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Thermal transport properties of amorphous carbon has attracted increasing attention due to its extreme thermal properties: It has been reported to have among the highest thermal conductivity for bulk amorphous solids up to $\sim$ 37…

Disordered Systems and Neural Networks · Physics 2024-05-14 Jaeyun Moon , Zhiting Tian

Glasses usually represent the lower limit for the thermal conductivity of solids, but a fundamental understanding of lattice heat transport in amorphous materials can provide design rules to beat such a limit. Here we investigate the role…

Materials Science · Physics 2021-01-27 Nicholas W. Lundgren , Giuseppe Barbalinardo , Davide Donadio

Hydrogenated amorphous silicon (a-Si:H) has garnered considerable attention in the semiconductor industry, particularly for its use in solar cells and passivation layers for high performance silicon solar cells, owing to its exceptional…

Materials Science · Physics 2025-02-14 Zhuo Chen , Yuejin Yuan , Yanzhou Wang , Penghua Ying , Shouhang Li , Cheng Shao , Wenyang Ding , Gang Zhang , Meng An

Normal mode decomposition of atomic vibrations has been used to provide microscopic under-standing of thermal transport in amorphous solids for decades. In normal mode methods, it is naturally assumed that atoms vibrate around their…

Materials Science · Physics 2021-08-25 Jaeyun Moon

The thermal properties of amorphous materials have attracted significant attention due to their technological importance in electronic devices. Additionally, the disorder-induced breakdown of the phonon gas model makes vibrational transport…

Applied Physics · Physics 2024-06-12 Wanyue Peng , Richard Wilson

Amorphous Si (a-Si) nanostructures are ubiquitous in numerous electronic and optoelectronic devices. Amorphous materials are considered to possess the lower limit to the thermal conductivity (k), which is ~1 W/m-K for a-Si. However, recent…

Materials Science · Physics 2017-01-03 Soonshin Kwon , Jianlin Zheng , Matthew C. Wingert , Shuang Cui , Renkun Chen

Porous materials provide a large surface to volume ratio, thereby providing a knob to alter fundamental properties in unprecedented ways. In thermal transport, porous nanomaterials can reduce thermal conductivity by not only enhancing…

Amorphous materials are also distinguished from crystals by their thermal properties. The structural disorder seems to be responsible both for a significant increase in heat capacity compared to crystals of the same composition, but also…

Disordered Systems and Neural Networks · Physics 2023-07-28 Anne Tanguy

Amorphous alumina is employed ubiquitously as a high-dielectric-constant material in electronics, and its thermal-transport properties are of key relevance for heat management in electronic chips and devices. Experiments show that the…

Materials Science · Physics 2023-12-27 Angela F. Harper , Kamil Iwanowski , William C. Witt , Mike C. Payne , Michele Simoncelli

We describe epitaxial Ge/Si multilayers with cross-plane thermal conductivities which can be systematically reduced to exceptionally low values, as compared both with bulk and thin-film SiGe alloys of the same average concentration, by…

Materials Science · Physics 2013-01-04 Peixuan Chen , N. A. Katcho , J. P. Feser , Wu Li , M. Glaser , O. G. Schmidt , David G. Cahill , N. Mingo , A. Rastelli

Which sizes of nanoparticles embedded in a crystalline solid yield the lowest thermal conductivity? Nanoparticles have long been demonstrated to reduce the thermal conductivity of crystals by scattering phonons, but most previous works…

Materials Science · Physics 2015-02-17 Hang Zhang , Austin J. Minnich

The reduction of the thermal conductivity in nanostructures opens up the possibility of exploiting for thermoelectric purposes also materials such as silicon, which are cheap, available and sustainable but with a high thermal conductivity…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 G. Pennelli , E. Dimaggio , M. Macucci

Thermal transport properties of amorphous materials at low temperatures are governed by the interaction between phonons and localized excitations referred to as tunneling two level systems (TLS). The temperature variation of the thermal…

Mesoscale and Nanoscale Physics · Physics 2017-04-26 Adib Tavakoli , Christophe Blanc , Hossein Ftouni , Kunal Lulla , Andrew Fefferman , Eddy Collin , Olivier Bourgeois

Anomalous heat transport in one-dimensional nanostructures, such as nanotubes and nanowires, is a widely debated problem in condensed matter and statistical physics, with contradicting pieces of evidence from experiments and simulations.…

Mesoscale and Nanoscale Physics · Physics 2021-07-14 Giuseppe Barbalinardo , Zekun Chen , Haikuan Dong , Zheyong Fan , Davide Donadio

We have shown theoretically that a combination of cross-section modulation and acoustic mismatch in the core-shell Si/Ge nanowires can lead to a drastic reduction of the thermal conductivity. Our calculations, which utilized two different…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Denis L. Nika , Alexandr I. Cocemasov , Dmitrii V. Crismari , Alexander A. Balandin

Several hitherto unexplained features of thermal conductivity in group IV materials, such as the change in the slope as a function of sample size for pure vs. alloyed samples and the fast decay in thermal conductivity for low impurity…

Materials Science · Physics 2015-09-04 P. Torres , C. de Tomas , A. Lopeandia , X. Cartoixà , X. Alvarez

The value measured in the amorphous structure with the same chemical composition is often considered as a lower bound for the thermal conductivity of any material: the heat carriers are strongly scattered by disorder, and their lifetimes…

Materials Science · Physics 2015-09-17 Hideyuki Mizuno , Stefano Mossa , Jean-Louis Barrat

This paper focuses on the structural, electronic, and vibrational features of amorphous graphite [R. Thapa $\textit{et. al.}$, Phys. Rev. Lett. 128, 236402 (2022)]. The structure order in amorphous graphite is discussed and compared with…

Materials Science · Physics 2023-05-09 C. Ugwumadu , K. Nepal , R. Thapa , D. A. Drabold

Thermal conductivities $\Lambda $ of amorphous carbon thin films are measured in the temperatures range 80--400 K using the $3\omega $ method. Sample films range from soft a-C:H prepared by remote-plasma deposition ($\Lambda = 0.20$ W…

Materials Science · Physics 2009-10-31 Andrew J. Bullen , Keith E. O'Hara , David G. Cahill , Othon Monteiro , Achim von Keudell

Polymers are usually considered as thermal insulators and their applications are limited by their low thermal conductivity. However, recent studies showed that certain polymers have surprisingly high thermal conductivity, some of which are…

Mesoscale and Nanoscale Physics · Physics 2018-05-17 Xiangfan Xu , Jie Chen , Jun Zhou , Baowen Li
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