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Properly designed colloidal semiconductor quantum dots (QDs) have already been shown to exhibit high sensitivity to external electric fields via the quantum confined Stark effect (QCSE). Yet, detection of the characteristic spectral shifts…

We experimentally demonstrate that the interaction between plasma and nanometer-sized semiconductor quantum dots (QDs) is directly connected to a change in their photoluminescence (PL) spectrum. This is done by taking in-situ, high…

Plasma Physics · Physics 2022-01-12 Zahra Marvi , Tim Donders , Mohammad Hasani , Guido Klaassen , Job Beckers

Colloidal semiconductor quantum dots are robust emitters implemented in numerous prototype and commercial optoelectronic devices. However, active fluorescence color tuning, achieved so far by electric-field induced Stark effect, has been…

Mesoscale and Nanoscale Physics · Physics 2023-05-16 Yonatan Ossia , Adar Levi , Yossef E. Panfil , Somnath Koley , Einav Scharf , Nadav Chefetz , Sergei Remennik , Atzmon Vakahi , Uri Banin

We optimized the performance of quantum confined Stark effect QCSE based voltage nanosensors. A high throughput approach for single particle QCSE characterization was developed and utilized to screen a library of such nanosensors. Type II…

Mesoscale and Nanoscale Physics · Physics 2021-08-04 Yung Kuo , Jack Li , Xavier Michalet , Alexey Chizhik , Noga Meir , Omri Bar-Elli , Emory Chan , Dan Oron , Joerg Enderlein , Shimon Weiss

Continuous and concerted development of colloidal quantum-dot light-emitting diodes over the past two decades has established them as a bedrock technology for the next generation of displays. However, a fundamental issue that limits the…

Spectral diffusion (SD) represents a substantial obstacle towards implementation of solid-state quantum emitters as a source of indistinguishable photons. By performing high-resolution emission spectroscopy for individual colloidal quantum…

Mesoscale and Nanoscale Physics · Physics 2023-11-21 Frieder Conradt , Vincent Bezold , Volker Wiechert , Steffen Huber , Stefan Mecking , Alfred Leitenstorfer , Ron Tenne

Quantum dots (QDs) are semiconductor nanostructures in which a three dimensional potential trap produces an electronic quantum confinement, thus mimicking the behaviour of single atomic dipole-like transitions. However unlike atoms, QDs can…

Active modulation of quantum dot thin film photoluminescence (PL) has far-reaching potential applications in biomedical and optoelectronic systems, but challenges remain in achieving large PL modulation depth and fast temporal response.…

Applied Physics · Physics 2024-06-19 Sihan Xie , Han Zhu , Melissa Li , Vladimir Bulović

The quantum confinement effect on the spectrum of near-field thermal radiation by periodic and random arrays of quantum dots (QDs) is investigated. The local density of states (LDOS) thermally emitted by QD arrays made of three lead…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Saman Zare , Sheila Edalatpour

The optics of dangling-bond-free van der Waals heterostructures containing transition metal dichalcogenides are dominated by excitons. A crucial property of a confined exciton is the quantum confined Stark effect (QCSE). Here, such a…

The $k\cdot p$ effective mass approximation (EMA) predicts large, nearly size-independent exciton oscillator strengths in quantum confined semiconductors. Yet, experimental reports have concluded that the total oscillator strength of the…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Yanhao Tang , Mersedeh Saniepay , Chenjia Mi , Rémi Beaulac , John A. McGuire

Recently, there has been tremendous research interest in novel bismide semiconductor materials (such as GaBi$_x$As$_{1-x}$) for wavelength-engineered, low-loss optoelectronic devices. We report a first study of the quantum confined Stark…

Materials Science · Physics 2019-07-19 Muhammad Usman

Quantum Stark effect in semiconductor nanocrystals is theoretically investigated, using the effective mass formalism within a $4\times 4$ Baldereschi-Lipari Hamiltonian model for the hole states. General expressions are reported for the…

Materials Science · Physics 2009-11-10 Eduardo Ariel Menendez Proupin , Carlos Trallero Giner

The energy levels and optical transitions of tetrahedral core/shell InP/ZnSe quantum dots (QDs) are investigated by means of multi-band k$\cdot$p theory. Despite the $\overline{T}_d$ symmetry relaxing spherical selection rules, the…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Josep Planelles , Juan I. Climente

Colloidal quantum dots (cQDs) are now a mature nanomaterial with optical properties customizable through varying size and composition. However, their use in optical devices is limited as they are not widely available in convenient forms…

Demonstrating the quantum-confined Stark effect (QCSE) in silicon nanocrystals (NCs) embedded in oxide has been rather elusive, unlike the other materials. Here, the recent experimental data from ion-implanted Si NCs is unambiguously…

Mesoscale and Nanoscale Physics · Physics 2010-04-23 Ceyhun Bulutay , Mustafa Kulakci , Raşit Turan

We report on a temporal evolution of photoluminescence (PL) spectroscopy of CuInS$_{2}$/ZnS colloidal quantum dots (QDs) by drop-casting on SiO$_{2}$/Si substrates and high quality factor microdisks (MDs) under different atmospheric…

Telecom wavelength quantum dots (QDs) are emerging as a promising solution for generating deterministic single photons compatible with existing fiber optic infrastructure. Emission in the low loss C band minimizes transmission losses,…

Achieving localized light emission from monolayer two-dimensional (2D) transition metal dichalcogenides (TMDs) embedded in the matrix of another TMD has been theoretically proposed but not experimentally proven. In this study, we used…

In this paper, we analyze the performance of an electro-optic modulator based on a single quantum dot strongly coupled to a nano-resonator, where electrical control of the quantum dot frequency is achieved via quantum confined Stark effect.…

Quantum Physics · Physics 2011-01-20 Arka Majumdar , Nicolas Manquest , Andrei Faraon , Jelena Vuckovic
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