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Polarization-entangled photon pairs generated from second-order nonlinear optical media have been extensively studied for both fundamental research and potential applications of quantum information. In spontaneous parametric down-conversion…

Quantum Physics · Physics 2024-10-01 B. S. Ham

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…

The quantum entanglement enables the precision measurement and frequency metrology beyond the standard quantum limit that is imposed by the quantum projection noise and photon shot noise. Here we propose employing the entangled atoms in the…

Quantum Physics · Physics 2023-05-10 Deshui Yu , Jingbiao Chen , Shougang Zhang

Spontaneous parametric down-conversion is a vital method for generating correlated photon pairs in the visible and near-infrared spectral regions; however, its extension to X-ray frequencies has faced substantial barriers. Here, we present…

We measure the joint temporal intensity of signal and idler photon pairs generated by spontaneous four wave mixing in a silicon nitride microresonator by time-resolved coincidence detection. This technique can be applied to any high-Q…

Quantum Physics · Physics 2025-05-19 Massimo Borghi , Paula Lujan Pagano , Marco Liscidini , Daniele Bajoni , Matteo Galli

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…

Quantum Physics · Physics 2022-05-31 Bryce P. Hickam , Manni He , Nathan Harper , Szilard Szoke , Scott Cushing

Decay of a four-level diamond scheme via a cascade is a potential source of entangled photon pairs. A solid-state implementation is the biexciton cascade in a semiconductor quantum dot. While high entanglement fidelities have been…

We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

We demonstrate sub-shot-noise photon-number correlations in a (temporal) multimode mesoscopic ($\sim 10^3$ detected photons) twin-beam produced by ps-pulsed spontaneous non-degenerate parametric downconversion. We have separately detected…

Quantum Physics · Physics 2009-11-13 Maria Bondani , Alessia Allevi , Guido Zambra , Matteo G. A. Paris , Alessandra Andreoni

Coincidence detection is a key technique used in nonlocal quantum-correlation measurements to test Bell inequality violation between remotely separated local detectors. With individual uniform intensity of local measurements, the nonlocal…

Quantum Physics · Physics 2022-03-16 B. S. Ham

We propose and demonstrate experimentally a new method based on the spatial entanglement for the absolute calibration of analog detector. The idea consists on measuring the sub-shot-noise intensity correlation between two branches of…

High-dimensional entanglement is a promising resource for quantum technologies. Being able to certify it for any quantum state is essential. However, to date, experimental entanglement certification methods are imperfect and leave some…

The Hong-Ou-Mandel interference effect lies at the heart of many emerging quantum technologies whose performance can be significantly enhanced with increasing numbers of entangled modes one could measure and thus utilize. Photon pairs…

Quantum Physics · Physics 2022-06-08 Xiaoqin Gao , Yingwen Zhang , Alessio D'Errico , Khabat Heshami , Ebrahim Karimi

Temporal photon correlations have been a crucial resource for quantum and quantum-enabled optical science for over half a century. However, attaining non-classical information through these correlations has typically been limited to a…

Photon-pair correlations in spontaneous parametric down conversion are ubiquitous in quantum photonics. The ability to engineer their properties for optimising a specific task is essential, but often challenging in practice. We demonstrate…

Quantum Physics · Physics 2024-03-11 Chloé Vernière , Hugo Defienne

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

The aim of this review paper is to enlighten some recent progresses in quantum optical metrology in the part of quantum efficiency measurements of photo-detectors performed with bi-photon states. The intrinsic correlated nature of entangled…

Quantum Physics · Physics 2015-06-26 G. Brida , M. Genovese , M. Gramegna

A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…

We demonstrate a method to measure coincidences between polarization-entangled photons distributed to distant locations, eliminating traditional synchronization by employing a compact, chip-scale atomic clock for precise timing.

We have experimentally demonstrated a clock comparison scheme utilizing time-correlated photon pairs generated from the spontaneous parametric down conversion process of a laser pumped beta-barium borate crystal. The coincidence of…

Optics · Physics 2015-09-30 Shi-Wei Zhang , Jia-Zheng Song , Yin-Ping Yao , Ren-Gang Wan , Tong-Yi Zhang