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Representation of molecular vibrational degrees of freedom by independent harmonic oscillators, when describing electronic spectra or electronic excitation energy transport, raises unfavourable effects as vibrational energy relaxation…

Chemical Physics · Physics 2018-07-26 Mantas Jakučionis , Vladimir Chorošajev , Darius Abramavičius

We investigate the dynamics of coherence and entanglement of vibrating qubits. Firstly, we consider a single trapped ion qubit inside a perfect cavity and successively we use it to construct a bipartite system made of two of such…

Quantum Physics · Physics 2018-05-14 Ali Mortezapour , Ghasem Naeimi , Rosario Lo Franco

Two elastically coupled nanomechanical resonators driven independently near their resonance frequencies show intricate nonlinear dynamics. The dynamics provide a scheme for realizing a nanomechanical system with tunable frequency and…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 R. B. Karabalin , M. C. Cross , M. L. Roukes

We have investigated the phonon dynamics of a single-molecule embedded in a mechanical resonator made of an organic crystal. The whole system is placed in an optical resonator within the bad cavity limit. We have found that the optical…

Quantum Physics · Physics 2024-01-05 Victor Ceban , Mihai A. Macovei

We propose a novel approach to calculate dynamical processes at ultrafast time scale in molecules in which vibrational and electronic motions are strongly mixed. The relevant electronic orbitals and their interactions are described by a…

Strongly Correlated Electrons · Physics 2009-11-07 L. Arrachea , A. A. Aligia , G. E. Santoro

Determining the vibrational structure of a molecule is central to fundamental applications in several areas, from atmospheric science to catalysis, fuel combustion modeling, biochemical imaging, and astrochemistry. However, when significant…

Quantum Physics · Physics 2021-12-22 Nicolas P. D. Sawaya , Francesco Paesani , Daniel P. Tabor

A method is provided for approximating random slow manifolds of a class of slow-fast stochastic dynamical systems. Thus approximate, low dimensional, reduced slow systems are obtained analytically in the case of sufficiently large time…

Dynamical Systems · Mathematics 2013-03-12 Jian Ren , Jinqiao Duan , Christopher K. R. T. Jones

The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

Dynamical decoupling is the leading technique to remove unwanted interactions in a vast range of quantum systems through fast rotations. But what determines the time-scale of such rotations in order to achieve good decoupling? By providing…

Quantum Physics · Physics 2021-08-11 Daniel Burgarth , Paolo Facchi , Martin Fraas , Robin Hillier

For many biological applications of molecular dynamics (MD) the importance of good sampling in conformational space makes it necessary to eliminate the fastest motions from the system in order to increase the time step. An accurate…

Computational Physics · Physics 2007-05-23 Alexey K. Mazur

Isolated many-body quantum systems quenched far from equilibrium can eventually equilibrate, but it is not yet clear how long they take to do so. To answer this question, we use exact numerical methods and analyze the entire evolution, from…

Disordered Systems and Neural Networks · Physics 2021-08-20 Talía L. M. Lezama , E. Jonathan Torres-Herrera , Francisco Pérez-Bernal , Yevgeny Bar Lev , Lea F. Santos

Understanding how the effectiveness of natural photosynthetic energy harvesting systems arises from the interplay between quantum coherence and environmental noise represents a significant challenge for quantum theory. Recently it has begun…

Biological Physics · Physics 2015-06-16 E. K. Irish , R. Gómez-Bombarelli , B. W. Lovett

We study a noisy oscillator with pulse delayed feedback, theoretically and in an electronic experimental implementation. Without noise, this system has multiple stable periodic regimes. We consider two types of noise: i) phase noise acting…

Adaptation and Self-Organizing Systems · Physics 2020-08-26 Vladimir Klinshov , Dmitry Shchapin , Otti D'Huys

We examine microscopic mechanisms for coupling stochastic oscillators so that they display similar and correlated temporal variations. Unlike oscillatory motion in deterministic dynamical systems, complete synchronization of stochastic…

Quantitative Methods · Quantitative Biology 2009-09-29 Amitabha Nandi , G. Santhosh , R. K. Brojen Singh , Ram Ramaswamy

Machine learning over-fitting caused by data scarcity greatly limits the application of machine learning for molecules. Due to manufacturing processes difference, big data is not always rendered available through computational chemistry…

Machine Learning · Computer Science 2020-11-20 Ziyang Zhang , Yingtao Luo

As circuits continue to miniaturize, noise has become a significant obstacle to performance optimization. Stochastic resonance in logic circuits offers an innovative approach to harness noise constructively; however, current implementations…

Adaptation and Self-Organizing Systems · Physics 2024-10-11 Mengen Shen , Jianhua Yang , Miguel A. F. Sanjuán , Huatao Chen , Zhongqiu Wang

We describe a method that focuses sampling effort on a user-defined selection of a large system, which can lead to substantial decreases in computational effort by speeding up the calculation of nonbonded interactions. A naive approach can…

Statistical Mechanics · Physics 2023-08-28 Joshua Fass , Forrest York , Matthew Wittmann , Joseph Kaus , Yutong Zhao

We study collective oscillations of a two-flavor neutrino system with arbitrary but fixed density. In the vacuum limit, modes with different energies quickly de-phase (kinematical decoherence), whereas in the limit of infinite density they…

High Energy Physics - Phenomenology · Physics 2010-12-24 Georg G. Raffelt , Irene Tamborra

A dynamical decoupling method is presented which is based on embedding a deterministic decoupling scheme into a stochastic one. This way it is possible to combine the advantages of both methods and to increase the suppression of undesired…

Quantum Physics · Physics 2007-05-23 Oliver Kern , Gernot Alber

Spontaneous synchronization between coupled periodic systems occur in a wealth of classical physical setups. Here, we show theoretically that the phase of two distinct quantum harmonic oscillators spontaneously when they are strongly…

Quantum Physics · Physics 2019-09-04 Loic Henriet