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High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

High harmonic generation in benzene is studied using a mixed quantum-classical approach in which the electrons are described using time-dependent density functional theory while the ions move classically. The interaction with both…

Atomic Physics · Physics 2016-03-02 Abigail Wardlow , Daniel Dundas

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

Chiral discrimination with high harmonic generation (cHHG method) has been introduced in the recent work by R. Cireasa et al ( Nat. Phys. 11, 654 - 658, 2015). In its original implementation, the cHHG method works by detecting high harmonic…

Optics · Physics 2015-10-28 Olga Smirnova , Yann Mairesse , Serguei Patchkovskii

Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

We present an alternative theoretical model for a recent experiment [A.Fleischer et al., Nature Photon. 8, 543 (2014)] which used bichromatic, counter-rotating high intensity laser pulses to probe the conservation of spin angular momentum…

Atomic Physics · Physics 2014-12-11 Emilio Pisanty , Misha Ivanov , Suren Sukiasyan

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…

Optics · Physics 2022-01-25 Yigeng Peng , Tong Wu , Guanglu Yuan , Lihan Chi , Chao Yu , Ruifeng Lu

A recent paper reported elliptically polarized high-order harmonics from aligned N$_2$ using a linearly polarized driving field [X. Zhou \emph{et al.}, Phys. Rev. Lett. \textbf{102}, 073902 (2009)]. This observation cannot be explained in…

Atomic Physics · Physics 2010-03-29 Adam Etches , Christian Bruun Madsen , Lars Bojer Madsen

The generation of high-order harmonics in a medium of chiral molecules driven by intense bi-elliptical laser fields can lead to strong chiroptical response in a broad range of harmonic numbers and ellipticities [D. Ayuso et al, J. Phys. B…

Optics · Physics 2018-07-04 David Ayuso , Piero Decleva , Serguei Patchkovskii , Olga Smirnova

High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

Atomic and Molecular Clusters · Physics 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…

Atomic Physics · Physics 2019-10-23 Sebastian Gemsheim , Jan-Michael Rost

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

Materials Science · Physics 2020-12-23 G. P. Zhang , Y. H. Bai

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

Atomic Physics · Physics 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

We demonstrate arbitrary helicity control of circularly polarized light (CPL) emitted at room temperature from the cleaved side-facet of a lateral-type spin-polarized light-emitting diode (spin-LED) with two ferromagnetic electrodes in an…

Dynamic stabilization of atomic hydrogen against ionization in high-frequency single- and two-color, circularly polarized laser pulses is observed by numerically solving the three-dimensional, time-dependent Schr\"odinger equation. The…

Atomic Physics · Physics 2009-11-07 D. Bauer , F. Ceccherini

Production of electron-positron pairs by a high-energy $\gamma$ photon and a bichromatic laser wave is considered where the latter is composed of a strong low-frequency and a weak high-frequency component, both with circular polarization.…

High Energy Physics - Phenomenology · Physics 2023-06-06 N. Mahlin , S. Villalba-Chávez , C. Müller

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We demonstrated nonperturbative high harmonics induced by intense mid-infrared light up to 18th order that well exceed the material bandgap in monolayer transition metal dichalcogenides. The intensities of the even-order high-harmonic…

Mesoscale and Nanoscale Physics · Physics 2019-08-20 Naotaka Yoshikawa , Kohei Nagai , Kento Uchida , Yuhei Takaguchi , Shogo Sasaki , Yasumitsu Miyata , Koichiro Tanaka

The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti