Related papers: Alignment dependent ultrafast electron-nuclear dyn…
When a chemical bond is broken, the molecular structure undergoes a transformation. An ideal experiment should probe the change in the electronic and nuclear structure simultaneously. Here, we present a method for the simultaneous…
We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…
We investigate high-harmonic generation in closed systems, using the two-level atom as a simplified model. By means of a windowed Fourier transform of the time-dependent dipole acceleration, we extract the main contributions to this process…
Highly nonlinear optical phenomena can provide access to properties of electronic systems which are otherwise difficult to access through conventional linear optical spectroscopies. In particular, high harmonic generation (HHG) in…
High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…
Two different induced effects of a laser falling edge on high-order harmonic generation are resolved by solving numerically full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the Born-Oppenheimer approximation. The…
High harmonic generation (HHG) is a nonlinear process that enables table-top generation of tunable, high-energy, coherent, ultrashort radiation pulses in the extreme ultraviolet (EUV) to soft X-ray range. These pulses find applications in…
Recent measurements on high-order harmonic generation (HHG) from N$_2$ aligned perpendicular to the driving laser polarization [B. K. McFarland {\it el al}, Science {\bf 322}, 1232 (2008)] have shown a maximum at the rotational…
We show that the Floquet approach with a Sturmian basis means an efficient description of high-order harmonic generation with monochromatic excitation. This method, although involves numerical calculations, is close to analytic approaches…
High-harmonic generation (HHG) is one of the fundamental processes at the heart of attosecond physics. Traditionally viewed as an effective single-particle effect, recent advances have focused on contributions beyond this single-particle…
High order harmonic (HOH) generation by interacting extremely intense electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. We consider here the process in the lowest order of a…
The generation of high-order harmonics in diatomic molecules is investigated within the framework of the strong-field approximation. We show that the conventional saddle-point approximation is not suitable for large internuclear distances.…
An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…
We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…
The sub-cycle dynamics of electrons driven by strong laser fields is central to the emerging field of attosecond science. We demonstrate how the dynamics can be probed through high-order harmonic generation, where different trajectories…
High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…
High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…
High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…
A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…
Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…