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We study the depolarization dynamics of a dense ensemble of dipolar interacting spins, associated with nitrogen-vacancy centers in diamond. We observe anomalously fast, density-dependent, and non-exponential spin relaxation. To explain…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol…

Quantum Physics · Physics 2023-08-14 Abhishek Kejriwal , Dasika Shishir , Sumiran Pujari , Kasturi Saha

An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

We perform sensitive nuclear magnetic resonance (NMR) with spin ensembles which are polarized by nitrogen vacancy centers (NV centers) in diamond at room-temperature. With a near shot-noise-limited photoluminescence detection and a highly…

We study the coupling of a single nitrogen-vacancy center in diamond to a nearby single nitrogen defect at room temperature. The magnetic dipolar coupling leads to a splitting in the electron spin resonance frequency of the nitrogen-vacancy…

Quantum Physics · Physics 2007-05-23 R. Hanson , F. M. Mendoza , R. J. Epstein , D. D. Awschalom

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Nan Zhao , Jörg Wrachtrup , Ren-Bao Liu

The long coherence time of a single nitrogen vacancy (NV) center spin in diamond is a crucial advantage for implementing quantum information processing. However, the realization of strong coupling between single NV spins is challenging.…

Quantum Physics · Physics 2021-05-19 Wei Xiong , Jiaojiao Chen , Baolong Fang , Mingfeng Wang , Liu Ye , J. Q. You

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

Quantum Physics · Physics 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy…

Quantum Physics · Physics 2013-04-01 Ran Fischer , Andrey Jarmola , Pauli Kehayias , Dmitry Budker

Systems of spins with strong dipolar interactions and controlled dimensionality enable new explorations in quantum sensing and simulation. In this work, we investigate the creation of strong dipolar interactions in a two-dimensional…

The nitrogen-vacancy (NV) center in diamond is of high importance in quantum information processing applications which relies on the efficient optical polarization of its electron spin. However, the full optical spinpolarization process, in…

Quantum Physics · Physics 2018-09-12 Gergő Thiering , Adam Gali

We experimentally investigate the protection of electron spin coherence of nitrogen vacancy (NV) center in diamond by dynamical nuclear polarization. The electron spin decoherence of an NV center is caused by the magnetic ield fluctuation…

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

Understanding fully the dynamics of coupled electron-nuclear spin systems, which are important for the development of long-lived qubits based on solid-state systems, remains a challenge. We show that in a singly charged semiconductor…

Mesoscale and Nanoscale Physics · Physics 2010-07-26 Wenxian Zhang , Jian-Liang Hu , Jun Zhuang , J. Q. You , Ren-Bao Liu

We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two…

Quantum Physics · Physics 2024-01-17 Shishir Khandelwal , Shashwat Kumar , Nicolas Palazzo , Géraldine Haack , Mayeul Chipaux

Spin ensembles of nitrogen vacancy (NV) centers in diamond are emerging as powerful spin-based sensors for magnetic, electric and thermal field imaging with high spatial and temporal resolution. Here we characterize the formation of…

Materials Science · Physics 2019-11-13 Tim R. Eichhorn , Claire A. McLellan , Ania C. B. Jayich
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