English
Related papers

Related papers: Electronic excitations in $\gamma$-Li$_2$IrO$_3$

200 papers

Honeycomb Na$_2$IrO$_3$ is a prototype spin-orbit Mott insulator and Kitaev magnet. We report a combined structural and electrical resistivity study of Na$_2$IrO$_3$ single crystals. Laue back-scattering diffraction indicates twinning with…

Strongly Correlated Electrons · Physics 2023-12-12 Franziska A. Breitner , Julian Kaiser , Anton Jesche , Philipp Gegenwart

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

Optical conductivity measurements are combined with density functional theory calculations in order to understand the electrodynamic response of the frustrated Mott insulators Herbertsmithite $\mathrm{ZnCu_{3}(OH)_{6}Cl_{2}}$ and the…

Strongly Correlated Electrons · Physics 2018-01-10 Andrej Pustogow , Ying Li , Ievgen Voloshenko , Pascal Puphal , Cornelius Krellner , Igor I. Mazin , Martin Dressel , Roser Valentí

The realization of Kitaev spin liquid, where spins on a honeycomb lattice are coupled ferromagnetically by bond-dependent anisotropic interactions, has been a sought-after dream. 5d iridium oxides $\alpha$-Li2IrO3 and $\alpha$-Na2IrO3 with…

Strongly Correlated Electrons · Physics 2015-03-05 T. Takayama , A. Kato , R. Dinnebier , J. Nuss , H. Takagi

We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir$^{4+}$ ions in a family of layered iridates $A_2$IrO$_3$ ($A$=Li,Na). Depending on the microscopic parameters, the…

Strongly Correlated Electrons · Physics 2014-11-20 Jiri Chaloupka , George Jackeli , Giniyat Khaliullin

Transition metal oxides display a great variety of quantum electronic behaviours where correlations often play an important role. The achievement of high quality epitaxial interfaces involving such materials gives a unique opportunity to…

Direct experimental investigations of the low-energy electronic structure of the Na$_2$IrO$_3$ iridate insulator are sparse and draw two conflicting pictures. One relies on flat bands and a clear gap, the other involves dispersive states…

The recently-synthesized iridate $\beta$-Li$_2$IrO$_3$ has been proposed as a candidate to display novel magnetic behavior stabilized by frustration effects from bond-dependent, anisotropic interactions (Kitaev model) on a three-dimensional…

Strongly Correlated Electrons · Physics 2014-12-02 A. Biffin , R. D. Johnson , Sungkyun Choi , F. Freund , S. Manni , A. Bombardi , P. Manuel , P. Gegenwart , R. Coldea

The electrodynamic response of organic spin liquids with highly-frustrated triangular lattices has been measured in a wide energy range. While the overall optical spectra of these Mott insulators are governed by transitions between the…

Strongly Correlated Electrons · Physics 2018-08-09 A. Pustogow , Y. Saito , E. Zhukova , B. Gorshunov , R. Kato , T. -H. Lee , S. Fratini , V. Dobrosavljević , M. Dressel

The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

Kitaev's honeycomb spin-liquid model and its proposed realization in materials such as $\alpha$-RuCl$_3$, Li$_2$IrO$_3$ and Na$_2$IrO$_3$ continue to present open questions about how the dynamics of a spin-liquid are modified in the…

Strongly Correlated Electrons · Physics 2020-02-12 R. Sarkar , Z. Mei , A. Ruiz , G. Lopez , H. -H. Klauss , J. G. Analytis , I. Kimchi , N. J. Curro

Electronic transport near the insulator-metal transition is investigated in the molecular beam epitaxy-grown SrTiO3/Nd1-xTiO3/SrTiO3 heterostructures using temperature dependent magnetotransport measurements. It was found that Nd-vacancies…

Materials Science · Physics 2019-07-03 Laxman Raju Thoutam , Jin Yue , Peng Xu , Bharat Jalan

Thermomagnetic and inelastic neutron scattering measurements on Na2PrO3 are reported. This material is an antiferromagnetic honeycomb magnet based on the tetravalent lanthanide Pr4+ and has been proposed to host dominant antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-03-17 Marcus J. Daum , Arun Ramanathan , Alexander I. Kolesnikov , Stuart A. Calder , Martin Mourigal , Henry S. La Pierre

We investigate the dynamical properties of ${\rm Na_2IrO_3}$. For five effective models proposed for ${\rm Na_2IrO_3}$, we numerically calculate dynamical structure factors (DSFs) with an exact diagonalization method. An effective model…

Strongly Correlated Electrons · Physics 2015-11-25 Takafumi Suzuki , Takuto Yamada , Youhei Yamaji , Sei-ichiro Suga

The electronic structure of the honeycomb lattice iridates Na2IrO3 and Li2IrO3 has been investigated using resonant inelastic x-ray scattering (RIXS). Crystal-field split d-d excitations are resolved in the high-resolution RIXS spectra. In…

A pseudo honeycomb system Li2RuO3 exhibits a second-order-like transition at temperature T=Tc=540 K to a low-T nonmagnetic phase with a significant lattice distortion forming Ru-Ru pairs. For this system, we have calculated the band…

Strongly Correlated Electrons · Physics 2015-05-13 Yoko Miura , Masatoshi Sato , Youichi Yamakawa , Tatsuro Habaguchi , Yoshiaki Ono

The anisotropy of low energy (0$\sim$5eV) optical excitations in strongly correlated transition-metal oxides is closely related to the spin and orbital orderings. The recent successes of LDA+$U$ method in describing the magnetic and…

Strongly Correlated Electrons · Physics 2009-11-07 Zhong Fang , Naoto Nagaosa , Kiyoyuki Terakura

Inelastic light scattering from Dirac-type electrons in graphene is shown to be dominated by the generation of the inter-band electronic modes which are odd in terms of time-inversion symmetry and belong to the irreducible representation…

Mesoscale and Nanoscale Physics · Physics 2010-01-25 Oleksiy Kashuba , Vladimir I. Fal'ko

We explore the response of Ir $5d$ orbitals to pressure in $\beta$-$\mathrm{Li_2IrO_3}$, a hyperhoneycomb iridate in proximity to a Kitaev quantum spin liquid (QSL) ground state. X-ray absorption spectroscopy reveals a reconstruction of the…

Two recent theoretical works studied the role of Kitaev interactions in the newly observed incommensurate magnetic order in the hyper-honeycomb ($\beta$-Li$_2$IrO$_3$) and stripy-honeycomb ($\gamma$-Li$_2$IrO$_3$) iridates. Each of these…

Strongly Correlated Electrons · Physics 2016-05-25 Eric Kin-Ho Lee , Jeffrey G. Rau , Yong Baek Kim