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High harmonic generation in polarizable multi-electron systems is investigated in the framework of multi-configuration time-dependent Hartree-Fock. The harmonic spectra exhibit two cut offs. The first cut off is in agreement with the well…

Quantum Physics · Physics 2009-11-11 J. Zanghellini , Ch. Jungreuthmayer , T. Brabec

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We theoretically investigate mechanisms of higher-order harmonic generation in solid-state materials under a high-intensity ac electric field. A new theoretical framework presented in this Letter holds the legitimacy of Bloch theorem even…

Materials Science · Physics 2017-01-12 T. Tamaya , A. Ishikawa , T. Ogawa , K. Tanaka

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

Optics · Physics 2023-05-03 Lun Yue , Mette B. Gaarde

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

The strong-field approximation for high-harmonic generation in near-infrared and infrared laser pulses is formulated in the accelerated Kramers-Henneberger frame. The accompanying physical picture is discussed and the nature of the…

Quantum Physics · Physics 2021-10-04 Lars Bojer Madsen

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

Plasma Physics · Physics 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

We present theoretical results on the high-harmonic generation (HHG) in bulk diamond induced by intense laser pulse of wavelength 800 nm and duration 15 fs. For laser intensity in the range $1 \le I \le 50 $ TW/cm$^2$ above bandgap…

Atomic Physics · Physics 2018-02-23 Tzveta Apostolova , Boyan Obreshkov

We study the crystal-momentum-resolved contributions to the high-order harmonic generation (HHG) in band-gap materials, and identify the relevant initial crystal momenta for the first and higher plateaus of the HHG spectra. We do so by…

Atomic Physics · Physics 2020-09-09 Chuan Yu , Hossein Iravani , Lars Bojer Madsen

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

In the present paper, we investigate the high-order harmonic generation (HHG) from diatomic molecules with large internuclear distance using a strong field approximation (SFA) model. We find that the hump and dip structure emerges in the…

Atomic Physics · Physics 2009-11-13 Y. J. Chen , J. Liu

Kerr-type nonlinearities form the basis for our physical understanding of nonlinear optical phenomena in condensed matter, such as self-focusing, solitary waves, and wave mixing. In strong fields, they are complemented by higher-order…

The development of sources delivering non-classical states of light is one of the main needs for applications of optical quantum information science. Here, we demonstrate the generation of non-classical states of light using strong-laser…

We present an analytic, and fully quantum theory of high harmonic generation by low frequency laser fields for a two-state hydrogenlike atom model. The model is valid for an arbitrary atomic potential role of dipole matrix elements and can…

Optics · Physics 2011-04-19 S Batebi , M Mohebbi

Interaction of intense laser beam with an inversion symmetric third order nonlinear medium is modeled as a quartic anharmonic oscillator. A first order operator solution of the model Hamiltonian is used to study the possibilities of…

Quantum Physics · Physics 2022-06-10 Anirban Pathak

The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is,…

Quantum Physics · Physics 2026-02-19 Christian Saugbjerg Lange , Lars Bojer Madsen

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…

Atomic Physics · Physics 2018-07-04 Nehzat Safaei

Squeezing of optical fields, used as a powerful resource for many applications, and the radiation properties in the process of high harmonic generation have thus far been considered separately. In this Letter, we want to clarify that the…