Related papers: Time-resolved spectroscopy with entangled photons
We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…
In this theoretical study we demonstrate that entangled states are able to significantly extend the functionality of Hong-Ou-Mandel (HOM) interferometers. By generating a coherent superposition of parametric-down-conversion photons and…
We theoretically investigate the quantum interference of entangled two-photon states generated in a nonlinear crystal pumped by femtosecond optical pulses. Interference patterns generated by the polarization analog of the Hong-Ou-Mandel…
High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also…
Resonance fluorescence in the Heitler regime provides access to single photons with coherence well beyond the Fourier transform limit of the transition, and holds the promise to circumvent environment-induced dephasing common to all…
We examine the precision limits of Hong-Ou-Mandel (HOM) timing measurements, as well as precision limits applying to generalized two-photon measurements. As a special case, we consider the use of two-photon measurements using photons with…
The multiple scattering of coherent light is a problem of both fundamental and applied importance. In optics, phase conjugation allows spatial focussing and imaging through a multiply scattering medium; however, temporal control is…
Hong-Ou-Mandel (HOM) interference is an intrinsic quantum phenomena that goes beyond the possibilities of classical physics, and enables various applications in quantum metrology. While the timing resolution of HOM-based sensor is generally…
Time-resolved scattering experiments enable imaging of materials at the molecular scale with femtosecond time resolution. However, in disordered media they provide access to just one radial dimension thus limiting the study of orientational…
When two indistinguishable photons are each incident on separate input ports of a beamsplitter they `bunch' deterministically, exiting via the same port as a direct consequence of their bosonic nature. This two-photon interference effect…
It depends. For a single molecule interacting with one mode of a biphoton probe, we show that the spectroscopic information has three contributions, only one of which is a genuine two-photon contribution. When all the scattered light can be…
Spectroscopy is a well-established nonintrusive tool that has played an important role in identifying substances and quantifying their compositions, from quantum descriptions to chemical and biomedical diagnostics. Challenges exist in…
Conventional femtosecond coherent laser spectroscopy predominantly focuses on the temporal phase coherence through time- or frequency-resolved methods. In this work, we suggest an alternative experimental framework based on spatial phase…
The photoexcited state in superconducting metals and alloys was studied via pump-probe spectroscopy. A pulsed Ti:sapphire laser was used to create the non-equilibrium state and the far-infrared pulses of a synchrotron storage ring, to which…
Based on the second-order quantum interference between frequency entangled photons that are generated by parametric down conversion, a quantum strategic algorithm for synchronizing two spatially separated clocks has been recently presented.…
We present a quantum optical scheme for imaging transversely displaced thermal sources of arbitrary intensities by employing multiphoton interference with a reference single-photon Fock state at a beamsplitter. Obtaining an analytical form…
Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…
Unveiling and controlling the coherent evolution of low energy states is a key to attain light driven new functionalities of materials. Here we investigate the coherent evolution of non-equilibrium photon-phonon Raman interactions in the…
The quantum interference of entangled photons forms a key phenomenon underlying various quantum-optical technologies. It is known that the quantum interference patterns of entangled photon pairs can be reconstructed classically by the…
A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…