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We consider two weakly coupled systems and adopt a perturbative approach based on the Ruelle response theory to study their interaction. We propose a systematic way to parametrize the effect of the coupling as a function of only the…

Statistical Mechanics · Physics 2012-08-16 Jeroen Wouters , Valerio Lucarini

We generalize the Aufbau suppressed coupled cluster formalism into the realm of doubly excited states by deriving, implementing, and testing a wave function initialization strategy that allows the zeroth order wave function to match the…

Chemical Physics · Physics 2026-05-11 Qasim Javed , Harrison Tuckman , Eric Neuscamman

Recently a number of analytic prescriptions for computing the non-linear matter power spectrum have appeared in the literature. These typically involve resummation or closure prescriptions which do not have a rigorous error control, thus…

Cosmology and Nongalactic Astrophysics · Physics 2009-11-06 Jordan Carlson , Martin White , Nikhil Padmanabhan

We develop and test methods that include second and third-order perturbation theory (MP3) using orbitals obtained from regularized orbital-optimized second-order perturbation theory, $\kappa$-OOMP2, denoted as MP3:$\kappa$-OOMP2. Testing…

Chemical Physics · Physics 2019-10-15 Luke W. Bertels , Joonho Lee , Martin Head-Gordon

Particle MCMC involves using a particle filter within an MCMC algorithm. For inference of a model which involves an unobserved stochastic process, the standard implementation uses the particle filter to propose new values for the stochastic…

Computation · Statistics 2016-09-26 Paul Fearnhead , Loukia Meligkotsidou

This research identifies a gap in weakly-labelled multivariate time-series classification (TSC), where state-of-the-art TSC models do not per-form well. Weakly labelled time-series are time-series containing noise and significant…

Machine Learning · Computer Science 2021-09-20 Surayez Rahman , Chang Wei Tan

In various applications with large spatial regions, the relationship between the response variable and the covariates is expected to exhibit complex spatial patterns. We propose a spatially clustered varying coefficient model, where the…

Methodology · Statistics 2020-07-21 Fangzheng Lin , Yanlin Tang , Huichen Zhu , Zhongyi Zhu

This chapter presents the theory behind the CASPT2 method and its adaptation to a multi-state formalism. The chapter starts with an introduction of the theory of the CASPT2 method - an application of Rayleigh-Schr\"odinger perturbation…

Chemical Physics · Physics 2023-05-12 Stefano Battaglia , Ignacio Fdez. Galván , Roland Lindh

We propose a modified coupled cluster Monte Carlo algorithm that stochastically samples connected terms within the truncated Baker--Campbell--Hausdorff expansion of the similarity transformed Hamiltonian by construction of coupled cluster…

Chemical Physics · Physics 2019-06-19 Charles J. C. Scott , Roberto Di Remigio , T. Daniel Crawford , Alex J. W. Thom

We propose a clustered local projection (clustered LP) method to estimate impulse response functions in a class of time-varying models where parameter variation is linked to a low-dimensional matrix of observables. We show that the…

Econometrics · Economics 2026-05-04 Ana Maria Herrera , Elena Pesavento , Alessia Scudiero

We construct a novel class of stochastic blockmodels using Bayesian nonparametric mixtures. These model allows us to jointly estimate the structure of multiple networks and explicitly compare the community structures underlying them, while…

Methodology · Statistics 2016-06-17 Perla Reyes , Abel Rodriguez

We introduce perturbation and coupled-cluster theories based on a cluster mean-field reference for describing the ground state of strongly-correlated spin systems. In cluster mean-field, the ground state wavefunction is written as a simple…

While limited coupled cluster theory is \textit{formally} nonvariational, it is not broadly appreciated whether this is a major issue \textit{in practice}. We carried out a detailed comparison with \textit{de facto} full CI energies for a…

Chemical Physics · Physics 2024-10-03 Jan M. L. Martin , Emmanouil Semidalas

We develop an algorithm which can learn from partially labeled and unsegmented sequential data. Most sequential loss functions, such as Connectionist Temporal Classification (CTC), break down when many labels are missing. We address this…

Machine Learning · Computer Science 2022-03-07 Vineel Pratap , Awni Hannun , Gabriel Synnaeve , Ronan Collobert

The multiscale model combining the multiconfigurational self-consistent field (MCSCF) method with the fully atomistic polarizable Fluctuating Charges (FQ) force field (J. Chem. Theory Comput. 2024, 20, 9954-9967) is here extended to the…

Chemical Physics · Physics 2025-11-14 Francesco Mazza , Marco Trinari , Chiara Sepali , Chiara Cappelli

The Chord Length Sampling (CLS) algorithm is a powerful Monte Carlo method that models the effects of stochastic media on particle transport by generating on-the-fly the material interfaces seen by the random walkers during their…

Statistical Mechanics · Physics 2018-03-14 Colline Larmier , Adam Lam , Patrick Brantley , Fausto Malvagi , Todd Palmer , Andrea Zoia

We investigate a stochastic version of the synthetic multicellular clock model proposed by Garcia-Ojalvo, Elowitz and Strogatz. By introducing dynamical noise in the model and assuming that the partial observations of the system can be…

Computation · Statistics 2015-12-15 Inés P. Mariño , Joaquin Miguez , Alexey Zaikin

In this paper, we address the problem of designing stochastic model predictive control (MPC) schemes for linear systems affected by unbounded disturbances. The contribution of the paper is twofold. First, motivated by the difficulty of…

Systems and Control · Electrical Eng. & Systems 2024-06-21 Mirko Fiacchini , Martina Mammarella , Fabrizio Dabbene

Ab initio methods based on the second-order and higher connected moments, or cumulants, of a reference function have seen limited use in the determination of correlation energies of chemical systems throughout the years. Moment-based…

Chemical Physics · Physics 2023-08-25 Brad Ganoe , Martin Head-Gordon

As a very popular multi-label classification method, Classifiers Chain has recently been widely applied to many multi-label classification tasks. However, existing Classifier Chains methods are difficult to model and exploit the underlying…

Artificial Intelligence · Computer Science 2022-04-14 Gao Pengfei , Lai Dedi , Zhao Lijiao , Liang Yue , Ma Yinglong