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Control over the charge states of color centers in solids is necessary in order to fully utilize them in quantum technologies. However, the microscopic charge dynamics of deep defects in wide-bandgap semiconductors are complex, and much…

Mesoscale and Nanoscale Physics · Physics 2021-09-08 A. Gardill , I. Kemeny , M. C. Cambria , Y. Li , H. T. Dinani , A. Norambuena , J. R. Maze , V. Lordi , S. Kolkowitz

The fluorescent nitrogen-vacancy (NV) defect in diamond has remarkable photophysical properties, including high photostability, which allows stable fluorescence emission for hours; as a result, there has been much interest in using…

The charge degree of freedom in solid-state defects fundamentally underpins the electronic spin degree of freedom, a workhorse of quantum technologies. Here we study charge state properties of individual near-surface nitrogen-vacancy (NV)…

Mesoscale and Nanoscale Physics · Physics 2019-02-26 Dolev Bluvstein , Zhiran Zhang , Ania C. Bleszynski Jayich

In recent years, solid-state spin systems have emerged as promising candidates for quantum information processing (QIP). Prominent examples are the Nitrogen-Vacancy (NV) center in diamond, phosphorous dopants in silicon (Si:P), rare-earth…

Nitrogen-vacancy (NV) centers in diamond have attracted considerable interest in sensing of weak magnetic fields, such as those created by biological systems. Detecting such feeble signals requires near-surface NV centers, to reduce the…

Mesoscale and Nanoscale Physics · Physics 2019-05-01 R. Giri , C. Dorigoni , S. Tambalo , F. Gorrini , A. Bifone

Nitrogen vacancy (NV-) color centers in diamond are a prime candidate for use in quantum information devices, owing to their spin-1 ground state, straightforward optical initialization and readout, and long intrinsic coherence times in a…

Quantum Physics · Physics 2015-06-19 Anna J. Parker , Hai-Jing Wang , Yiran Li , Alexander Pines , Jonathan P. King

We utilize nonlinear absorption to design all-optical protocols that improve both charge state initialization and spin readout for the nitrogen-vacancy (NV) center in diamond. Non-monotonic variations in the equilibrium charge state as a…

Quantum Physics · Physics 2016-12-14 David A. Hopper , Richard R. Grote , Annemarie L. Exarhos , Lee C. Bassett

A dense layer of nitrogen-vacancy (NV) centers near the surface of a diamond can be interrogated in a widefield optical microscope to produce spatially resolved maps of local quantities such as magnetic field, electric field and lattice…

We demonstrate fully three-dimensional and patterned localization of nitrogen-vacancy (NV) centers in diamond with coherence times in excess of 1 ms. Nitrogen {\delta}-doping during CVD diamond growth vertically confines nitrogen to 4 nm…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Claire A. McLellan , Bryan A. Myers , Stephan Kraemer , Kenichi Ohno , David D. Awschalom , Ania C. Bleszynski Jayich

The nitrogen-vacancy (NV) center in diamond exists in different charge states with distinct photoluminescence properties, which are sensitive to the nanoscale electrochemical environment. Hence, the NV charge state is emerging as a powerful…

Mesoscale and Nanoscale Physics · Physics 2026-05-12 Patrick Voorhoeve , Hiroshi Abe , Takeshi Ohshima , Qiang Sun , Anita Quigley , Rob Kapsa , Nikolai Dontschuk , Philipp Reineck

Nanodiamonds containing negatively charged nitrogen vacancy centres (${\text{NV}}^{-}$) have applications as localized sensors in biological material and have been proposed as a platform to probe the macroscopic limits of spatial…

Nitrogen-vacancy centres (NVs) in diamond are attractive for research straddling quantum information science and nanoscale magnetometry and thermometry. While ultrapure bulk diamond NVs sustain the longest spin coherence times among…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Helena S. Knowles , Dhiren M. Kara , Mete Atature

Optically active solid-state spin defects have the potential to become a versatile resource for quantum information processing applications. Nitrogen-vacancy defect centers (NV) in diamond act as quantum memories and can be interfaced by…

Although the spin properties of superficial shallow nitrogen-vacancy (NV) centers have been the subject of extensive scrutiny, considerably less attention has been devoted to studying the dynamics of NV charge conversion near the diamond…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 Siddharth Dhomkar , Harishankar Jayakumar , Pablo R. Zangara , Carlos A. Meriles

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol…

Quantum Physics · Physics 2023-08-14 Abhishek Kejriwal , Dasika Shishir , Sumiran Pujari , Kasturi Saha

The nitrogen-vacancy center (NV) in diamond, with its exceptional spin coherence and convenience in optical spin initialization and readout, is increasingly used both as a quantum sensor and as a building block for quantum networks.…

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical…

Quantum Physics · Physics 2015-03-05 Yiwen Chu , Matthew Markham , Daniel J. Twitchen , Mikhail D. Lukin

The nitrogen-vacancy (NV) center spin represents an appealing candidate for quantum information processing. Besides the widely used microwave control, its coherent manipulation may also be achieved using laser as mediated by the excited…

Quantum Physics · Physics 2022-05-05 Jiazhao Tian , Tianyi Du , Yu Liu , Haibin Liu , Fangzhou Jin , Ressa S. Said , Jianming Cai

As a potential candidate for quantum computation and metrology, the nitrogen vacancy (NV)center in diamond presented both challenges and opportunities resulted from charge state conversion. By utilizing different lasers for the…

Quantum Physics · Physics 2014-10-20 Xiangdong Chen , Changling Zou , Zhaojun Gong , Chunhua Dong , Guangcan Guo , Fangwen Sun

Recent advancements in quantum technology have highlighted the potential of nitrogen-vacancy (NV) centers in diamond. However, fully realizing this potential requires addressing challenges related to the size, complexity, and cost of…