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Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Demagnetization in ferromagnetic transition metals driven by a femtosecond laser pulse is a fundamental problem in solid state physics, and its understanding is essential to the development of spintronics devices. Ab initio calculation of…

Materials Science · Physics 2024-01-02 Mitsuko Murakami , G. P. Zhang

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

Materials Science · Physics 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Induced by an ultra-short laser pulse, the electronic structure of a material undergoes strong modifications leading to a fast demagnetization in magnetic materials. Induced spin-flip transitions are one of the reasons for demagnetization,…

Materials Science · Physics 2024-04-29 Sergiy Mankovsky , Svitlana Polesya , Hubert Ebert

The dynamics of ultrafast demagnetisation in 3$d$ magnets is complicated by the presence of both spin ${\v S}$ and orbital ${\v L}$ angular momentum, with the microscopic mechanism by which the magnetic moment is redistributed to the…

Materials Science · Physics 2021-09-01 J. K. Dewhurst , S. Shallcross , P. Elliott , S. Eisebitt , C. v. Korff Schmising , Sangeeta Sharma

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr$_{2}$O$_{3}$. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast…

Strongly Correlated Electrons · Physics 2017-06-29 Feng Guo , Na Zhang , Wei Jin , Jun Chang

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

Materials Science · Physics 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

It is now well established that a laser pulse can demagnetize a ferromagnet. However, for a long time, it has not had an analytic theory because it falls into neither nonlinear optics (NLO) nor magnetism. Here we attempt to fill this gap by…

Materials Science · Physics 2025-10-30 G. P. Zhang , Y. H. Bai , Thomas F. George

Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

Materials Science · Physics 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

The ultrafast demagnetization (UFD) dynamics of itinerant ferromagnets is theoretically investigated as a function of the characteristics of the initial laser excitation. A many-body pd-band Hamiltonian is considered which takes into…

Strongly Correlated Electrons · Physics 2019-07-10 W. Töws , G. M. Pastor

Laser-induced demagnetization is theoretically studied by explicitly taking into account interactions among electrons, spins and lattice. Assuming that the demagnetization processes take place during the thermalization of the sub-systems,…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 A. Manchon , Q. Li , L. Xu , S. Zhang

With the goal of pushing Spintronic devices towards faster and faster timescales, we demonstrate, using ab-intio time-dependent density functional theory simulations of bulk Heusler compounds subject to ultrashort intense laser pulses, that…

Materials Science · Physics 2016-03-18 P. Elliott , T. Müller , J. K. Dewhurst , S. Sharma , E. K. U. Gross

A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films. Experimentally dynamics of spins is studied by determining the time-dependent…

Laser induced modulation of the magnetization dynamics occurring over various time-scales have been unified here for a Ni80Fe20 thin film excited by amplified femtosecond laser pulses. The weak correlation between demagnetization time and…

Mesoscale and Nanoscale Physics · Physics 2018-12-21 Sucheta Mondal , Anjan Barman

Since the discovery of ultrafast demagnetization in Ni thin films in 1996, laser-induced ultrafast spin dynamics have become a prominent research topic in the field of magnetism and spintronics. This development offers new possibilities for…

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