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A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived…

Chemical Physics · Physics 2020-01-08 Jonggu Jeon , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

Supersonic engine development requires accurate and detailed measurements of fluidic and thermodynamic parameters to optimize engine designs and benchmark computational fluid dynamic (CFD) simulations. Here, we demonstrate that dual…

Optical frequency combs have revolutionized precision measurement, time-keeping, and molecular spectroscopy. A substantial effort has developed around "microcombs": integrating comb-generating technologies into compact, reliable photonic…

We investigate the power spectral density emitted by a superconducting artificial atom coupled to the end of a semi-infinite transmission line and driven by two continuous radio-frequency fields. In this setup, we observe the generation of…

Mechanical frequency combs are poised to bring the applications and utility of optical frequency combs into the mechanical domain. So far, their main challenge has been strict requirements on drive frequencies and power, which complicate…

We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to…

Instrumentation and Detectors · Physics 2018-08-15 David R. Carlson , Daniel D. Hickstein , Daniel C. Cole , Scott A. Diddams , Scott B. Papp

Optical frequency comb devices have unlocked new capabilities in telecommunications, sensing, and metrology. Yet, precise in situ control of the comb spectral envelope remains extremely challenging. By introducing mode coupling with…

Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…

Optics · Physics 2024-03-08 Bingxin Xu , Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Frequency combs have revolutionized time and frequency metrology and in recent years, new frequency comb lasers that are highly compact or even on-chip have been demonstrated in the mid-infrared and THz regions of the electromagnetic…

Optics · Physics 2019-07-17 Giacomo Scalari , Jérôme Faist , Nathalie Picqué

Electromagnetic scattering in accelerating reference frames inspires a variety of phenomena, requiring employment of general relativity for their description. While the quasi-stationary field analysis could be applied to slowly-accelerating…

Classical Physics · Physics 2017-02-21 Vitali Kozlov , Dmitrii Filonov , Yefim Yankelevich , Pavel Ginzburg

Dual-comb spectroscopy (DCS) is a powerful Fourier-transform spectroscopic technique that provides high-speed, high-resolution, and broadband measurements without moving parts. However, the high peak power of mode-locked pulses limits the…

Optics · Physics 2025-09-30 Wei Long , Xinru Cao , Xiangze Ma , Jiaqi Zhou , Wenbin He , Dijun Chen

We report experimental observation of velocity-selective resonances in the Doppler-broadened probe absorption spectra of 85Rb and 87Rb D2 transitions in the presence of a strong copropagating pump laser locked to a frequency within the…

Classical Physics · Physics 2009-11-10 S. Chakrabarti , A. Pradhan , A. Bandyopadhyay , A. Ray , B. Ray , N. Kar , P. N. Ghosh

We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…

Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength…

CMOS-compatible Kerr microcombs have drawn substantial interest as mass-manufacturable, compact alternatives to bulk frequency combs. This could enable deployment of many comb-reliant applications previously confined to laboratories.…

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

Optical frequency combs have revolutionised time and frequency metrology [1, 2]. The advent of microresonator-based frequency combs ('microcombs' [3-5]) is set to lead to the miniaturisation of devices that are ideally suited to a wide…

We describe methods using frequency combs and optical resonators for recording two-dimensional (2D) ultrafast spectroscopy signals with high sensitivity. By coupling multiple frequency combs to higher-order modes of one or more optical…

Optics · Physics 2017-01-25 Thomas K. Allison

Optical frequency combs are laser sources which are capable of generating discrete, equal-spaced and highly coherent comb modes. Optical frequency comb technique provides a significant bridge to transfer the stability between optical…

Optics · Physics 2022-04-14 Haochen Tian

Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…