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We have extended our experimentally constrained molecular relaxation technique (P. Biswas {\it et al}, Phys. Rev. B {\bf 71} 54204 (2005)) to hydrogenated amorphous silicon: a 540-atom model with 7.4 % hydrogen and a 611-atom model with 22…

Materials Science · Physics 2009-11-13 Parthapratim Biswas , Raymond Atta-Fynn , David A. Drabold

Modern bandgap engineered electronic devices are typically made of multi-semiconductor multi-layer heterostructures that pose a major challenge to silicon-era characterization methods. As a result, contemporary bandgap engineering relies…

Applied Physics · Physics 2018-01-18 Yury Turkulets , Ilan Shalish

Halide perovskites have been extensively studied as materials of interest for optoelectronic applications. There is a major emphasis on ways to tailor the stability, defect behavior, electronic band structure, and optical absorption in…

Materials Science · Physics 2023-09-29 Jiaqi Yang , Arun Mannodi-Kanakkithodi

Halide perovskites consist a class of materials under intense investigation due to their potential technological applications like solar cells, optoelectronic devices and catalysis. Recently we have studied using electronic band structure…

Materials Science · Physics 2018-10-17 G. Moschou , A. Koliogiorgos , I. Galanakis

Complementary angle-resolved photoemission and bulk-sensitive k-resolved resonant inelastic x-ray scattering of divalent hexaborides reveal a >1 eV X-point gap between the valence and conduction bands, in contradiction to the band overlap…

Strongly Correlated Electrons · Physics 2009-11-07 J. D. Denlinger , J. A. Clack , J. W. Allen , G. -H. Gweon , D. M. Poirier , C. G. Olson , J. L. Sarrao , A. D. Bianchi , Z. Fisk

Organic dopants are frequently used to surface-dope inorganic semiconductors. The resulted hybrid inorganic-organic materials have a crucial role in advanced functional materials and semiconductor devices. In this article, we study charge…

Materials Science · Physics 2017-08-01 Xiaoming Wang , Keivan Esfarjani , Mona Zebarjadi

First principle band calculations based on local versions of density functional theory (DFT), together with results from nearly free-electron models, can describe many typical but unusual properties of the high-$T_C$ copper oxides. The…

Superconductivity · Physics 2009-08-20 T. Jarlborg

We study the electronic structures and dielectric functions of the simple hydrides LiH, NaH, MgH2 and AlH3, and the complex hydrides Li3AlH6, Na3AlH6, LiAlH4, NaAlH4 and Mg(AlH4)2, using first principles density functional theory and GW…

Materials Science · Physics 2007-05-23 M. J. van Setten , V. A. Popa , G. A. de Wijs , G. Brocks

In this second paper, we develop transferable semi-empirical parameters for the technologically important material, silicon, using Extended Huckel Theory (EHT) to calculate its electronic structure. The EHT-parameters areoptimized to…

Materials Science · Physics 2009-11-11 Diego Kienle , Jorge I. Cerda , Kirk H. Bevan , Gengchiau Liang , Lutfe Siddiqui , Avik W. Ghosh

We present a tight-binding (TB) model and $\mathbf{k\cdot p}$ theory for electrons in monolayer and few-layer InSe. The model is constructed from a basis of all $s$ and $p$ valence orbitals on both indium and selenium atoms, with…

Mesoscale and Nanoscale Physics · Physics 2017-01-05 S. J. Magorrian , V. Zólyomi , V. I. Fal'ko

The electronic structure, chemical bonding and interface component in ZrN-AlN nanocomposites formed by phase separation during thin film deposition of metastable Zr1-xAlxN (x=0.0, 0.12, 0.26, 0.40) is investigated by resonant inelastic…

Materials Science · Physics 2020-03-19 Martin Magnuson , Weine Olovsson , Naureen Ghafoor , Magnus Odén , Lars Hultman

The need for semiconductor technology for crystalline silicon of the highest purity and homogeneity has provided samples exhibiting low optical absorption in the infrared range. Such silicon has become the basis for photonic elements in the…

We compute the electronic band structure and optical properties of boron arsenide using the relativistic quasiparticle self-consistent $GW$ approach, including electron-hole interactions through solution of the Bethe-Salpeter equation. We…

Materials Science · Physics 2019-06-07 John Buckeridge , David O. Scanlon

The bandgap and band bowing parameter of semiconductor alloys are calculated with a fast and realistic approach. The method is a dielectric scaling approximation that is based on a scissor approximation. It adds an energy shift to the…

Materials Science · Physics 2010-04-08 Titus Sandu , Radu I. Iftimie

Silicon materials play a key role in many technologically relevant fields, ranging from the electronic to the photovoltaic industry. A systematic search for silicon allotropes was performed by employing a modified ab initio minima hopping…

Heat transfer at the interface between two materials is becoming increasingly important as the size of electronic devices shrinks. Most studies concentrate on the interfacial thermal conductance between either crystalline-crystalline or…

Mesoscale and Nanoscale Physics · Physics 2024-09-09 Julien El Hajj , Christophe Adessi , Michaël de San Feliciano , Gilles Ledoux , Samy Merabia

Ab initio electronic structure studies of prototypical polar interfaces of wurtzite III-V nitrides show that large uniform electric fields exist in epitaxial nitride overlayers, due to the discontinuity across the interface of the…

Materials Science · Physics 2009-10-30 Fabio Bernardini , Vincenzo Fiorentini

We have used tight-binding molecular-dynamics simulations to investigate the role of point defects (vacancies and interstitials) on structural relaxation in amorphous silicon. Our calculations give unambiguous evidence that point defects…

Materials Science · Physics 2007-05-23 Cristiano L. Dias , Laurent J. Lewis , S. Roorda

For a wide class of technologically relevant compound III-V and II-VI semiconductor materials AC and BC mixed crystals (alloys) of the type A(x)B(1-x)C can be realized. As the electronic properties like the bulk band gap vary continuously…

Materials Science · Physics 2015-06-03 Daniel Mourad , Gerd Czycholl

Exciton dissociation at heterojunctions in photovoltaic devices is not completely understood despite being fundamentally necessary to generate electrical current. One of the fundamental issues for ab initio calculations is that hybrid…

Mesoscale and Nanoscale Physics · Physics 2017-06-20 Michael J. Waters , Daniel Hashemi , John Kieffer