Related papers: Probing and controlling terahertz-driven structura…
The ability to manipulate the space-time structure of light waves diversifies light-matter interaction and light-driven applications. Conventionally, metasurfaces are employed to locally control the amplitude and phase of light fields by…
The resonant modes of optical cavities provide a powerful resource for laser-frequency stabilization, underpinning high-precision metrology and coherent signal generation. Photonic resonators in which the optical mode propagates through…
Monolayer transition-metal dichalcogenides (TMDCs) present high second-order optical nonlinearity, which is extremely desirable for, e.g., frequency conversion in nonlinear photonic devices. On the other hand, the atomic thickness of 2D…
Truly chiral phonons are lattice eigenmodes that combine broken mirror symmetry with circular atomic motion. They can mediate angular-momentum-selective interactions in quantum materials, yet directly resolving both their chirality and…
Tailored light excitation and nonlinear control of lattice vibrations have emerged as powerful strategies to manipulate the properties of quantum materials out of equilibrium. Generalizing the use of coherent phonon-phonon interactions to…
Topological materials provide an exclusive platform to study the dynamics of relativistic particles in table-top experiments and offer the possibility of wide-scale technological applications. ZrSiS is a newly discovered topological…
Extending the high-harmonic cutoff with experimentally accessible fields is essential for advancing tabletop coherent extreme ultraviolet (EUV) and soft X-ray sources. Although terahertz (THz) assistance offers a promising route, cutoff…
We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…
Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…
We investigate the ultrafast optical response of PbTe to an intense single-cycle terahertz pulse, resonant with the soft transverse optical (TO) phonon mode of the crystal. We detect multifrequency oscillations of the reflectance…
Two-dimensional transition metal dichalcogenides (TMDC) have shown promise for various applications in optoelectronics and so-called valleytronics. Their operation and performance strongly depend on the stacking of individual layers. Here,…
We present a single-shot detection method of terahertz-correlated second harmonic generation in plasma-based sources by directly mixing an optical probe into femtosecond laser-induced plasma filaments in air. The single-shot second harmonic…
We present an analytical theory of second harmonic generation (SHG) in hybrid structures combining a nonlinear 2D crystal with a dielectric metasurface waveguide. The theory describes the excitation spectrum and enhancement of SHG at both…
Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…
Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…
Optical-field sampling using second-harmonic generation (SHG) from strong-field ionization enables ultrabroadband terahertz detection, but the microscopic origin of the SHG signal and its ultrabroadband response have been unclear. Here we…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
Ultrafast charge transport in strongly biased semiconductors is at the heart of highspeed electronics, electro-optics, and fundamental solid-state physics. Intense light pulses in the terahertz (THz) spectral range have opened fascinating…
Driving coherent lattice motion with THz pulses has emerged as a novel pathway for achieving dynamic stabilization of exotic phases that are inaccessible in equilibrium quantum materials. In this work, we present a previously unexplored…
Understanding surface collective dynamics in quantum materials is crucial for advancing quantum technologies. For example, surface phonon modes in quantum paraelectrics are thought to play an essential role in facilitating interfacial…