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The competition between the electron-hole Coulomb attraction and the three-dimensional dielectric screening dictates the optical properties of layered semiconductors. In low-dimensional materials, the equilibrium dielectric environment can…

Harnessing low energy photons is of paramount importance for multi-junction high efficiency solar cells as well as for thermo-photovoltaic applications. However, semiconductor absorbers with bandgap lower than 0.8 eV have been limited to…

We study the carrier relaxation dynamics in thin black phosphorus (bP) using time-resolved differential transmission measurements. The inter-band and intra-band transitions, relaxation, and carrier recombination lifetimes are revealed by…

Materials Science · Physics 2018-08-15 Y. Aytac , M. Mittendoff , T. E. Murphy

Black phosphorus is a quasi-two-dimensional layered semiconductor with a narrow direct band gap of 0.3 eV. A giant surface Stark effect can be produced by the potassium doping of black phosphorus, leading to a semiconductor to semimetal…

Materials Science · Physics 2021-07-21 G. Kremer , M. Rumo , C. Yue , A. Pulkkinen , C. W. Nicholson , T. Jaouen , F. O. von Rohr , P. Werner , C. Monney

The ability to detect light over a broad spectral range is central for practical optoelectronic applications, and has been successfully demonstrated with photodetectors of two-dimensional layered crystals such as graphene and MoS2. However,…

Chemical doping of bulk black phosphorus is a well-recognized way to reduce surface oxidation and degradation. Here, we report on the fabrication of terahertz frequency detectors consisting of an antenna-coupled field-effect transistor…

Mesoscale and Nanoscale Physics · Physics 2019-03-08 Leonardo Viti , Antonio Politano , Kai Zhang , Miriam Serena Vitiello

Revived attention in black phosphorus (bP) has been tremendous in the past decade. While many photoinitiated experiments have been conducted, a cross-examination of bP's photocarrier and structural dynamics is still lacking. In this report,…

Materials Science · Physics 2023-05-24 Mazhar Chebl , Xing He , Ding-Shyue Yang

Atomic layers of Black Phosphorus (BP) present unique opto-electronic properties dominated by a direct tunable bandgap in a wide spectral range from visible to mid-infrared. In this work, we investigate the infrared photoluminescence of BP…

Mesoscale and Nanoscale Physics · Physics 2021-01-13 Etienne Carré , Lorenzo Sponza , Alain Lusson , Ingrid Stenger , Etienne Gaufrès , Annick Loiseau , Julien Barjon

A long-wavelength infrared (IR) photodetector based on two-dimensional materials working at room temperature would have wide applications in many aspects in remote sensing, thermal imaging, biomedical optics, and medical imaging. However,…

Black phosphorous (BP) is a layered semiconductor with high carrier mobility, anisotropic optical response and wide bandgap tunability. In view of its application in optoelectronic devices, understanding transient photo-induced effects is…

Mesoscale and Nanoscale Physics · Physics 2022-09-07 H. Hedayat , A. Ceraso , G. Soavi , S. Akhavan , A. Cadore , C. Dallera , G. Cerullo , A. C. Ferrari , E. Carpene

Nonlinear interferometers allow for mid-infrared spectroscopy with near-infrared detection using correlated photons. Previous implementations have demonstrated a spectral resolution limited by spectrally selective detection. In our work, we…

Controlling the bandgap through local-strain engineering is an exciting avenue for tailoring optoelectronic materials. Two-dimensional crystals are particularly suited for this purpose because they can withstand unprecedented…

Black phosphorus is a very promising material for telecommunication due to its direct bandgap and strong resonant absorption in near-infrared wavelength range. However, ultrafast nonlinear photonic applications relying on the ultrafast…

Mid-infrared photodetectors are susceptible to background noise since every object in the surroundings emits thermal radiation from different directions. To reduce this background noise and enhance signal-to-noise ratio of mid-infrared…

Optics · Physics 2025-04-30 Ziwei Fan , Taeseung Hwang , Yixin Chen , Zi Jing Wong

Harvesting hot carriers before they lose energy to the lattice is a critical route toward surpassing the conventional thermodynamic limit in optical-to-electrical (O-E) conversion. However, photocurrent from such hot carriers has remained…

Mesoscale and Nanoscale Physics · Physics 2025-06-18 Katsumasa Yoshioka , Taro Wakamura , Takuya Okamoto , Norio Kumada

While advancing a physics-based comprehensive photodetector-simulation model, we propose a novel device design of the mid-wavelength infrared nBn photodetectors by exploiting the inherit flexibility of the $InAs_{1-x}Sb_{x}$ ternary alloy…

Mesoscale and Nanoscale Physics · Physics 2023-10-03 Rohit Kumar , Bhaskaran Muralidharan

We report visible light detection with in-plane BiFeO3 (BFO) thin films grown on pre-patterned inter-digital electrodes. In-plane configured BFO film displayed photocurrents with a 40:1 photo-to-dark-current ratio and improved photo-sensing…

Materials Science · Physics 2015-06-19 Avneesh Anshul , Hitesh Borkar , Paritosh Singh , Prabir Pal , Sunil S Kushvaha , Ashok Kumar

Phosphorene, a single atomic layer of black phosphorus, has recently emerged as a new twodimensional (2D) material that holds promise for electronic and photonic technology. Here we experimentally demonstrate that the electronic structure…

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

Strongly Correlated Electrons · Physics 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

We demonstrate thin-film metamaterials with resonances in the mid-infrared wavelength range. Our structures are numerically modeled and experimentally characterized by reflection and angularly-resolved thermal emission spectroscopy. We…

Optics · Physics 2011-08-18 J. A. Mason , S. Smith , D. Wasserman