English
Related papers

Related papers: Multiple Rabi Splittings under Ultra-Strong Vibrat…

200 papers

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

Plasmonic dimer cavities can induce extreme electric-field hot spots that allow one to access ultrastrong coupling regimes using Raman-type spectroscopy on single vibrating molecules. Using a generalized master equation, we study resonant…

Quantum Physics · Physics 2021-07-29 Stephen Hughes , Alessio Settineri , Salvatore Savasta , Franco Nori

We consider an ensemble of homonuclear diatomic molecules coupled to the two polarization directions of a Fabry-P\'erot cavity via fully quantum simulations. Accompanied by analytical results, we identify a coupling mechanism mediated…

Chemical Physics · Physics 2024-01-22 Niclas Krupp , Oriol Vendrell

Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial…

We investigate coherent nonlinear dynamics of 2D electrons under ultrafast intersubband excitation by mid-IR pulses. We include the effects of relaxation and dephasing, both homogeneous and inhomogeneous, as well as detuning within a…

Statistical Mechanics · Physics 2016-08-31 D. McPeake , F. T. Vasko , E. P. O'Reilly

We present a quantitative study of the nonlinear optical response of layered perovskites placed inside planar photonic microcavities in the regime of strong light matter coupling, when excitonic and photonic modes hybridize and give rise to…

Mesoscale and Nanoscale Physics · Physics 2022-11-15 A. D. Belogur , D. A. Baghdasaryan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

When the coupling between light and matter becomes comparable to the energy gap between different excited states they hybridize, leading to the appearance of a rich and complex phenomenology which attracted remarkable interest in recent…

Strong coupling between light and matter is possible with a variety of organic materials. In contrast to the simpler inorganic case, organic materials often have a complicated spectrum, with vibrationally dressed electronic transitions.…

Mesoscale and Nanoscale Physics · Physics 2018-02-02 M. Ahsan Zeb , Peter G. Kirton , Jonathan Keeling

The nonlinear optical response of organic polaritonic matter has received increasing attention due to their enhanced and controllable nonlinear response and their potential for novel optical devices such as compact photon sources and…

Vacuum Rabi splitting relies on symmetrical splitting of the common resonance frequency of atoms and the cavity in which the atoms reside. In this work, we argue that vacuum Rabi splitting is a manifestation of virtual light-matter two-mode…

Quantum Physics · Physics 2024-03-20 Karol Gietka

Optical trapping of molecules with long coherence times is crucial for many protocols in quantum information and metrology. However, the factors that limit the lifetimes of the trapped molecules remain elusive and require improved…

Atomic Physics · Physics 2020-10-14 K. H. Leung , I. Majewska , H. Bekker , C. -H. Lee , E. Tiberi , S. S. Kondov , R. Moszynski , T. Zelevinsky

Nonperturbative coupling of light with condensed matter in an optical cavity is expected to reveal a host of coherent many-body phenomena and states. In addition, strong coherent light-matter interaction in a solid-state environment is of…

We report on strong coupling between surface plasmon polaritons (SPP) and Rhodamine 6G (R6G) molecules, with double vacuum Rabi splitting energies up to 230 and 110 meV. In addition, we demonstrate the emission of all three energy branches…

We investigate the regime of strong coupling of an ensemble of two-dimensional electrons to a single-mode cavity resonator. In particular, we realized such a regime of light-matter interaction by coupling the cyclotron motion of a…

Mesoscale and Nanoscale Physics · Physics 2018-12-26 Jiabao Chen , Oleksiy Zadorozhko , Denis Konstantinov

We study a semiconductor based quantum metamaterial which has the optical characteristics of a metal in two directions, but behaves like a collection of artificial atoms, whose properties can be designed in using quantum theory, in the…

Other Condensed Matter · Physics 2009-11-13 Jonathan Plumridge , Edmund Clarke , Ray Murray , Chris Phillips

Enhancement of light-matter interactions is of great importance for many nanophotonic devices, and one way to achieve it is to feed energy perfectly to the strongly coupled system. Here, we propose gap-perturbed dimerized gratings based on…

Optics · Physics 2023-02-08 Xin Gu , Xing Liu , Xiaofei Yan , Qi Lin , Wenjuan Du , Lingling Wang , Guidong Liu

We propose a hybrid quantum system where the strong coupling regime can be achieved between a Rydberg atomic ensemble and propagating surface phonon polaritons on a piezoelectric superlattice. By exploiting the large electric dipole moment…

Optics · Physics 2016-09-07 Jiteng Sheng , Yuanxi Chao , James P. Shaffer

We theoretically demonstrate that chemical reaction rate constant can be significantly suppressed by coupling molecular vibrations with an optical cavity, exhibiting both the collective coupling effect and the cavity-frequency modification…

Chemical Physics · Physics 2022-01-26 Arkajit Mandal , Xinyang Li , Pengfei Huo

We demonstrate a new type of transition within the strong coupling regime, which alters the coupling mechanism in multimode cavities. We show that this transition drastically modifies the Hamiltonian describing the polaritons, such that…

Mesoscale and Nanoscale Physics · Physics 2021-06-16 M. Balasubrahmaniyam , C. Genet , T. Schwartz

Modeling the dielectric behavior of molecular materials made up of large pi-conjugated molecules is an interesting and complex task. Here we address linear polarizabilities, and the related dielectric constant, of molecular crystals and…

Chemical Physics · Physics 2007-05-23 Francesca Terenziani , Anna Painelli , Zoltan G. Soos