Related papers: Attosecond Control of Relativistic Electron Bunche…
When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…
A theoretical investigation on the quantum control of optical coherent four-wave mixing interactions in two-level systems driven by two intense synchronized femtosecond laser pulses of central angular frequencies $\omega$ and $3\omega$ is…
Ultrashort light pulses can selectively excite charges, spins and phonons in materials, providing a powerful approach for manipulating their properties. Here we use femtosecond laser pulses to coherently manipulate the electron and phonon…
The field of laser-matter interaction traditionally deals with the response of atoms, molecules and plasmas to an external light wave. However, the recent sustained technological progress is opening up the possibility of employing intense…
Extreme intensity contrast is considered essential for ultraintense, femtosecond laser excitation of solid targets, in particular for studies with structured or ultra-thin targets. Second-harmonic generation has been used to maximize the…
The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…
Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…
Generation of attosecond bunches of energetic electrons offers significant potential from ultrafast physics to novel radiation sources. However, it is still a great challenge to stably produce such electron beams with lasers, since the…
Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…
The hot and dense QCD matter produced in nuclear collisions at ultrarelativistic energy is characterized by very intense electromagnetic fields which attain their maximal strength in the early pre-equilibrium stage and interplay with the…
Attosecond spectroscopy of materials has provided invaluable insight into light-driven coherent electron dynamics. However, attosecond spectroscopies have so far been focused on weakly-correlated materials. As a result, the behavior of…
Tracing ultrafast processes induced by interaction of light with matter is often very challenging. In molecular systems, the initially created electronic coherence becomes damped by the slow nuclear rearrangement on a femtosecond timescale…
We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…
Precise control of the electron phase accumulated during its sub-cycle motion within intense laser fields is essential in strong-field physics, yet remains mostly indirect and complicated so far. In this Letter, we develop a novel approach…
The coupling of electronic and nuclear motion in polyatomic molecules is at the heart of attochemistry. The molecular properties, transient structures and reaction mechanism of these many-body quantum objects are defined on the level of…
We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…
Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…
Ultracold temperatures in dilute quantum gases opened the way to an exquisite control of matter at the quantum level. Here we focus on the control of ultracold atomic collisions using a laser to engineer their interactions at large…
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…