangle complex interactions in quantum materials due to their different timescales. We used pump-probe Raman scattering to investigate the apical oxygen vibration in…
Cu$_2$O has appealing properties as an electrode for photo-electrochemical water splitting, yet its practical performance is severely limited by inefficient charge extraction at the interface. Using hybrid DFT calculations, we investigate…
A short overview of theoretical models for the description of the relaxation processes in metals excited by a short laser pulse is presented. The main effort is given to description of different processes which are taking place after…
The role played by electronic and phononic excitations in the femtosecond laser induced desorption and oxidation of CO coadsorbed with O on Ru(0001) is investigated using ab initio molecular dynamics with electronic friction. To this aim,…
Matrix-operator difference-differential equations for dynamics of spectroscopic transitions in 1D multiqubit exchange coupled (para)magnetic and optical systems by strong dipole-photon and dipole-phonon coupling are derived within the…
Metals at the brink of electronic quantum phase transitions display high-temperature superconductivity, competing orders, and unconventional charge transport, revealing strong departures from conventional Fermi liquid behavior.…
Interpretation of experiments on quantum dot (QD) lasers presents a challenge: the phonon bottleneck, which should strongly suppress relaxation and dephasing of the discrete energy states, often seems to be inoperative. We suggest and…
The microscopic mechanism leading to stabilization of cubic and tetragonal forms of zirconia (ZrO$_2$) is analyzed by means of a self-consistent tight-binding model. Using this model, energies and structures of zirconia containing different…