English
Related papers

Related papers: Electron Doping a Kagome Spin Liquid

200 papers

We report the thermodynamic and muon spin relaxation ($\mu$SR) evidences for a possible gapless spin liquid in Tm$_{3}$Sb$_{3}$Zn$_{2}$O$_{14}$, with the rare-earth ions Tm$^{3+}$ forming a two-dimensional kagom\'{e} lattice. We extract the…

Strongly Correlated Electrons · Physics 2018-11-09 Zhaofeng Ding , Yanxing Yang , Jian Zhang , Cheng Tan , Zihao Zhu , Gang Chen , Lei Shu

Frustrated magnetism on the kagome lattice has been a fertile ground for rich and fascinating physics, ranging from experimental evidence of a spin liquid to theoretical predictions of exotic superconductivity. Among experimentally realized…

Strongly Correlated Electrons · Physics 2015-12-16 Yasir Iqbal , Harald O. Jeschke , Johannes Reuther , Roser Valentí , I. I. Mazin , Martin Greiter , Ronny Thomale

A quantum spin liquid state has long been predicted to arise in spin-1/2 Heisenberg square-lattice antiferromagnets at the boundary region between N\'eel (nearest-neighbor interaction dominates) and columnar (next-nearest-neighbor…

We study the effects of doping a Mott insulator on the honeycomb lattice where spins interact via direction dependent Kitaev couplings J_K, and weak antiferromagnetic Heisenberg couplings J. This model is known to have a spin liquid ground…

Strongly Correlated Electrons · Physics 2012-08-30 Yi-Zhuang You , Itamar Kimchi , Ashvin Vishwanath

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

To capture the high-field magnetization process of herbertsmithite (ZnCu3(OH)6Cl2), Faraday rotation (FR) measurements were carried out on a single crystal in magnetic fields of up to 190 T. The magnetization data evaluated from the FR…

Strongly Correlated Electrons · Physics 2020-09-29 Ryutaro Okuma , Daisuke Nakamura , Shojiro Takeyama

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

Spin-1/2 kagome materials have recently attracted a resurgence of interest as they are considered an ideal host of the quantum spin liquid (QSL) state, which can underpin functionality such as superconductivity. Here we report the first…

Strongly Correlated Electrons · Physics 2023-06-27 M. Georgopoulou , D. Boldrin , B. Fåk , P. Manuel , A. Gibbs , J. Ollivier , E. Suard , A. S. Wills

We present a microscopic study of a doped quantum spin liquid candidate, the hyperkagome Na$_3$Ir$_3$O$_8$ compound by using $^{23}$Na NMR. We determine the intrinsic behavior of the uniform \textbf{q} $ = 0$ susceptibility via shift…

Strongly Correlated Electrons · Physics 2021-03-17 G. Simutis , T. Takayama , Q. Barthélemy , F. Bert , H. Takagi , P. Mendels

A series of compounds M$_{0.1}$Sr$_{0.9}$Cu$_2$(BO$_3$)$_2$ with Sr substituted by M=Al, La, Na and Y were prepared by solid state reaction. XRD analysis showed that these doping compounds are isostructural to SrCu$_2$(BO$_3$)$_2$. The…

Strongly Correlated Electrons · Physics 2009-11-10 G. T. Liu , J. L. Luo , T. Xiang , N. L. Wang , Z. H. Wu , X. N. Jing , D. Jin

To obtain high-performance spintronic devices with high integration density, two-dimensional (2D) half-metallic materials are eagerly pursued all along. Here, we propose a stable 2D material with a honeycomb-kagome lattice, i.e., the Mg3C2…

Materials Science · Physics 2018-07-04 Hongzhe Pan , Yin Han , Jianfu Li , Hongyu Zhang , Youwei Du , Nujiang Tang

Density functional calculations are used to investigate the doping dependence of the electronic structure and magnetic properties in hexagonal Na$_x$CoO$_2$. The electronic structure is found to be highly two dimensional, even without…

Superconductivity · Physics 2009-11-10 D. J. Singh

Quantum spin liquid is a nontrivial magnetic state of longstanding interest, in which spins are strongly correlated and entangled but do not order1, 2; further intriguing is its doped version, which possibly hosts strange metal and…

Strongly Correlated Electrons · Physics 2023-07-12 K. Wakamatsu , Y. Suzuki , T. Fujii , K. Miyagawa , H. Taniguchi , K. Kanoda

The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of…

Strongly Correlated Electrons · Physics 2011-03-16 Philippe Mendels , Fabrice Bert

Optical conductivity measurements are combined with density functional theory calculations in order to understand the electrodynamic response of the frustrated Mott insulators Herbertsmithite $\mathrm{ZnCu_{3}(OH)_{6}Cl_{2}}$ and the…

Strongly Correlated Electrons · Physics 2018-01-10 Andrej Pustogow , Ying Li , Ievgen Voloshenko , Pascal Puphal , Cornelius Krellner , Igor I. Mazin , Martin Dressel , Roser Valentí

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

Herbertsmithite (ZnCu3(OH)6Cl2) is often discussed as the best realization of the highly frustrated antiferromagnetic kagome lattice known so far. We employ density functional theory calculations to determine eight exchange coupling…

Strongly Correlated Electrons · Physics 2014-01-31 Harald O. Jeschke , Francesc Salvat-Pujol , Roser Valenti

The electron-doping-driven collapse of the charge gap and staggered magnetization of the spin-orbit-assisted Mott insulator Sr$_{3}$Ir$_{2}$O$_{7}$ is explored via first-principles computational methods. In the antiferromagnetic phase, the…

Strongly Correlated Electrons · Physics 2018-08-15 Michael W. Swift , Zach Porter , Stephen D. Wilson , Chris G. Van de Walle

The $S=1/2$ antiferromagnetic Heisenberg spin chain compound Sr$_2$CuO$_3$ doped with $1 \%$ and $2 \%$ of Ni impurities has been studied by means of $^{63}$Cu nuclear magnetic resonance. A strong decrease of the spin-lattice relaxation…