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Angle-resolved Raman spectroscopy (ARRS) is an effective method to analyze the symmetry of phonons and other excitations in molecules and solid-state crystals. While there are several configurations of ARRS instruments, the measurement…

Undoubtedly, Raman spectroscopy is one of the most elaborated spectroscopy tools in materials science, chemistry, medicine and optics. However, when it comes to the analysis of nanostructured specimens, accessing the Raman spectra resulting…

Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to…

Instrumentation and Detectors · Physics 2018-07-10 Matthew N. Ashner , William A. Tisdale

Strain engineering in semiconductor transistor devices has become vital in the semiconductor industry due to the ever increasing need for performance enhancement at the nanoscale. Raman spectroscopy is a non-invasive measurement technique…

Optics · Physics 2021-06-17 V. Prabhakara , T. Nuytten , H. Bender , W. Vandervorst , S. Bals , J. Verbeeck

We review an on-chip approach for spontaneous Raman spectroscopy and Surface Enhanced Raman Spectroscopy (SERS) based on evanescent excitation of the analyte as well as evanescent collection of the Raman signal using Complementary Metal…

Stimulated Raman scattering (SRS) microscopy has emerged as a powerful technique for probing the spatiotemporal dynamics of molecular bonds with exceptional sensitivity, resolution, and speed. However, classically, its performance remains…

We report results and modelling of an experiment performed at the TAW Vulcan laser facility, aimed at investigating laser-plasma interaction in conditions which are of interest for the Shock Ignition scheme to Inertial Confinement Fusion,…

Nonlinear optical methods, such as coherent anti-Stokes Raman scattering (CARS) and stimulated Raman scattering (SRS), are able to perform label free imaging, with chemical bonds specificity. Here, we demonstrate that the use of circularly…

Surface-enhanced Raman spectroscopy (SERS) is a powerful tool for vibrational spectroscopy as it provides several orders of magnitude higher sensitivity than inherently weak spontaneous Raman scattering by exciting localized surface plasmon…

In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…

Chemical Physics · Physics 2019-11-28 Giovanni Batignani , Carino Ferrante , Giuseppe Fumero , Tullio Scopigno

Stimulated Raman scattering (SRS) microscopy is a powerful label-free imaging technique that probes the vibrational response of chemicals with high specificity and sensitivity. High-power, quantum-enhanced SRS microscopes have been recently…

Raman lasers based on integrated silica whispering gallery mode resonant cavities have enabled numerous applications from telecommunications to biodetection. To overcome the intrinsically low Raman gain value of silica, these devices…

Optics · Physics 2020-01-06 Hyungwoo Choi , Dongyu Chen , Fan Du , Rene Zeto , Andrea M Armani

Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and…

In this work, we present a high pulse energy multi-wavelength Raman laser spanning from 1.53 um up to 2.4 um by employing the cascaded rotational stimulated Raman scattering (SRS) effect in a 5-m hydrogen (H2) -filled nested anti-resonant…

By measuring the thermal effects resulting from stimulated Raman excitations, stimulated Raman photothermal (SRP) microscope offers a new access to spatially and temporally resolved Raman signatures across various sample types. Unlike…

Optics · Physics 2026-03-03 Yifan Zhu , Hongli Ni , Hongjian He , Yueming Li , Meng Zhang , Ji-Xin Cheng

We present a novel approach to achieve hyper spectral resolution, high sensitive detection, and high speed data acquisition Stimulated Raman Spectroscopy by employing amplified offset-phase controlled fs-pulse bursts. In this approach, the…

Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…

Optics · Physics 2024-08-13 Minhaeng Cho

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

Charge-density waves (CDWs) are ordered quantum states of conduction electrons accompanied by periodic lattice distortions. Raman scattering (RS) spectroscopy is therefore well suited for probing CDW-induced structural modulations. We…

We report a singly resonant continuous-wave optical parametric oscillator (SRO), which is pumped by a semiconductor laser system and operates in the mid-infrared region (2.9 to 3.6 {\mu}m). Fast tuning of the mid-infrared output wavelength…

Optics · Physics 2018-07-06 Ville Ulvila , Markku Vainio