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We apply the density matrix expansion (DME) at Hartree-Fock level with long-range chiral effective field theory interactions defined in coordinate space up to next-to-next-to-leading order. We consider chiral potentials both with and…

Nuclear Theory · Physics 2017-05-26 A. Dyhdalo , S. K. Bogner , R. J. Furnstahl

Ab initio wave-function-based methods are employed for the study of quasiparticle energy bands of zinc-blende ZnS, with focus on the Zn 3d "semicore" states. The relative energies of these states with respect to the top of the S 3p valence…

Strongly Correlated Electrons · Physics 2013-07-11 A. Stoyanova , L. Hozoi , P. Fulde , H. Stoll

We propose a multiconfigurational hybrid density-functional theory which rigorously combines a multiconfiguration self-consistent-field calculation with a density-functional approximation based on a linear decomposition of the…

Chemical Physics · Physics 2012-08-20 Kamal Sharkas , Andreas Savin , Hans Jørgen Aa. Jensen , Julien Toulouse

In this systematic density functional theory study, we compare a standard gradient corrected functional (PBE) with a long-range hybrid functional (HSE06), with and without correction for the dispersion forces, relatively to their ability to…

Materials Science · Physics 2026-04-17 Da Chen , Pietro Andreozzi , Giulia Frigerio , Daniele Perilli , Paulo Siani , Cristiana Di Valentin

The collective dynamics in liquid water is an active research topic experimentally, theoretically and via simulations. Here, ab initio molecular dynamics simulations are reported in heavy and ordinary water at temperature 323.15 K, or…

Soft Condensed Matter · Physics 2016-03-24 T. Bryk , A. P. Seitsonen

Defect engineering can improve the linked charge, spin, and lattice behavior of thermoelectric topological insulators. Using density functional theory with spin orbit coupling, we study structural, electronic, optical, thermoelectric,…

Materials Science · Physics 2025-12-15 Muhammad Usman Javed , Sikander Azam , Qaiser Rafiq , Hamdy Khamees Thabet

Electronic properties and atomic structures of W, N, S, W/N, and W/S dopings of anatase TiO_2 have been systematically investigated using the density functional theory (DFT). The exchange and correlation effects have been treated with Heyd,…

Strongly Correlated Electrons · Physics 2012-11-19 Veysel Çelik , Ersen Mete

This paper presents an approach for obtaining accurate interaction energies at the DFT level for systems where dispersion interactions are important. This approach combines Becke and Johnson's [J. Chem. Phys. 127, 154108 (2007)] method for…

The electronic and magnetic properties of the hexanuclear ferric wheel [LiFe6(OCH3)12-(dbm)6]PF6 have been studied with all-electron Hartree-Fock and full-potential density functional calculations. The best agreement for the magnetic…

Other Condensed Matter · Physics 2007-05-23 H. Nieber , K. Doll , G. Zwicknagl

Photoabsorption in the low-energy region for C$_{60}$ and PTCDA molecular complexes is studied within linear response TDDFT. For the PBE, B3LYP and HSE exchange-correlation (xc) functionals the dependence of the accuracy of the exciton…

Mesoscale and Nanoscale Physics · Physics 2026-04-16 N. L. Matsko , Mahmoud A. Salem

The ab initio computational method known as Hubbard-corrected density functional theory (DFT+$U$) captures well ground electronic structures of a set of solids that are poorly described by standard DFT alone. Since lattice dynamical…

Materials Science · Physics 2025-06-17 Wooil Yang , Sabyasachi Tiwari , Feliciano Giustino , Young-Woo Son

While the exact total energy of a separated open system varies linearly as a function of average electron number between adjacent integers, the energy predicted by semi-local density functional approximations curves upward and the…

Range-separated methods combining a short-range density functional with long-range random phase approximations RPAs with or without exchange response kernel are tested on rare-gas dimers and the S22 benchmark set of weakly interacting…

Chemical Physics · Physics 2014-04-10 Wuming Zhu , Julien Toulouse , Andreas Savin , János G. Angyán

The construction of meta generalized gradient approximations based on the density matrix expansion (DME) is considered as one of the most accurate technique to design semilocal exchange energy functionals in two-dimensional density…

Materials Science · Physics 2018-05-09 Abhilash Patra , Subrata Jana , Prasanjit Samal

We present the WCCR10 data set of ten ligand dissociation energies of large cationic transition metal complexes for the assessment of approximate exchange--correlation functionals. We analyze nine popular functionals, namely BP86, BP86-D3,…

Chemical Physics · Physics 2014-09-30 Thomas Weymuth , Erik P. A. Couzijn , Peter Chen , Markus Reiher

The LMTO method based on the density-functional theory and the semi-empirical INDO method based on the Hartree--Fock formalism are used for the supercell study of the F centers in cubic and orthorhombic ferroelectric KNbO3 crystals. Two…

Materials Science · Physics 2009-10-31 R. I. Eglitis , E. A. Kotomin , A. V. Postnikov , N. E. Christensen , G. Borstel

We present an efficient implementation of the PBE0 hybrid functional within the full-potential linearized augmented-plane-wave (FLAPW) method. The Hartree-Fock exchange term, which is a central ingredient of hybrid functionals, gives rise…

Materials Science · Physics 2010-05-28 Markus Betzinger , Christoph Friedrich , Stefan Blügel

Energy barriers, which control the rates of chemical reactions, are seriously underestimated by computationally-efficient semi-local approximations for the exchange-correlation energy. The accuracy of a semi-local density functional…

Chemical Physics · Physics 2023-11-06 Bikash Kanungo , Aaron D. Kaplan , Chandra Shahi , Vikram Gavini , John P. Perdew

In the present work we investigate the adequacy of broken-symmetry unrestricted density functional theory (DFT) for constructing the potential energy curve of nickel dimer and nickel hydride, as a model for larger bare and hydrogenated…

Chemical Physics · Physics 2007-05-23 Cristian V. Diaconu , Art E. Cho , J. D. Doll , David L. Freeman

We present an effective field theory (EFT) framework for coupled-channel $B^{(*)}\bar D^{(*)}$ scattering, applying it to recent lattice QCD results by Alexandrou et al. [Phys. Rev. Lett. 132, 151902 (2024)]. Two complementary EFT…

High Energy Physics - Phenomenology · Physics 2026-02-03 Michael Abolnikov , Lu Meng , Vadim Baru , Evgeny Epelbaum , Arseniy A. Filin , Ashot M. Gasparyan
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