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Embedded density functional theory (e-DFT) is used to describe the electronic structure of strongly interacting molecular subsystems. We present a general implementation of the Exact Embedding (EE) method [J. Chem. Phys. 133, 084103 (2010)]…

Other Condensed Matter · Physics 2011-07-27 Jason D. Goodpaster , Taylor A. Barnes , Thomas F. Miller

We report a systematic and ab-initio electronic structure calculation of Ca0.75 M0.25 Fe2 As2 with M = Ca, Sr, Eu, La, Ce, Pr, Nd, Pm, Sm, Na, K, Rb. The recently reported experimentally observed structural trends in rare earths-doped CaFe2…

Superconductivity · Physics 2014-06-26 A. Sanna , G. Profeta , S. Massidda , E. K. U. Gross

The crystal structure of MoS$_2$ with strong covalent bonds in plane and weak Van der Waals interactions out of plane gives rise to interesting properties for applications such as solid lubrication, optoelectronics, and catalysis, which can…

Materials Science · Physics 2021-07-28 Rijan Karkee , Enrique Guerrero , David A. Strubbe

Density functional theory calculations are used to systematically investigate the structural and electronic properties of MX$_2$ transition metal dichalcogenide monolayers with M = Cr, Mo, W and X = S, Se, Te that are doped with single (V,…

Materials Science · Physics 2024-01-03 Yuqiang Gao , Paul J. Kelly

200 nm thick SiO2 layers grown on Si substrates and Ge ions of 150 keV energy were implanted into SiO2 matrix with Different fluences. The implanted samples were annealed at 950 C for 30 minutes in Ar ambience. Topographical studies of…

Materials Science · Physics 2017-05-31 R. P. Yadav , V. Baranwal , Sunil Kumar , Avinash C Pandey , A. K. Mittal

Reactive dopant atoms embedded in inert host metal surfaces define the active sites in single-atom alloys (SAAs), yet SAA synthesis remains challenging. To address this, we elucidate how dopant adatoms deposited on Cu and Ag surfaces become…

Materials Science · Physics 2025-12-01 Ioannis Karageorgiou , Angelos Michaelides , Fabian Berger

Control of dopants in silicon remains the most important approach to tailoring the properties of electronic materials for integrated circuits, with Group V impurities the most important n-type dopants. At the same time, silicon is finding…

In this work, the interaction of n-type dopants in Si doped (AlxGa1-x)2O3 films with varying Al content over the entire composition range (x = 0-100%) was analyzed using atom probe tomography. An almost uniform dopant distribution with…

Applied Physics · Physics 2020-09-04 Jith Sarker , A F M Anhar Uddin Bhuiyan , Zixuan Feng , Hongping Zhao , Baishakhi Mazumder

We report the electronic structure studies of well characterized polycrystalline Zn_{1-x}Fe_xO (x = 0.0, 0.01, 0.03, and 0.05) nanorods synthesized by a co-precipitation method through x-ray absorption fine structure (XAFS). X-ray…

Materials Science · Physics 2011-11-22 Sanjeev Gautam , S. Kumar , P. Thakur , K. H. Chae , Ravi Kumar , C. G. Lee

In-situ EXAFS experiments were performed at the Ag $K$-edge after adsorbing NO on the hydrogen reduced silver cluster. The coordination parameters, i.e. inter-atomic distance, coordination number and Debye-Waller factor were derived from a…

Materials Science · Physics 2015-10-12 Amgalanbaatar Baldansuren

Density functional theory (DFT) has become a standard tool for the study of point defects in materials. However, finding the most stable defective structures remains a very challenging task as it involves the solution of a multimodal…

Materials Science · Physics 2020-11-16 Marco Arrigoni , Georg K. H. Madsen

In the elastic scattering regime, probe position-averaged convergent beam electron diffraction (PACBED) patterns have proven robust for estimating specimen thickness and mistilt. Through simulation, we show that core-loss-filtered PACBED…

Other Condensed Matter · Physics 2025-10-27 Michael Deimetry , Timothy C. Petersen , Matthew Weyland , Scott D. Findlay

The combination of density functional theory (DFT) with a multiconfigurational wave function is an efficient way to include dynamical correlation in calculations with multiconfiguration self-consistent field wave functions. These methods…

Chemical Physics · Physics 2018-02-14 Geng Dong , Ulf Ryde , Hans Jørgen Aa. Jensen , Erik D. Hedegård

A thorough investigation of local structure, influencing macroscopic properties of the solid is of potential interest. We investigated the local structure of GaN nanowires (NWs) with different native defect concentration synthesized by the…

We investigate effects of doping on formation energy and concentration of oxygen vacancies at a metal oxide surface, using MgO (100) as an example. Our approach employs density-functional theory, where the performance of the…

Materials Science · Physics 2013-05-24 Norina A. Richter , Sabrina Sicolo , Sergey V. Levchenko , Joachim Sauer , Matthias Scheffler

We have investigated the influence of Ca ions substitution on the structural and superconducting properties of (Nd1-xCax)(Ba1.6La0.4)Cu3Oz system. Magnetization, X-ray diffraction and neutron diffraction studies have been carried out on a…

Superconductivity · Physics 2010-05-14 Amish G. Joshi , R. G. Kulkarni , W. B. Yelon , Ram Prasad , M. R. Gonal

The incorporation of phosphorus in silicon is studied by analyzing phosphorus delta-doped layers using a combination of scanning tunneling microscopy, secondary ion mass spectrometry and Hall effect measurements. The samples are prepared by…

Condensed Matter · Physics 2009-11-07 L. Oberbeck , N. J. Curson , M. Y. Simmons , R. Brenner , A. R. Hamilton , S. R. Schofield , R. G. Clark

Results of resonant inelastic X-ray scattering (RIXS) measurements at Fe L-edges and electronic structure calculations of LiFeAs and NaFeAs are presented. Both experiment and theory show that in the vicinity of the Fermi energy, the density…

We have investigated the electronic structure of Ba3InIr2O9 within the density-functional theory (DFT) using the generalized gradient approximation while considering strong Coulomb correlations (GGA+$U$) in the framework of the fully…

Strongly Correlated Electrons · Physics 2025-02-26 D. A. Kukusta , L. V. Bekenov , V. N. Antonov

We present a comprehensive computational framework for reproducing the full X-ray absorption fine structure (XAFS) through quantum-chemical simulations. The near-edge region is accurately captured using an efficient implementation of…

Materials Science · Physics 2025-12-04 Philipp Hönicke , Yves Kayser , Pouya Partovi-Azar