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Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 S. Alex Breitweiser , Mathieu Ouellet , Tzu-Yung Huang , Tim H. Taminiau , Lee C. Bassett

Precise timekeeping is critical to metrology, forming the basis by which standards of time, length and fundamental constants are determined. Stable clocks are particularly valuable in spectroscopy as they define the ultimate frequency…

This article reviews efforts to build a new type of quantum device, which combines an ensemble of electronic spins with long coherence times, and a small-scale superconducting quantum processor. The goal is to store over long times…

We present a novel spectroscopy protocol based on optimal control of a single quantum system. It enables measurements with quantum-limited sensitivity (\eta_\omega ~ 1/sqrt(T_2^*),T_2^* denoting the system's coherence time) but has an…

Sensing, localising and identifying individual nuclear spins or frequency components of a signal in the presence of a noisy environments requires the development of robust and selective methods of dynamical decoupling. An important…

We present a framework that formulates the quest for the most efficient quantum state tomography scheme as an optimization problem which can be solved numerically. This approach can be applied to a broad spectrum of relevant setups…

Quantum Physics · Physics 2021-12-17 Violeta N. Ivanova-Rohling , Guido Burkard , Niklas Rohling

Electron and nuclear spins of diamond nitrogen-vacancy (NV) centers are good candidates for quantum information processing as they have long coherence time and can be initialized and read out optically. However, creating a large number of…

Quantum Physics · Physics 2019-11-19 Zhujing Xu , Zhang-qi Yin , Qinkai Han , Tongcang Li

Solid-state quantum sensors based on ensembles of nitrogen-vacancy (NV) centers in diamond have emerged as powerful tools for precise sensing applications. Nuclear spin sensors are particularly well-suited for applications requiring long…

Quantum Physics · Physics 2025-05-14 Hanfeng Wang , Shuang Wu , Kurt Jacobs , Yuqin Duan , Dirk R. Englund , Matthew E. Trusheim

The realization of effective quantum error correction protocols remains a central challenge in the development of scalable quantum computers. Employing high-dimensional quantum systems (qudits) can offer more hardware-efficient protocols…

Quantum Physics · Physics 2025-03-18 Sumin Lim , Mikhail V. Vaganov , Junjie Liu , Arzhang Ardavan

Nitrogen-vacancy (NV) centers in diamond can be used as quantum sensors to image the magnetic field with nanoscale resolution. However, nanoscale electric-field mapping has not been achieved so far because of the relatively weak coupling…

Mesoscale and Nanoscale Physics · Physics 2021-05-04 Ke Bian , Wentian Zheng , Xianzhe Zeng , Xiakun Chen , Rainer Stohr , Andrej Denisenko , Sen Yang , Joerg Wrachtrup , Ying Jiang

We theoretically analyze the performance of the nuclear magnetic resonance (NMR) spectroscopy with a superconducting flux qubit (FQ). Such NMR with the FQ is attractive because of the possibility to detect the relatively small number of…

We demonstrate the simultaneous estimation of signal frequency and amplitude by a single quantum sensor in a single experimental shot. Sweeping the qubit splitting linearly across a span of frequencies induces a non-adiabatic Landau-Zener…

Sensors based on spin qubits in 2D crystals offer the prospect of nanoscale sensing volumes, where the close proximity of the sensor and source could provide access to otherwise inaccessible signals. For AC magnetometry, the sensitivity and…

Materials Science · Physics 2024-03-14 Charlie J. Patrickson , Simon Baber , Blanka B. Gaál , Andrew J. Ramsay , Isaac J. Luxmoore

Quantum probes can measure time-varying fields with high sensitivity and spatial resolution, enabling the study of biological, material, and physical phenomena at the nanometer scale. In particular, nitrogen-vacancy centers in diamond have…

Quantum Physics · Physics 2014-02-05 Alexandre Cooper , Easwar Magesan , Honam Yum , Paola Cappellaro

Quantum sensors can show unprecedented sensitivities, provided they are controlled in a very specific, optimal way. Here, we consider a spin sensor of time-varying fields in the presence of dephasing noise, and we show that the problem of…

Quantum Physics · Physics 2024-07-10 S. Hernández-Gómez , F. Balducci , G. Fasiolo , P. Cappellaro , N. Fabbri , A. Scardicchio

Quantum state tomography (QST) is the procedure for reconstructing unknown quantum states from a series of measurements of different observables. Depending on the physical system, different sets of observables have been used for this…

Quantum Physics · Physics 2023-03-02 Jingfu Zhang , Swathi S. Hegde , Dieter Suter

We describe a quantum memory spectral preparation strategy that maximises memory efficiency and bandwidth in materials such as 167 Er3+:Y2SiO5 in a high field regime, where the hyperfine structure is resolved. We demonstrate the method in…

Quantum Physics · Physics 2021-09-01 James Stuart , Morgan Hedges , Rose Ahlefeldt , Matthew Sellars

Knowing a quantum system's environment is critical for its practical use as a quantum device. Qubit sensors can reconstruct the noise spectral density of a classical bath, provided long enough coherence time. Here we present a protocol that…

Quantum Physics · Physics 2018-12-20 Santiago Hernández-Gómez , Francesco Poggiali , Paola Cappellaro , Nicole Fabbri

We demonstrate a method of magnetic resonance imaging with single nuclear-spin sensitivity under ambient conditions. It employs a network of isolated electronic-spin quantum bits (qubits) that act as quantum reporters on the surface of high…

The excellent sensitivities of quantum sensors are a double-edged sword: minuscule quantities can be observed, but any undesired signal acts as noise. This is challenging when detecting quantities that are obscured by such noise. Decoupling…

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