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The change of bonding status, typically occurring only in chemical processes, could dramatically alter the material properties. Here, we show that a tunable breaking and forming of a diatomic bond can be achieved through physical means,…

Materials Science · Physics 2017-02-23 Yao Wang , Shan-Shan Wang , Yunhao Lu , Jianzhong Jiang , Shengyuan A. Yang

Charge doping is an effective way to induce metal-insulate transition (MIT) in correlated materials for many important utilizations, which is however practically limited by problem of low stability. In this study, we have achieved…

We analyze magnetic phases of monolayers of transition metal dichalcogenides that are two-valley materials with electron-electron interactions. The exchange inter-valley scattering makes two-valley systems less stable to the spin…

Strongly Correlated Electrons · Physics 2019-07-31 Dmitry Miserev , Jelena Klinovaja , Daniel Loss

Emergent order at mesoscopic length scales in condensed matter can provide fundamental insight into the underlying competing interactions and their relationship with the order parameter. Using spectromicroscopy, we show that mesoscopic…

Strongly Correlated Electrons · Physics 2019-03-14 J. Laverock , V. Jovic , A. A. Zakharov , Y. R. Niu , S. Kittiwatanakul , B. Westhenry , J. W. Lu , S. A. Wolf , K. E. Smith

Metal-ion doping can effectively regulate the metal-insulator transition temperature in $\mathrm{VO}_2$. Experiments found that the pentavalent and hexavalent ion doping dramatically reduces the transition temperature while the trivalent…

Materials Science · Physics 2020-01-09 Yin Shi , Long-Qing Chen

VO2 samples are grown with different oxygen concentrations leading to different monoclinic, M1 and triclinic, T insulating phases which undergo a first order metal to insulator transition (MIT) followed by a structural phase transition…

Materials Science · Physics 2017-05-12 Raktima Basu , Manas Sardar , Santanu Bera , P. Magudapathy , Sandip Dhara

Ultrathin freestanding membranes with a pronounced metal-insulator transition (MIT) provides huge potential in future flexible electronic applications as well as a unique aspect of the study of lattice-electron interplay. However, the…

Transition metal dichalcogenide superlattices provide an exciting new platform for exploring and understanding a variety of phases of matter. The moir\'e continuum Hamiltonian, of two-dimensional jellium in a modulating potential, provides…

Strongly Correlated Electrons · Physics 2024-02-16 Yubo Yang , Miguel Morales , Shiwei Zhang

The insulator-to-metal transition (IMT) of the simple binary compound of vanadium dioxide VO$_2$ at $\sim 340$ K has been puzzling since its discovery more than five decades ago. A wide variety of photon and electron probes have been…

Strongly Correlated Electrons · Physics 2014-12-18 Brian T. O'Callahan , Joanna M. Atkin , Andrew C. Jones , Jae Hyung Park , David Cobden , Markus B. Raschke

We discuss a metal-insulator transition caused by random couplings of magnetic moments in itinerant systems. An analytic solution for the single particle Green function is derived from dynamical self consistency equations, the corresponding…

Strongly Correlated Electrons · Physics 2007-05-23 B. Rosenow , R. Oppermann

Elucidating the polymorphism of transition metal dichalcogenide layers and the interplay between structure and properties is a key challenge for the application of these materials. We identify a novel low energy metastable phase of…

Strongly Correlated Electrons · Physics 2021-09-22 Bing-Hua Lei , David J. Singh

We investigate a disordered two-dimensional lattice model for noninteracting electrons with long-range power-law transfer terms and apply the method of level statistics for the calculation of the critical properties. The eigenvalues used…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 H. Potempa , L. Schweitzer

For inhomogeneous high-T_c superconductors, hole-driven metal-insulator transition (MIT) theory explains that the gradual increase of conductivity with increasing hole doping is due to inhomogeneity with the local Mott system undergoing the…

Strongly Correlated Electrons · Physics 2008-05-02 Hyun-Tak Kim , Bong-Jun Kim , Yong Wook Lee , Byung-Gyu Chae , Sun Jin Yun , Kwang-Yong Kang

A brief review of metal-insulator transitions in three-dimensional doped semiconductors, with emphasis on the "critical exponent puzzle"; and new experimental findings that signal the possibility of an unexpected metal-insulator transition…

Strongly Correlated Electrons · Physics 2009-09-25 Myriam P. Sarachik

The interplay between strong Coulomb interactions and randomness has been a long-standing problem in condensed matter physics. According to the scaling theory of localization, in two-dimensional systems of noninteracting or weakly…

Strongly Correlated Electrons · Physics 2007-05-23 S. V. Kravchenko , M. P. Sarachik

Optical anisotropy in crystalline solids enables direction-dependent light-matter interactions and underpins a variety of advanced photonic functionalities. In this context, Vanadium dioxide (VO2) represents a prototypical material that…

In strongly correlated transition metal dichalcogenides, an intricate interplay of polaronic distortions, stacking arrangement, and electronic correlations determines the nature of the insulating state. Here, we study the response of the…

New calculations for vanadium dioxide, one of the most controversely discussed materials for decades, reveal that band theory as based on density functional theory is well capable of correctly describing the electronic and magnetic…

Strongly Correlated Electrons · Physics 2011-07-07 V. Eyert

Ferromagnetism in the two-dimensional materials is of great significance and has become an emerging topic. The ferromagnetic VS$_2$ and VSe$_2$ monolayers have been experimentally synthesized, and O element belongs to the same group as S…

Materials Science · Physics 2025-03-14 Lihui Han , Lujia Tian , Bing-Xin Liu , Zong-liang Li , Miao Gao , Fengjie Ma , Xun-Wang Yan

Systematic spectroscopic ellipsometry investigations have been performed in order to elucidate the asymmetric insulator-to-metal transition in thin VO$_2$ films. The comprehensive analysis of the obtained macroscopic optical response yields…