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Related papers: Soft Phonon Mode Dynamics in Aurivillius Type Stru…

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Temperature dependent inelastic neutron-scattering measurements of the generalized phonon density-of-states for superconducting MgCNi_3, T_c=8 K, give evidence for a soft-mode behavior of low-frequency Ni phonon modes. Results are compared…

Superconductivity · Physics 2009-11-10 R. Heid , B. Renker , H. Schober , P. Adelmann , D. Ernst , K. -P. Bohnen

Using first-principle calculations, we restrained the m=1 oxyfluoride Aurivillius Bi$_2$TiO4F$_2$ to adopt three ordered key configurations, such as tetragonal $I4/mmm$ phases with fluorine anions distributed either at the octahedral apical…

Materials Science · Physics 2021-06-01 Sarah Benomar , Hania Djani

Neutron scattering measurements of the lowest-energy TO phonons in the relaxor Pb(Mg1/3Nb2/3)O3 (PMN) are reported for 10<=T<=750 K. The soft mode, which is overdamped by the polar nanoregions below the Burns temperature T_d = 620 K,…

Materials Science · Physics 2009-11-07 S. Wakimoto , C. Stock , R. J. Birgeneau , Z. -G. Ye , W. Chen , W. J. L. Buyers , P. M. Gehring , G. Shirane

Metal-organic frameworks (MOFs) are crystalline materials consisting of metal centers and organic linkers forming open and porous structures. They have been extensively studied due to various possible applications exploiting their large…

Materials Science · Physics 2019-11-20 Tomas Kamencek , Natalia Bedoya-Martínez , Egbert Zojer

Comprehensive inelastic neutron-scattering measurements were performed to study the soft optical phonons in La2-xSrxCuO4 at x=0.10, 0.12 and 0.18. We found at x=0.18 that the softening of Z-point phonon, suggesting incipient structural…

Superconductivity · Physics 2009-10-31 H. Kimura , K. Hirota , C. H. Lee , K. Yamada , G. Shirane

We investigate the magnetization dynamics of $TmFeO_3$ single crystals across the spin-reorientation phase transition using broadband microwave absorption spectroscopy up to 87.5 GHz. Temperature- and magnetic-field-dependent…

The analysis of phonon anomalies provides valuable information about the cooperative dynamics of lattice, spin and charge degrees of freedom. Significant is the anomalous temperature dependence of the external modes observed in…

Strongly Correlated Electrons · Physics 2010-05-24 Ch. Hartinger , F. Mayr , A. Loidl , T. Kopp

Density-functional simulations are used to calculate structural properties and high-symmetry phonons of the hypothetical cubic phase, the stable orthorhombic phase and an intermediate tetragonal phase of magnesium silicate perovskite. We…

mtrl-th · Physics 2016-09-07 M. C. Warren , G. J. Ackland

The phonon dispersion and the electron-phonon interaction for the $\beta$-Po and the bcc high pressure phases of tellurium are computed with density-functional perturbation theory. Our calculations reproduce and explain the experimentally…

I study the experimentally observed metal-to-metal structural phase transition in NaTiO$_2$ using density functional calculations. I do not find the previously proposed low-temperature structure energetically favorable with respect to the…

Strongly Correlated Electrons · Physics 2017-05-31 Alaska Subedi

Ferropericlase (Fp), (Mg$_\mathrm{1-x}$Fe$_\mathrm{x}$)O, is the second most abundant phase in the Earths lower mantle. At relevant pressure-temperature conditions, iron in Fp undergoes a high spin (HS), S=2, to low spin (LS), S=0, state…

Geophysics · Physics 2020-10-28 Michel L. Marcondes , Fawei Zheng , Renata M. Wentzcovitch

The symmetry breaking induced by the ferroelectric transition often triggers the emergence of topological electronic states such as Weyl fermions in ferroelectric-like metals/semimetals. Such strong coupling between the lattice deformation…

Materials Science · Physics 2022-04-14 Y. Okamura , H. Handa , R. Yoshimi , A. Tsukazaki , K. S. Takahashi , M. Kawasaki , Y. Tokura , Y. Takahashi

THz-range dielectric spectroscopy and first-principle-based effective-Hamiltonian molecular dynamics simulations were employed to elucidate the dielectric response in the paraelectric phase of (Ba,Sr)TiO3 solid solutions. Analysis of the…

Materials Science · Physics 2012-11-30 J. Weerasinghe , L. Bellaiche , T. Ostapchuk , P. Kuzel , C. Kadlec , S. Lisenkov , I. Ponomareva , J. Hlinka

The novel ferroelectric-like structural transition observed in metallic LiOsO$_3$ [Y. Shi et al., Nat. Mater. 12, 1024 (2013)], has invoked many theoretical and experimental interests. In this work, we have performed polarized and…

Materials Science · Physics 2017-03-09 Feng Jin , Anmin Zhang , Jianting Ji , Kai Liu , Le Wang , Youguo Shi , Yong Tian , Xiaoli Ma , Qingming Zhang

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

Materials Science · Physics 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

Transition metal dichalcogenide monolayers and heterostructures are highly tunable material systems that provide excellent models for physical phenomena at the two-dimensional (2D) limit. While most studies to date have focused on electrons…

Phonon dispersion in a two-dimensional electron-lattice system described by a two-dimensional square-lattice version of Su-Schrieffer-Heeger's model and having the half-filled electronic band is studied theoretically at temperatures higher…

Soft Condensed Matter · Physics 2009-11-10 Shutaro Chiba , Yoshiyuki Ono

Despite extensive research interests in perovskite oxides, low energy consumption, non-destructive and maneuverable methods for phase transition in perovskite oxides are still the under its exploration, and the underlying mechanisms remain…

Materials Science · Physics 2023-08-10 Cong Zhou , Jian Zhou

We have used an effective model of ferroelectric PbTiO$_{3}$, which displays a representative soft mode-driven phase transition, to investigate how different features of the potential-energy surface affect the transition temperature $T_{\rm…

Materials Science · Physics 2013-12-05 Jacek C. Wojdeł , Jorge Íñiguez

We investigated phonon behavior of hexagonal close packed titanium under homogeneous shear deformation corresponding to the $\{10\bar{1}2\}$ twinning mode using first-principles calculation and phonon calculation. By this deformation, we…

Materials Science · Physics 2020-07-22 Atsushi Togo , Yuta Inoue , Isao Tanaka