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Time-resolved ultrafast x-ray scattering is an emerging approach to probe the temporally evolving electronic charge distribution in real-space and in real-time. In this contribution, time-resolved ultrafast x-ray scattering from an…

Atomic Physics · Physics 2015-06-18 Gopal Dixit , Robin Santra

We studied the photoelectron spectra generated by an intense few-cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering…

Atomic Physics · Physics 2008-04-04 T Morishita , A. T. Le , Z. Chen , C. D. Lin

We present a computationally efficient model that describes the interaction of intense, ultrashort infrared laser pulses with transparent materials in the strong ionization regime. The model is augmented with a detailed self-consistent…

Plasma Physics · Physics 2026-03-20 Julia Apportin , Christian Peltz , Pavel Polynkin , Misha Ivanov , Thomas Fennel , Anton Husakou

Transient X-ray absorption techniques can measure ultrafast dynamics of the elemental edges in a material or multiple layer junction, giving them immense potential for deconvoluting concurrent processes. However, the interpretation of the…

Materials Science · Physics 2021-06-10 Hanzhe Liu , Isabel M. Klein , Jonathan M. Michelsen , Scott K. Cushing

A cluster deposition method was used to produce films of loosely aggregated nanoclusters (NC) of Fe core-Fe3O4 shell or fully oxidized Fe3O4. Films of these NC on Si(100) or MgO(100)/Fe3O4(100) were irradiated to 10^16 Si2+/cm2 near room…

A novel scheme is proposed to generate uniform relativistic electron layers for coherent Thomson backscattering. A few-cycle laser pulse is used to produce the electron layer from an ultra-thin solid foil. The key element of the new scheme…

Plasma Physics · Physics 2015-03-13 Hui-Chun Wu , Juergen Meyer-ter-Vehn , Juan C. Fernandez , B. Manuel Hegelich

We report on measurements of visible extinction spectra of semicontinuous silver nanoshells grown on colloidal silica spheres. We find that thin, fractal shells below the percolation threshold exhibit geometrically tunable plasmon…

Optics · Physics 2009-11-11 Charles A. Rohde , Keisuke Hasegawa , Miriam Deutsch

We present results from the SPring-8 Angstrom Compact free electron LAser (SACLA) XFEL facility, using a high intensity ($\sim\!10^{20}\,$W/cm$^2$) X-ray pump X-ray probe scheme to observe changes in the ionic structure of silicon induced…

With a state-of-the-art numerical method for solving the integral-differential equation of radiative transfer, we investigate the flux of the Ly$\alpha$ photon $\nu_0$ emergent from an optically thick halo containing a central light source.…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-18 Ishani Roy , Chi-Wang Shu , Li-Zhi Fang

Nanoparticles supporting a distinct series of Mie resonances have enabled a new class of nanoantennas and provide efficient ways to manipulate light at the nanoscale. The ability to flexibly tune the optical resonances and scattering…

Optics · Physics 2021-05-26 Yiwei Dong , Yuanqing Yang

We propose a new concept of an electron source for ultrafast electron diffraction with sub-10~fs temporal resolution. Electrons are generated in a laser-plasma accelerator, able to deliver femtosecond electron bunches at 5 MeV energy with…

Accelerator Physics · Physics 2016-04-20 J. Faure , B. van der Geer , B. Beaurepaire , G. Gallé , A. Vernier , A. Lifschitz

The photoelectron momentum distribution in the strong-field ionization has a variety of structures that reveal the complicated dynamics of this process. Recently, we identified a low-energy interference structure in the case of a…

Atomic Physics · Physics 2022-04-27 Lei Geng , Hao Liang , Liang-You Peng

X-ray free-electron lasers (FELs) are promising tools for structural determination of macromolecules via coherent x-ray scattering. During ultrashort and ultraintense x-ray pulses with an atomic scale wavelength, samples are subject to…

Atomic Physics · Physics 2011-10-18 Sang-Kil Son , Linda Young , Robin Santra

We reconstructed intensities in Fourier space and electron densities in the real space for an azimuthally symmetric object Nanorice particle (Iron Oxide nanoparticle) exposed in the ultrashort, bright and coherent x-ray free electron laser…

Biological Physics · Physics 2020-07-14 S. S. Kim , P. Nepal , D. K. Saldin , C. H. Yoon

We report on time-resolved coherent diffraction imaging of gas-phase silver nanoparticles, strongly heated via their plasmon resonance. The x-ray diffraction images reveal a broad range of phenomena for different excitation strengths, from…

Not long after the laser was invented, it has been marked as a candidate source of strong, high-frequency electromagnetic radiation for acceleration of particles. Indeed, while the complex particle accelerator facilities today are an…

Accelerator Physics · Physics 2022-05-25 Roy Shiloh , Tomas Chlouba , Peter Hommelhoff

Laser-assisted electron scattering (LAES), a light-matter interaction process that facilitates energy transfer between strong light fields and free electrons, has so far been observed only in gas phase. Here we report on the observation of…

We propose an imaging technique to follow core-hole wave-packet oscillations in the nitrogen molecule. In this scheme, an attosecond x-ray pulse core-ionizes the nitrogen molecule and a subsequent attosecond x-ray pulse probes the evolution…

Chemical Physics · Physics 2019-08-15 Ludger Inhester , Loren Greenman , Artem Rudenko , Daniel Rolles , Robin Santra

The interaction of intense extreme ultraviolet (XUV) laser pulses ($\lambda=32\rm\,nm$, $I=10^{11-14}$\,W/cm$^2$) with small rare-gas clusters (Ar$_{147}$) is studied by quasi-classical molecular dynamics simulations. Our analysis supports…

Atomic and Molecular Clusters · Physics 2010-09-01 Mathias Arbeiter , Thomas Fennel
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