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We theoretically investigate the collisions between ultracold polar molecules in the presence of two lasers ensuring a Raman resonant transition on individual molecules to suppress photon scattering, taking the example of bosonic…

Sufficiently high densities in Bose-Einstein condensates provide favorable conditions for the production of ultralong-range polyatomic molecules consisting of one Rydberg atom and a number of neutral ground state atoms. The chemical binding…

Atomic Physics · Physics 2017-05-10 Matthew T Eiles , Jesus Perez-Rios , F Robicheaux , Chris H Greene

Ultracold temperatures in dilute quantum gases opened the way to an exquisite control of matter at the quantum level. Here we focus on the control of ultracold atomic collisions using a laser to engineer their interactions at large…

Quantum Gases · Physics 2022-02-23 T. Xie , A. Orbán , X. Xing , E. Luc-Koenig , R. Vexiau , O. Dulieu , N. Bouloufa-Maafa

This paper summarizes the recent theoretical works on inelastic collisions and chemical reactions at cold and ultracold temperatures involving neutral or ionic systems of atoms and molecules. Tables of zero-temperature rate constants of…

Chemical Physics · Physics 2010-01-28 Goulven Quéméner , Naduvalath Balakrishnan , Alexander Dalgarno

The application of random-matrix theory (RMT) to compound-nucleus (CN) reactions is reviewed. An introduction into the basic concepts of nuclear scattering theory is followed by a survey of phenomenological approaches to CN scattering. The…

Nuclear Theory · Physics 2015-05-18 G. E. Mitchell , A. Richter , H. A. Weidenmueller

The calculable $R$-matrix theory has been formulated successfully for regular boundary conditions with vanishing radial wave functions at the coordinate origins [P. Descouvemont and D. Baye, Rept. Prog. Phys. 73, 036301 (2010)]. We…

Nuclear Theory · Physics 2021-02-24 Dong Bai , Zhongzhou Ren

UKRmol+ is a new implementation of the UK R-matrix electron-molecule scattering code. Key features of the implementation are the use of quantum chemistry codes such as Molpro to provide target molecular orbitals; the optional use of mixed…

Computational Physics · Physics 2020-02-19 Zdeněk Mašín , Jakub Benda , Jimena D. Gorfinkiel , Alex G. Harvey , Jonathan Tennyson

Coherent control of atomic and molecular scattering relies on the preparation of colliding particles in superpositions of internal states, establishing interfering pathways that can be used to tune the outcome of a scattering process.…

Atomic Physics · Physics 2024-12-20 Adrien Devolder , Timur V. Tscherbul , Paul Brumer

Inspired by Wannier's threshold law, we recognize that collision complex decay meets the requirements of quantum-classical correspondence in sufficiently exothermic ultracold reactions. We make use of this correspondence to elucidate the…

Chemical Physics · Physics 2018-12-05 Micheline B. Soley , Eric J. Heller

A Feshbach resonance arises in cold atom scattering due to the complex interplay between several coupled channels. However, the essential physics of the resonance may be encapsulated in a simplified model consisting of just two coupled…

Other Condensed Matter · Physics 2009-11-11 Nicolai Nygaard , Barry I. Schneider , Paul S. Julienne

In this work we develop an approach for a molecular hydrogen ion (H2+) in the Born-Oppenheimer approximation while exposed to intense short-pulse radiation. Our starting point is the R-Matrix incorporating Time (RMT) formulation for atomic…

Atomic Physics · Physics 2016-01-01 Cathal Ó Broin , Lampros A. A. Nikolopoulos

Petaflop architectures are currently being utilized efficiently to perform large scale computations in Atomic, Molecular and Optical Collisions. We solve the Schroedinger or Dirac equation for the appropriate collision problem using the…

Distributed, Parallel, and Cluster Computing · Computer Science 2014-08-18 Brendan M. McLaughlin , Connor P. Ballance

Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…

An increasingly large variety of molecular species are being cooled down to low energies in recent years, and innovative ideas and powerful techniques continue to emerge to gain ever more precise control of molecular motion. In this brief…

Quantum Gases · Physics 2024-05-24 Tim Langen , Giacomo Valtolina , Dajun Wang , Jun Ye

Recent experimental advances in the cooling and manipulation of bialkali dimer molecules have enabled the production of gases of ultracold molecules that are not chemically reactive. It has been presumed in the literature that in the…

Multichannel quantum defect theory (MQDT) provides a powerful toolkit for describing and understanding collisions of cold alkali atoms. Various MQDT approximations differ primarily in how they characterize the so-called short-ranged…

Atomic Physics · Physics 2023-08-01 Alyson Laskowski , Nirav Mehta

The scattering of two charged strongly interacting particles is described on the basis of the P-matrix approach. In the P matrix, it is proposed to isolate explicitly the background term corresponding to purely Coulomb interaction, whereby…

Nuclear Theory · Physics 2007-05-23 V. A. Babenko , N. M. Petrov

We consider losses in collisions of ultracold molecules described by a simple statistical short-range model that explicitly accounts for the limited lifetime of classically chaotic collision complexes. This confirms that thermally sampling…

Atomic Physics · Physics 2021-11-05 Arthur Christianen , Gerrit C. Groenenboom , Tijs Karman

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

We investigate controlled collisions between trapped but separated ultracold atoms. The interaction between atoms is treated self-consistently using an energy-dependent delta-function pseudopotential model, whose validity we establish. At a…

Quantum Physics · Physics 2009-11-10 R. Stock , E. L. Bolda , I. H. Deutsch
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