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Although it is indeed commonly believed that, as frozen supercooled liquids, glasses should continue to flow over the years (e.g., in the case of the stained-glass windows of medieval cathedrals), the dramatic increase of their viscosity…

Disordered Systems and Neural Networks · Physics 2018-01-09 Yingtian Yu , John C. Mauro , Mathieu Bauchy

We propose an atomistic model for correlated particle dynamics in liquids and glasses predicting both slow stretched-exponential relaxation (SER) and fast compressed-exponential relaxation (CER). The model is based on the key concept of…

Statistical Mechanics · Physics 2021-08-11 K. Trachenko , A. Zaccone

Because the theory of SER is still a work in progress, the phenomenon itself can be said to be the oldest unsolved problem in science, as it started with Kohlrausch in 1847. Many electrical and optical phenomena exhibit SER with probe…

Soft Condensed Matter · Physics 2015-05-18 J. C. Phillips

A simple relaxation function I(t/tauzero; alpha, beta) unifying the stretched exponential with the compressed hyperbola is obtained, and its properties studied. The scaling parameter tauzero has dimensions of time, whereas the…

Computational Physics · Physics 2009-11-13 Mario Berberan-Santos

Glasses derive their functional properties from complex relaxation dynamics that remain enigmatic under extreme conditions. While the temperature dependence of these relaxation processes is well-established, their behavior under…

We propose a model of a heterogeneous glass forming liquid and compute the low-temperature behavior of a tagged molecule moving within it. This model exhibits stretched-exponential decay of the wavenumber-dependent, self intermediate…

Materials Science · Physics 2009-11-13 J. S. Langer , S. Mukhopadhyay

We analyze the density and size dependence of the relaxation time $\tau$ for kinetically constrained spin systems. These have been proposed as models for strong or fragile glasses and for systems undergoing jamming transitions. For the one…

Statistical Mechanics · Physics 2015-06-25 Nicoletta Cancrini , Fabio Martinelli , Cyril Roberto , Cristina Toninelli

By analyzing the experimental data for various glass-forming liquids and polymers, we find that non-exponentiality $\beta$ and the relaxation time $\tau$ are uniquely related: $\log(\tau)$ is an approximately linear function of $1/\beta$,…

Disordered Systems and Neural Networks · Physics 2008-07-15 K. Trachenko , C. M. Roland , R. Casalini

We develop a simple yet comprehensive nonlinear model to describe relaxation phenomena in amorphous glass-formers near the glass transition temperature. The model is based on the two-state, two-(time)scale (TS2) framework, and describes the…

Soft Condensed Matter · Physics 2024-03-12 Valeriy V. Ginzburg , Oleg V. Gendelman , Alessio Zaccone

Using Monte Carlo simulations we show that the autocorrelation function $C(t)$ in the d=3 Ising model with a plaquette interaction has a stretched-exponential decay in a supercooled liquid phase. Such a decay characterizes also some…

Statistical Mechanics · Physics 2015-06-11 Adam Lipowski

We identify a link between the glass transition and percolation of mobile regions in configuration space. We find that many hallmarks of glassy dynamics, for example stretched-exponential response functions and a diverging structural…

Statistical Mechanics · Physics 2009-11-13 Gregg Lois , Jerzy Blawzdziewicz , Corey S. O'Hern

The dynamics of glass-forming liquids display several outstanding features, such as two-step relaxation and dynamic heterogeneities, which are difficult to predict quantitatively from first principles. In this work, we revisit a simple…

Statistical Mechanics · Physics 2022-11-23 Daniele Coslovich , Atsushi Ikeda

Temporal relaxation of density fluctuations in supercooled liquids near the glass transition occurs in multiple steps. The short-time $\beta$-relaxation is generally attributed to spatially local processes involving the rattling motion of a…

Statistical Mechanics · Physics 2016-03-02 Smarajit Karmakar , Chandan Dasgupta , Srikanth Sastry

Recent experiments and computer simulations show that supercooled liquids around the glass transition temperature are "dynamically heterogeneous" [1]. Such heterogeneity is expected from the random first order transition theory of the glass…

Disordered Systems and Neural Networks · Physics 2009-10-31 Xiaoyu Xia , Peter G. Wolynes

We consider the diffusion constant, D, of a probe particle coupled to the East model, extending previous numerical results for this model to encompass a total of twelve orders of magnitude in relaxation time, {\tau}. Our considerations thus…

Statistical Mechanics · Physics 2013-09-24 YounJoon Jung , Soree Kim , Juan P. Garrahan , David Chandler

Simulations of a stochastic fixed-energy sandpile in one and two dimensions reveal slow relaxation of the order parameter, even far from the critical point. The decay of the activity is best described by a stretched-exponential form. The…

Statistical Mechanics · Physics 2009-11-07 Ronald Dickman

Diffusion on a diluted hypercube has been proposed as a model for glassy relaxation and is an example of the more general class of stochastic processes on graphs. In this article we determine numerically through large scale simulations the…

Statistical Mechanics · Physics 2015-05-28 N. Lemke , I. A. Campbell

Measured exponents associated with Stretched Exponential Relaxation (SER) are widely scattered in microscopically inhomogeneous glasses, but accurately bifurcate into two "magic" values, 3/5 and 3/7, in a wide variety of microscopically…

Soft Condensed Matter · Physics 2015-05-28 G. G. Naumis , J. C. Phillips

The spin glasses show intriguing characteristic features that are not well understood yet, as for instance its aging, rejuvenation and memory effects. Here a model based on a stretched exponential decay of its magnetization is proposed,…

Materials Science · Physics 2022-08-25 Leandro Bufaiçal

We perform a numerical simulation of energy relaxation in three-dimensional electron glasses in the strongly localized regime at finite temperatures. We consider systems with no interactions, with long-range Coulomb interactions and with…

Disordered Systems and Neural Networks · Physics 2009-10-31 A. Perez-Garrido , M. Ortuno , A. Diaz-Sanchez , E. Cuevas