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A finite-temperature many-body perturbation theory is presented that expands in power series the electronic grand potential, chemical potential, internal energy, and entropy on an equal footing. Sum-over-states and sum-over-orbitals…

Chemical Physics · Physics 2020-07-15 So Hirata , Punit K. Jha

A comprehensive and detailed account is presented for the finite-temperature many-body perturbation theory for electrons that expands in power series all thermodynamic functions on an equal footing. Algebraic recursions in the style of the…

Statistical Mechanics · Physics 2021-09-21 So Hirata

Low-order perturbation corrections to the electronic grand potential, internal energy, chemical potential, and entropy of a gas of noninteracting, identical molecules at a nonzero temperature are determined numerically as the…

Chemical Physics · Physics 2019-10-21 Punit K. Jha , So Hirata

A formalism for energy-dependent many-body perturbation theory (MBPT), previously indicated in our recent review articles (Lindgren et al., Phys.Rep. 389,161(2004), Can.J.Phys. 83,183(2005)), is developed in more detail. The formalism…

Quantum Physics · Physics 2009-11-13 Ingvar Lindgren , Sten Salomonson , Daniel Hedendahl

A finite-temperature perturbation theory for the grand canonical ensemble is introduced that expands chemical potential in a perturbation series and conserves the average number of electrons, ensuring charge neutrality of the system at each…

Chemical Physics · Physics 2019-10-21 So Hirata , Punit K. Jha

A unified theory is presented for finite-temperature many-body perturbation expansions of the anharmonic vibrational contributions to thermodynamic functions: the free energy, internal energy, and entropy. The theory is diagrammatically…

Statistical Mechanics · Physics 2023-08-29 Xiuyi Qin , So Hirata

The widely used thermal Hartree-Fock (HF) theory is generalized to include the effect of electron correlation while maintaining its quasi-independent-particle framework. An electron-correlated internal energy (or grand potential) is…

Statistical Mechanics · Physics 2024-08-22 So Hirata

A finite temperature many-particle theory of condensed matter systems is formulated using the functional Schroedinger picture. Using the interacting electron gas as a model system, we solve the equation of motion for the density matrix…

Strongly Correlated Electrons · Physics 2008-02-03 Hyun Sik Noh , Sang Koo You , Chul Koo Kim

We develop a variational approach at finite temperature that incorporates many-body correlation self-consistently. The grand potential is constructed in terms of Green's function expressed by the variational parameters. We apply this…

Quantum Gases · Physics 2019-05-30 Akimitsu Kirikoshi , Wataru Kohno , Takafumi Kita

We present a new algorithm to evaluate the grand potential at finite and high-temperature series expansion via many-body perturbation theory. This algorithm allows us to formulate each order as a divided difference. Further, we apply this…

Strongly Correlated Electrons · Physics 2021-12-30 Mohamed Amine Tag , Abid Boudiar , Mohamed El-Hadi Mansour , Abdelkader Hafdallah , Chafia Bendjeroudib

A simple, but general solution is proposed for the Kohn-Luttinger problem, i.e., the nonconvergence of the finite-temperature many-body perturbation theory with its zero-temperature counterpart as temperature is lowered to zero under some…

Statistical Mechanics · Physics 2022-06-16 So Hirata

Many-body perturbation theory (MBPT) based on Green's functions and Feynman diagrams provides a fundamental theoretical framework for various \emph{ab initio} computational approaches in molecular and materials science, including the random…

Quantum Physics · Physics 2025-03-20 Yuqi Wang , Wei-Hai Fang , Zhendong Li

We investigate the order-by-order convergence behavior of many-body perturbation theory (MBPT) as a simple and efficient tool to approximate the ground-state energy of closed-shell nuclei. To address the convergence properties directly, we…

Nuclear Theory · Physics 2016-04-20 Alexander Tichai , Joachim Langhammer , Sven Binder , Robert Roth

The connection between many-body theory (MBPT)--in perturbative and non-perturbative form--and quantum-electrodynamics (QED) is reviewed for systems of two fermions in an external field. The treatment is mainly based upon the recently…

Quantum Physics · Physics 2009-11-11 Ingvar Lindgren

Many methods for computing electronic correlation effects at finite temperature are related to many-body perturbation theory in the grand-canonical ensemble. In most applications, however, the average number of electrons is known rather…

Materials Science · Physics 2022-10-21 Felix Hummel

This thesis describes several topics related to finite temperature studies of strongly correlated systems: finite temperature density matrix embedding theory (FT-DMET), finite temperature metal-insulator transition, and quantum algorithms…

Strongly Correlated Electrons · Physics 2023-03-01 Chong Sun

It is shown analytically and numerically that the finite-temperature many-body perturbation theory in the grand canonical ensemble has zero radius of convergence at zero temperature when the energy ordering or degree of degeneracy for the…

Chemical Physics · Physics 2021-02-03 So Hirata

A recent description of an exact map for the equilibrium structure and thermodynamics of a quantum system onto a corresponding classical system is summarized. Approximate implementations are constructed by pinning exact limits (ideal gas,…

Statistical Mechanics · Physics 2015-04-14 Jeffrey Wrighton , James Dufty , Sandipan Dutta

Treating electron correlation more accurately and efficiently is at the heart of the development of electronic structure methods. In the present work, we explore the use of stochastic approaches to evaluate high-order electron correlation…

Chemical Physics · Physics 2020-01-29 Zhendong Li

Quantum systems of indistinguishable particles are commonly described using the formalism of second quantisation, which relies on the assumption that any admissible quantum state must be either symmetric or anti-symmetric under particle…

Quantum Physics · Physics 2023-07-13 Benjamin Yadin , Benjamin Morris , Kay Brandner
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