Related papers: Deceleration of a supersonic beam of SrF molecules…
We demonstrate that a bichromatic standing-wave laser field can exert a significantly larger force on a molecule than ordinary radiation pressure. Our experiment measures the deflection of a pulsed supersonic beam of CaF molecules by a…
A continuous guided atomic beam of $^{88}\mathrm{Sr}$ with a phase-space density exceeding $10^{-4}$ in the moving frame and a flux of $3 \times 10^{7} \, \mathrm{at \, s^{-1}}$ is demonstrated. This phase-space density is around three…
We present the design, construction, and characterisation of longitudinal- and transverse-field Zeeman slowers, based on arrays of permanent magnets, for slowing thermal beams of atomic Sr. The slowers are optimised for operation with…
A novel traveling-wave Zeeman decelerator based on a double-helix coil geometry capable of decelerating paramagnetic molecules with high efficiency is presented. Moving magnetic traps are generated by applying time-dependent currents…
Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…
We demonstrate laser slowing of a hot thulium atomic beam using the nearly closed cycling transition…
Slow beams of neutral molecules are of great interest for a wide range of applications, from cold chemistry through precision measurements to tests of the foundations of quantum mechanics. We report on the quantitative observation of…
We demonstrate a scheme for optical cycling in the polar, diatomic molecule strontium monofluoride (SrF) using the $X ^2\Sigma^+\toA^2\Pi_{1/2}$ electronic transition. SrF's highly diagonal Franck-Condon factors suppress vibrational…
Radio frequency particle accelerators are ubiquitous in ultra-small and ultrafast science, but their size and cost has prompted exploration of compact and scalable alternatives like the dielectric laser accelerator. We present the first…
We propose a scheme for direct laser deceleration of molecules based on a vibrational transition-mediated bichromatic force (VBCF). By precisely engineering mid-infrared optical fields, we establish coherent absorption-stimulated emission…
Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…
We examine two approaches for significantly extending the velocity range of the optical bichromatic force (BCF), to make it useful for laser deceleration of atomic and molecular beams. First, we present experimental results and calculations…
Beams of helium atoms in Rydberg-Stark states with principal quantum number $n=48$ and electric dipole moments of 4600~D have been decelerated from a mean initial longitudinal speed of 2000~m/s to zero velocity in the laboratory-fixed…
Fermilab is developing a compact superconducting CSRF accelerator as a source of a high-power, high-energy electron beam to produce an x-ray beam comparable to $\geq$ 2 MCi of cobalt-60. As part of this development, we are presently…
We have focused and decelerated benzonitrile (C$_7$H$_5$N) molecules from a molecular beam, using an array of time-varying inhomogeneous electric fields in alternating gradient configuration. Benzonitrile is prototypical for large…
We demonstrate buffer-gas cooling, high-resolution spectroscopy and cycling fluorescence of cold barium monofluoride (BaF) molecules. Our source produces an intense and internally cold molecular beam containing the different BaF…
Multistage Zeeman deceleration is a technique used to reduce the velocity of neutral molecules with a magnetic dipole moment. Here we present a Zeeman decelerator that consists of 100 solenoids and 100 magnetic hexapoles, that is based on a…
Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…
Stark deceleration is a technique that uses time-varying inhomogeneous electric fields to decelerate polar molecules for various molecular beam and trapping experiments. New ring-geometry Stark decelerators with continuously varying…
The maximum energy of electrons accelerated by supernova remnants (SNR) is typically limited by radiative losses. In this scenario, the synchrotron cooling time scale is equal to the acceleration time scale. On the other hand, the low…