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Heat transport in bulk materials is well described using the Debye theory of 3D vibrational modes (phonons) and the acoustic match model. However, in cryogenic nanodevices, phonon wavelengths exceed device dimensions, leading to confinement…

Mesoscale and Nanoscale Physics · Physics 2024-10-14 M. Sidorova , A. D. Semenov , A. Zaccone , I. Charaev , M. Gonzalez , A. Schilling , S. Gyger , S. Steinhauer

We present an \emph{ab-initio} study that identifies the main electron-phonon scattering channels in $n$-type PbTe. We develop an electronic transport model based on the Boltzmann transport equation within the transport relaxation time…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 Jiang Cao , Jose D. Querales-Flores , Aoife R. Murphy , Stephen Fahy , Ivana Savić

We study heat transport in semiconductor nanostructures by solving the Boltzmann Transport Equation (BTE) by means of the Discrete Ordinate Method (DOM). Relaxation time and phase and group velocitiy spectral dependencies are taken into…

Classical Physics · Physics 2009-11-13 Damian Terris , Karl Joulain , David Lacroix , Denis Lemonnier

While thermal anisotropicity is a desirable materials property for many applications, including transverse thermoelectrics and thermal management in electronic devices, it remains elusive in practical natural compounds. In this work, we…

Materials Science · Physics 2017-04-05 Giuseppe Romano , Alexie M. Kolpak

We present ab-initio phonon dispersion relations for the three lead chalcogenides PbS, PbSe, and PbTe. The acoustic branches are in very good agreement with inelastic neutron-scattering data and calculations of the specific heat give good…

Materials Science · Physics 2013-08-07 Ondrej Kilian , Guy Allan , Ludger Wirtz

Efficient and precise calculations of thermal transport properties and figure of merit, alongside a deep comprehension of thermal transport mechanisms, are essential for the practical utilization of advanced thermoelectric materials. In…

We study nondiffusive thermal transport by phonons at small distances within the framework of the Boltzmann transport equation (BTE) and demonstrate that the transport is significantly affected by the distribution of phonons emitted by the…

Mesoscale and Nanoscale Physics · Physics 2017-10-05 Vazrik Chiloyan , Samuel Huberman , Alexei A. Maznev , Keith A. Nelson , Gang Chen

Dislocations can greatly enhance the figure of merit of thermoelectric materials by prominently reducing thermal conductivity. However, the evolution of phonon modes with different energies when they propagate through a single dislocation…

Applied Physics · Physics 2019-10-07 Yandong Sun , Yanguang Zhou , Jian Han , Wei Liu , Cewen Nan , Yuanhua Lin , Ming Hu , Ben Xu

Two-dimensional transition metal dichalcogenides (TMDCs) are finding promising electronic and optical applications due to their unique properties. In this letter, we systematically study the phonon transport and thermal conductivity of…

Materials Science · Physics 2014-09-30 Xiaokun Gu , Ronggui Yang

Phonon Boltzmann transport equation (BTE) is an important tool for studying the nanoscale thermal transport. Because phonons have a large spread in their properties, the non-gray (i.e. considering different phonon bands) phonon BTE is…

Computational Physics · Physics 2021-09-29 Yue Hu , Yongxing Shen , Hua Bao

Intervalley collisions, which scatter electrons from one valley or band to another, can be detrimental to thermoelectric performance in materials with multiple valleys/bands. In this study, density functional theory is used to investigate…

Materials Science · Physics 2023-02-08 Vahid Askarpour , Jesse Maassen

Understanding the microscopic processes affecting the bulk thermal conductivity is crucial to develop more efficient thermoelectric materials. PbTe is currently one of the leading thermoelectric materials, largely thanks to its low thermal…

Materials Science · Physics 2011-06-07 O. Delaire , J. Ma , K. Marty , A. F. May , M. A. McGuire , M. -H. Du , D. J. Singh , A. Podlesnyak , G. Ehlers , M. Lumsden , B. C. Sales

Two-dimensional (2-D) transition metal dichalcogenides (TMDs) have shown numerous interesting physical and chemical properties, making them promising materials for electronic, optoelectronic, and energy applications. Tuning thermal…

Materials Science · Physics 2016-09-07 Xiaokun Gu , Ronggui Yang

We determine the size effect on the lattice thermal conductivity of nanoscale wire and multilayer structures formed in and by some typical semiconductor materials, using the Boltzmann transport equation and focusing on the Knudsen flow…

Materials Science · Physics 2009-11-11 Eleni Ziambaras , Per Hyldgaard

It has been proposed for a long time now that the reduction of the thermal conductivity by reducing the phonon mean free path is one of the best way to improve the current performance of thermoelectrics. By measuring the thermal conductance…

By using a first-principles approach, monolayer PbI$_2$ is found to have great potential in thermoelectric applications. The linear Boltzmann transport equation is applied to obtain the perturbation to the electron distribution by different…

Materials Science · Physics 2021-05-24 Bo Peng , Haodong Mei , Hao Zhang , Hezhu Shao , Ke Xu , Gang Ni , Qingyuan Jin , Costas M. Soukoulis , Heyuan Zhu

We calculate the thermal conductivity of free-standing silicene using the phonon Boltzmann transport equation within the relaxation time approximation. In this calculation, we investigate the effects of sample size and different scattering…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 M. Barati , T. Vazifehshenas , T. Salavati-fard , M. Farmanbar

We thoroughly investigate the microscopic mechanisms of the thermal transport in orthorhombic \textit{o}-CsCu$_5$S$_3$ by integrating the first-principles-based self-consistent phonon calculations (SCP) with the linearized Wigner transport…

Materials Science · Physics 2024-04-17 Jincheng Yue , Jiongzhi Zheng , Junda Li , Siqi Guo , Wenling Ren , Han Liu , Yanhui Liu , Tian Cui

Biphenylene nanotubes (BPNNTs) represent a novel class of carbon-based nanomaterials, constructed by rolling a biphenylene network (BPN) monolayer into a one-dimensional tubular structure. In this study, the thermal transport properties of…

Materials Science · Physics 2025-09-24 Jhionathan de Lima , Cristiano F. Woellner

The thermal transport properties of single-wall carbon nanotubes (SWCNTs) are re-investigated using the iterative solution of the Boltzmann transport equation by including four-phonon scattering. Using only three-phonon scattering, the…

Materials Science · Physics 2023-11-07 Ankit Jain