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If one-electron observables of a many-electron system are of interest, a many-electron dynamics can be represented exactly by a one-electron dynamics with effective potentials. The formalism for this reduction is provided by the Exact…

Chemical Physics · Physics 2021-01-04 Jakub Kocák , Axel Schild

We propose a method using reduced size of Hilbert space to describe an electron dynamics in molecule and aggregate based on our previous theoretical scheme [ T. Yonehara and T. Nakajima, J. Chem. Phys. \textbf{147}, 074110 (2017) ]. The…

Chemical Physics · Physics 2019-09-09 Takehiro Yonehara , Takahito Nakajima

We first apply functional-integral approach to a multiband Hubbard model near the critical pairing temperature, and derive a generic effective action that is quartic in the fluctuations of the pairing order parameter. Then we consider…

Superconductivity · Physics 2023-06-13 M. Iskin

A stochastic approach to time-dependent density functional theory (TDDFT) is developed for computing the absorption cross section and the random phase approximation (RPA) correlation energy. The core idea of the approach involves…

Chemical Physics · Physics 2016-11-04 Yi Gao , Daniel Neuhauser , Roi Baer , Eran Rabani

Solving the time-dependent Schr\"odinger equation (TDSE) is pivotal for modeling non-adiabatic electron dynamics, a key process in ultrafast spectroscopy and laser-matter interactions. However, exact solutions to the TDSE remain…

Chemical Physics · Physics 2025-12-29 Bizi Huang , Weizhong Fu , Ji Chen

The polarization density of a broadband electrodynamic lattice-Boltzmann method (ELBM) is generalized to represent frequency-dispersion of materials interacting with electromagnetic waves. The frequency-dependent refractive index and…

Systems and Control · Electrical Eng. & Systems 2022-10-03 Cael Warner , Loïc Markley , Kenneth J. Chau

A simple approximate solution to the linear response equations of time-dependent density functional theory (TDDFT) is given. This extends the single-pole approximation (SPA) to two strongly-coupled poles. The analysis provides both an…

Materials Science · Physics 2009-11-11 H. Appel , E. K. U. Gross , K. Burke

The Quantum-Electrodynamical Time-Dependent Density Functional Theory (QED-TDDFT) equations are solved by time propagating the wave function on a tensor product of a Fock-space and real-space grid. Applications for molecules in cavities…

Quantum Physics · Physics 2022-11-30 Justin Malave , Alexander Ahrens , Daniel Pitagora , Cody Covington , Kálmán Varga

We report on an element- and time-resolved investigation of femtosecond laser induced ultrafast dynamics of 3d and 4f spins in a ferrimagnetic Co80Dy20 alloy as a function of temperature. We observe an increase of the Co3d characteristic…

Polarization in ferroelectrics, described by the Landau-Ginzburg Hamiltonian, is considered, based on a multi-dimensional Fokker-Planck equation. This formulation describes the time evolution of the probability distribution function over…

Statistical Mechanics · Physics 2015-06-24 J. Kaupuzs , J. Rimshans , N. F. Smyth

Within the finite-field Kohn-Sham framework, static electric response properties of diatomic molecules are presented. The electronic energy, dipole moment ({\boldmath$\mu$}), static dipole polarizability ({\boldmath$\alpha$}) and…

Chemical Physics · Physics 2019-04-26 Abhisek Ghosal , Tanmay Mandal , Amlan K. ~Roy

We propose a discrete functional analysis result suitable for proving compactness in the framework of fully discrete approximations of strongly degenerate parabolic problems. It is based on the original exploitation of a result related to…

Numerical Analysis · Mathematics 2015-04-16 Boris Andreianov , Clément Cancès , Ayman Moussa

An explicit expression for the quadratic density-response function of a many-electron system is obtained in the framework of the time-dependent density-functional theory, in terms of the linear and quadratic density-response functions of…

Materials Science · Physics 2009-11-10 V. U. Nazarov , J. M. Pitarke , C. S. Kim , Y. Takada

An ultrafast anisotropic electro-optic effect of the zinc sulfide crystal is predicted employing a numerical pump-probe simulation. The numerical results indicate that the time-dependence of the anisotropic response of ZnS exhibits a phase…

Optics · Physics 2019-09-11 T. Otobe

Multifractal properties of the energy time series of short $\alpha$-helix structures, specifically from a polyalanine family, are investigated through the MF-DFA technique ({\it{multifractal detrended fluctuation analysis}}). Estimates for…

Biological Physics · Physics 2010-01-13 P. H. Figueirêdo , E. Nogueira , M. A. Moret , Sérgio Coutinho

The objective of this article is to study the behavior of electromagnetic field under X-ray diffraction by time-dependent deformed crystals. Derived system of differential equations looks like the Takagi equations in the case of…

Computational Physics · Physics 2007-05-23 Svetlana Sytova

Time-dependent density-functional theory (TDDFT) is a central tool for studying the dynamical electronic structure of molecules and solids, yet aspects of its mathematical foundations remain insufficiently understood. In this work, we…

We employ the time-dependent Hartree-Fock (TDHF) method to study various aspects of the reactions utilized in searches for superheavy elements. These include capture cross-sections, quasifission, prediction of $P_{\mathrm{CN}}$, and other…

Nuclear Theory · Physics 2016-04-12 A. S. Umar , V. E. Oberacker

This paper studies the performance of time-dependent density-functional theory (TDDFT) for calculating the dielectric function of semiconductors and insulators at finite momentum transfer, comparing against the standard Bethe-Salpeter…

Materials Science · Physics 2025-03-03 Didarul Alam , Jiuyu Sun , Carsten A. Ullrich

Particles subject to weak contact interactions in a finite-size lattice tend to thermalise. The Hamiltonian evolution ensures energy conservation and the final temperature is fully determined by the initial conditions. In this work we show…

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