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We propose an intuitive method, called time-dependent population imaging (TDPI), to map the dynamical processes of high harmonic generation (HHG) in solids by solving the time-dependent Schr\"{o}dinger equation (TDSE). It is shown that the…

Atomic Physics · Physics 2017-06-28 Xi Liu , Xiaosong Zhu , Pengfei Lan , Xiaofan Zhang , Dian Wang , Qingbin Zhang , Peixiang Lu

High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far…

Materials Science · Physics 2018-09-12 G. P. Zhang , M. S. Si , M. Murakami , Y. H. Bai , Thomas F. George

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

Atomic Physics · Physics 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

In frequently studied two-band models for solid-state high-harmonic generation, interband harmonics in principle can range from the minimum to the maximum bandgap. However, it is known that a laser-intensity dependent cutoff exists that may…

Optics · Physics 2024-03-13 Lina Bielke , Hannah Jürß , Vincent Burgtorf , Dieter Bauer

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We demonstrate a simple method to improve the Lewenstein model for the description of high-order harmonic generation (HHG). It is shown that HHG spectra can be expressed as the product of a returning electron wave packet and the…

Atomic Physics · Physics 2007-07-31 Anh-Thu Le , Toru Morishita , C. D. Lin

This paper focuses on investigating high-order harmonic generation (HHG) in graphene quantum dots (GQDs) under intense near-infrared laser fields. To model the GQD and its interaction with the laser field, we utilize a mean-field approach.…

Mesoscale and Nanoscale Physics · Physics 2023-09-15 H. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian

High harmonic generation (HHG) is a crucial technology for compact, high-brightness extreme ultraviolet (XUV) and soft X-ray sources, which are key to advancing both fundamental and applied sciences. The availability of advanced driving…

Optics · Physics 2025-10-07 Robert Klas , Martin Gebhardt , Jan Rothhardt , Jens Limpert

We report theoretical calculations of high harmonic generation (HHG) by intense infrared lasers in atomic and molecular targets taking into account the macroscopic propagation of both fundamental and harmonic fields. On the examples of Ar…

Atomic Physics · Physics 2011-02-28 Cheng Jin , Anh-Thu Le , C. D. Lin

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

Real-space picture of electron recollision with the parent ion guides our understanding of the highly nonlinear response of atoms and molecules to intense low-frequency laser fields. It is also among several leading contestants for the…

Optics · Physics 2019-11-06 Mrudul M. S. , Adhip Pattanayak , Misha Ivanov , Gopal Dixit

High-harmonic generation has emerged as a pivotal process in strong-field physics, yielding extreme ultraviolet radiation and attosecond pulses with a wide range of applications. Furthermore, its emergent connection with the field of…

We demonstrate that the strongly nonlinear regime of the magnetic dynamics driven high harmonic generation (HHG) can be captured through an adiabatic treatment. The underlying instantaneous energy dispersion reveal a highly nonlinear term…

Mesoscale and Nanoscale Physics · Physics 2024-06-26 O. Ly

By using the Floquet eigenstates, we derive a formula to calculate the high-harmonic components of the electric current (HHC) in the setup where a monochromatic laser field is turned on at some time. On the basis of this formulation, we…

Other Condensed Matter · Physics 2018-12-27 Tatsuhiko N. Ikeda , Koki Chinzei , Hirokazu Tsunetsugu

High-harmonic spectroscopy (HHS) is a nonlinear all-optical technique with inherent attosecond temporal resolution, which has been applied successfully to a broad variety of systems in the gas phase and solid state. Here, we extend HHS to…

High-order sideband generation (HSG), as an analogue of the interband processes in high-harmonic generation (HHG) in solids, is a nonperturbative nonlinear optical phenomenon in semiconductors that are simultaneously driven by a relatively…

Optics · Physics 2023-05-31 Qile Wu , Mark S. Sherwin

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…

Atomic Physics · Physics 2014-02-06 Francois Mauger , A. D. Bandrauk , Adam Kamor , Turgay Uzer , Cristel Chandre